Reconstructing PM2.5 Data Record for the Kathmandu Valley Using a Machine Learning Model

• Published in: Atmosphere Vol. 14; no. 7; p. 1073
• Main Authors: Bhatta, Surendra, Yang, Yuekui
• Format: Journal Article
• Language: English
• Published: Goddard Space Flight Center MPDI 01-07-2023; MDPI AG
• Subjects: Aerosols; Air pollution; Air quality; Air quality standards; Atmospheric pressure; Carbon; Dust; Earth Resources and Remote Sensing; Geosciences (General); Kathmandu Valley; Kilns; Learning algorithms; Machine learning; Meteorological data; Meteorology and Climatology; Modelling; Monsoons; Nitrous oxide; Outdoor air quality; Ozone; Particulate emissions; Particulate matter; Pollutants; reconstructed historical PM2.5; Root-mean-square errors; Suspended particulate matter; Trends; Valleys; Nepal; Machine Learning; Kathmandu Valley; Reconstructed Historical Pm2.5
• ISSN: 2073-4433; 2073-4433
• DOI: 10.3390/atmos14071073

This paper presents a method for reconstructing the historical hourly concentrations of particulate matter 2.5 (PM2.5) over the Kathmandu Valley from 1980 to the present. The method uses a machine learning model that is trained using PM2.5 readings from US Embassy (Phora Durbar) as a ground truth, and the meteorological data from Modern-Era Retrospective Analysis for Research and Applications v2 (MERRA2) as input. The Extreme Gradient Boosting (XGBoost) model acquires a credible 10-fold cross-validation (CV) score of ~83.4%, an r2-score of ~84%, a Root Mean Square Error (RMSE) of ~15.82 µg/m3, and a Mean Absolute Error (MAE) of ~10.27 µg/m3. Further demonstrating the model's applicability to years other than those for which truth values are unavailable, the multiple cross-test with an unseen data set offered r2-scores for 2018, 2019, and 2020 ranging from 56% to 67%. The model-predicted data agrees with true values and indicates that MERRA2 underestimates PM2.5 over the region. It strongly agrees with ground-based evidence showing substantially higher mass concentrations in the dry pre- and post-monsoon seasons than in the monsoon months. It also shows a strong anti-correlation between PM2.5 concentration and humidity. The results also demonstrate that none of the years fulfilled the annual mean air quality index (AQI) standards set by the World Health Organization (WHO).