Self-Motility of an Active Particle Induced by Correlations in the Surrounding Solution

Self-Motility of an Active Particle Induced by Correlations in the Surrounding Solution

Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative mechanism, in which a diffuse interface emerges solely due to a nonvanishing correlation length of the surrounding solution. This mechani...

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Published in:Physical review letters Vol. 125; no. 26; p. 268002
Main Authors: Domínguez, Alvaro, Popescu, M N, Rohwer, C M, Dietrich, S
Format: Journal Article
Language:English
Published: United States American Physical Society 31-12-2020
Subjects:
Correlation
Micrometers
Motility
Phenomenology
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Abstract Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative mechanism, in which a diffuse interface emerges solely due to a nonvanishing correlation length of the surrounding solution. This mechanism can drive self-motility of a chemically active particle. Numerical estimates indicate that the velocity can reach micrometers per second. The predicted phenomenology includes a bilinear dependence of the velocity on the activity and a possible double velocity reversal upon varying the correlation length.
AbstractList Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative mechanism, in which a diffuse interface emerges solely due to a nonvanishing correlation length of the surrounding solution. This mechanism can drive self-motility of a chemically active particle. Numerical estimates indicate that the velocity can reach micrometers per second. The predicted phenomenology includes a bilinear dependence of the velocity on the activity and a possible double velocity reversal upon varying the correlation length.
ArticleNumber 268002
Author Rohwer, C M
Domínguez, Alvaro
Dietrich, S
Popescu, M N
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  organization: Department of Mathematics & Applied Mathematics, University of Cape Town, 7701 Rondebosch, Cape Town, South Africa
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  surname: Dietrich
  fullname: Dietrich, S
  organization: IV. Institut für Theoretische Physik, Universität Stuttgart, Pfaffenwaldring 57, D-70569 Stuttgart, Germany
BackLink https://www.ncbi.nlm.nih.gov/pubmed/33449719$$D View this record in MEDLINE/PubMed
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Snippet Current models of phoretic transport rely on molecular forces creating a "diffuse" particle-fluid interface. We investigate theoretically an alternative...
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SubjectTerms Correlation
Micrometers
Motility
Phenomenology
Title Self-Motility of an Active Particle Induced by Correlations in the Surrounding Solution
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