Dynamic properties of the electric double layer in electrolytes
The aim of this paper is to numerically investigate the characteristics of the Electrical Double Layer in electrolytes. The surface adsorption is neglected, which means there is no electric current injected to the solution from the electrode. The analysis is done for a one-dimensional model as the D...
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| Published in: | Journal of electrostatics Vol. 71; no. 5; pp. 829 - 838 |
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01-10-2013
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| Abstract | The aim of this paper is to numerically investigate the characteristics of the Electrical Double Layer in electrolytes. The surface adsorption is neglected, which means there is no electric current injected to the solution from the electrode. The analysis is done for a one-dimensional model as the Debye length for electrolytes is much smaller than other dimensions of the system. The discussion is focused on the behaviour of the electric current and the layer impedance at different frequencies of the supply voltage.
•Numerical model for simulating transient process in electrical double layer.•Dynamics of electric potential and space charge formation for the step voltage.•Impedance calculation for sinusoidal excitation.•Effect of the voltage level on current distortion.•Effect of voltage, solution concentration on the layer impedance. |
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| AbstractList | The aim of this paper is to numerically investigate the characteristics of the Electrical Double Layer in electrolytes. The surface adsorption is neglected, which means there is no electric current injected to the solution from the electrode. The analysis is done for a one-dimensional model as the Debye length for electrolytes is much smaller than other dimensions of the system. The discussion is focused on the behaviour of the electric current and the layer impedance at different frequencies of the supply voltage.
•Numerical model for simulating transient process in electrical double layer.•Dynamics of electric potential and space charge formation for the step voltage.•Impedance calculation for sinusoidal excitation.•Effect of the voltage level on current distortion.•Effect of voltage, solution concentration on the layer impedance. The aim of this paper is to numerically investigate the characteristics of the Electrical Double Layer in electrolytes. The surface adsorption is neglected, which means there is no electric current injected to the solution from the electrode. The analysis is done for a one-dimensional model as the Debye length for electrolytes is much smaller than other dimensions of the system. The discussion is focused on the behaviour of the electric current and the layer impedance at different frequencies of the supply voltage. |
| Author | Hossain, Roksana Adamiak, Kazimierz |
| Author_xml | – sequence: 1 givenname: Roksana surname: Hossain fullname: Hossain, Roksana email: rhossain@ucalgary.ca organization: University of Calgary, Department of Electrical and Computer Engineering, Calgary, Alberta T2N 1N4, Canada – sequence: 2 givenname: Kazimierz surname: Adamiak fullname: Adamiak, Kazimierz email: kadamiak@eng.uwo.ca organization: University of Western Ontario, Department of Electrical and Computer Engineering, London, Ontario N6A 5B9, Canada |
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| Cites_doi | 10.1016/j.jcis.2006.08.049 10.1006/jcis.2001.7651 10.1088/0022-3727/39/5/007 10.1103/PhysRevE.61.4019 10.1039/b608092h 10.1103/PhysRevE.70.021506 10.1006/jcis.2000.7125 10.1016/j.jcis.2005.05.037 10.1109/TIA.2010.2074170 10.1016/j.jcis.2007.10.056 10.1146/annurev.fluid.36.050802.122124 10.1109/TIA.2010.2057394 10.1039/f29827800457 10.1007/s10800-009-9966-3 10.1016/j.mee.2009.01.045 10.1016/S0378-7753(96)80014-0 10.1103/PhysRevE.67.056302 10.1006/jcis.2000.7126 10.1039/b403341h 10.1006/jcis.1999.6346 10.1006/jcis.1995.1131 |
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| Keywords | Electrolytes Numerical simulation Charge transport Electric field Electroosmosis |
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| SubjectTerms | Charge transport Double layer Electric current Electric double layer Electric field Electrodes Electrolytes Electroosmosis Mathematical models Numerical simulation Surface chemistry Voltage |
| Title | Dynamic properties of the electric double layer in electrolytes |
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