Conducting and stretchable emulsion styrene butadiene rubber composites using SiO2@Ag core-shell particles and polydopamine coated carbon nanotubes
In the present scenario of development in technology, the applications of stretchable conductive elastomers in modern electronic equipments have aroused great interest. Non-covalent bonding modification of carbon nanotubes (CNTs) using dopamine has improved the dispersion of CNT@PDA and interfacial...
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| Published in: | Polymer testing Vol. 115; p. 107722 |
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| Main Authors: | , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Ltd
01-11-2022
Elsevier |
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| Abstract | In the present scenario of development in technology, the applications of stretchable conductive elastomers in modern electronic equipments have aroused great interest. Non-covalent bonding modification of carbon nanotubes (CNTs) using dopamine has improved the dispersion of CNT@PDA and interfacial interaction with the rubber matrix. The SiO2@Ag core-shell particles were prepared by coated with silver nanoparticles (AgNPs) on the surface of SiO2 using dopamine oxidation self-polymerization and electroless plating process. ESBR composites were prepared by latex co-coagulation method, where CNT@PDA and SiO2@Ag were used to develop an 1D-3D synergistic conductive network in ESBR composites. One-dimensional (1D) CNT@PDA were incorporated in three-dimensional (3D) spherical SiO2@Ag core-shell particles, which effectively prevented the agglomeration of SiO2@Ag and CNT@PDA. Again, 1D CNT@PDA could also be used as bridges to interact with 3D SiO2@Ag to develop the charge transfer more effectively in ESBR composites. The optimum electrical conductivity of the ESBR/CNT@PDA/SiO2@Ag composites was 0.2 S/cm, which was found to be higher than that of single filler. Moreover, the high electrical conductivity can be controlled at low tensile strain. The mechanical property of ESBR/CNT@PDA/SiO2@Ag composite was also improved by 105.4% as compared by ESBR/CNTs. This work provides a new idea for the fabrication of stretchable conductive elastomer composites with high performance.
•SiO2@Ag core-shell particles were prepared by dopamine oxidation self-polymerization and electroless plating process.•PDA was used to modify CNTs by non-covalent binding interaction.•CNT@PDA and SiO2@Ag were used to develop an 1D-3D synergistic conductive network.•The high electrical conductivity can be maintained at low tensile strain. |
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| AbstractList | In the present scenario of development in technology, the applications of stretchable conductive elastomers in modern electronic equipments have aroused great interest. Non-covalent bonding modification of carbon nanotubes (CNTs) using dopamine has improved the dispersion of CNT@PDA and interfacial interaction with the rubber matrix. The SiO2@Ag core-shell particles were prepared by coated with silver nanoparticles (AgNPs) on the surface of SiO2 using dopamine oxidation self-polymerization and electroless plating process. ESBR composites were prepared by latex co-coagulation method, where CNT@PDA and SiO2@Ag were used to develop an 1D-3D synergistic conductive network in ESBR composites. One-dimensional (1D) CNT@PDA were incorporated in three-dimensional (3D) spherical SiO2@Ag core-shell particles, which effectively prevented the agglomeration of SiO2@Ag and CNT@PDA. Again, 1D CNT@PDA could also be used as bridges to interact with 3D SiO2@Ag to develop the charge transfer more effectively in ESBR composites. The optimum electrical conductivity of the ESBR/CNT@PDA/SiO2@Ag composites was 0.2 S/cm, which was found to be higher than that of single filler. Moreover, the high electrical conductivity can be controlled at low tensile strain. The mechanical property of ESBR/CNT@PDA/SiO2@Ag composite was also improved by 105.4% as compared by ESBR/CNTs. This work provides a new idea for the fabrication of stretchable conductive elastomer composites with high performance.
•SiO2@Ag core-shell particles were prepared by dopamine oxidation self-polymerization and electroless plating process.•PDA was used to modify CNTs by non-covalent binding interaction.•CNT@PDA and SiO2@Ag were used to develop an 1D-3D synergistic conductive network.•The high electrical conductivity can be maintained at low tensile strain. In the present scenario of development in technology, the applications of stretchable conductive elastomers in modern electronic equipments have aroused great interest. Non-covalent bonding modification of carbon nanotubes (CNTs) using dopamine has improved the dispersion of CNT@PDA and interfacial interaction with the rubber matrix. The SiO2@Ag core-shell particles were prepared by coated with silver nanoparticles (AgNPs) on the surface of SiO2 using dopamine oxidation self-polymerization and electroless plating process. ESBR composites were prepared by latex co-coagulation method, where CNT@PDA and SiO2@Ag were used to develop an 1D-3D synergistic conductive network in ESBR composites. One-dimensional (1D) CNT@PDA were incorporated in three-dimensional (3D) spherical SiO2@Ag core-shell particles, which effectively prevented the agglomeration of SiO2@Ag and CNT@PDA. Again, 1D CNT@PDA could also be used as bridges to interact with 3D SiO2@Ag to develop the charge transfer more effectively in ESBR composites. The optimum electrical conductivity of the ESBR/CNT@PDA/SiO2@Ag composites was 0.2 S/cm, which was found to be higher than that of single filler. Moreover, the high electrical conductivity can be controlled at low tensile strain. The mechanical property of ESBR/CNT@PDA/SiO2@Ag composite was also improved by 105.4% as compared by ESBR/CNTs. This work provides a new idea for the fabrication of stretchable conductive elastomer composites with high performance. |
| ArticleNumber | 107722 |
| Author | Borah, Jyotishmoy Liu, Fumin Li, Qiao Jing, Yuan Zhang, Su Wang, Haitong Lin, Guangyi |
| Author_xml | – sequence: 1 givenname: Qiao orcidid: 0000-0001-8797-8607 surname: Li fullname: Li, Qiao organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao, 266061, PR China – sequence: 2 givenname: Guangyi surname: Lin fullname: Lin, Guangyi organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao, 266061, PR China – sequence: 3 givenname: Su surname: Zhang fullname: Zhang, Su organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao, 266061, PR China – sequence: 4 givenname: Haitong surname: Wang fullname: Wang, Haitong organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao, 266061, PR China – sequence: 5 givenname: Jyotishmoy surname: Borah fullname: Borah, Jyotishmoy organization: B.B. Engineering College, Kokrajhar, Assam, 783370, India – sequence: 6 givenname: Yuan surname: Jing fullname: Jing, Yuan organization: Qingdao University of Science and Technology Guangrao Rubber Industry Research Institute, Dongying, 257029, PR China – sequence: 7 givenname: Fumin surname: Liu fullname: Liu, Fumin email: liufumin@qust.edu.cn organization: College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao, 266061, PR China |
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| Keywords | Electrical conductivity Poly-dopamine Core-shell particles Conductive elastomer composites |
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| Title | Conducting and stretchable emulsion styrene butadiene rubber composites using SiO2@Ag core-shell particles and polydopamine coated carbon nanotubes |
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