Bulk and surface band structure of the new family of semiconductors BiTeX (X=I, Br, Cl)
•We provide an ARPES comparison between the three tellurohalides BiTeX (X=I, Br, Cl).•They present a similar band structure with namely spin-split bulk and surface states.•They offer, except for BiTeCl, the possibility of ambipolar conduction.•They can be easily doped.•From the data appeared so far,...
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| Published in: | Journal of electron spectroscopy and related phenomena Vol. 201; no. C; pp. 115 - 120 |
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| Main Authors: | , , , , , , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier B.V
01-05-2015
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| Abstract | •We provide an ARPES comparison between the three tellurohalides BiTeX (X=I, Br, Cl).•They present a similar band structure with namely spin-split bulk and surface states.•They offer, except for BiTeCl, the possibility of ambipolar conduction.•They can be easily doped.•From the data appeared so far, BiTeBr may be the most appealing for applications.
We present an overview of the new family of semiconductors BiTeX (X=I, Br, Cl) from the perspective of angle resolved photoemission spectroscopy. The strong band bending occurring at the surface potentially endows them with a large flexibility, as they are capable of hosting both hole and electron conduction, and can be modified by inclusion or adsorption of foreign atoms. In addition, their trigonal crystal structure lacks a center of symmetry and allows for both bulk and surface spin-split bands at the Fermi level. We elucidate analogies and differences among the three materials, also in the light of recent theoretical and experimental work. |
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| AbstractList | •We provide an ARPES comparison between the three tellurohalides BiTeX (X=I, Br, Cl).•They present a similar band structure with namely spin-split bulk and surface states.•They offer, except for BiTeCl, the possibility of ambipolar conduction.•They can be easily doped.•From the data appeared so far, BiTeBr may be the most appealing for applications.
We present an overview of the new family of semiconductors BiTeX (X=I, Br, Cl) from the perspective of angle resolved photoemission spectroscopy. The strong band bending occurring at the surface potentially endows them with a large flexibility, as they are capable of hosting both hole and electron conduction, and can be modified by inclusion or adsorption of foreign atoms. In addition, their trigonal crystal structure lacks a center of symmetry and allows for both bulk and surface spin-split bands at the Fermi level. We elucidate analogies and differences among the three materials, also in the light of recent theoretical and experimental work. |
| Author | Denlinger, J. Rotenberg, E. Kim, K.S. Bugnon, Ph Autès, G. Johannsen, J.C. Bostwick, A. Berger, H. Moser, S. Yazyev, O.V. Crepaldi, A. Grioni, M. Magrez, A. Moreschini, L. |
| Author_xml | – sequence: 1 givenname: L. surname: Moreschini fullname: Moreschini, L. email: lmoreschini@lbl.gov organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 2 givenname: G. surname: Autès fullname: Autès, G. organization: Institute of Theoretical Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 3 givenname: A. surname: Crepaldi fullname: Crepaldi, A. organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 4 givenname: S. surname: Moser fullname: Moser, S. organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 5 givenname: J.C. surname: Johannsen fullname: Johannsen, J.C. organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 6 givenname: K.S. surname: Kim fullname: Kim, K.S. organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 7 givenname: H. surname: Berger fullname: Berger, H. organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 8 givenname: Ph surname: Bugnon fullname: Bugnon, Ph organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 9 givenname: A. surname: Magrez fullname: Magrez, A. organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 10 givenname: J. surname: Denlinger fullname: Denlinger, J. organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 11 givenname: E. surname: Rotenberg fullname: Rotenberg, E. organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 12 givenname: A. surname: Bostwick fullname: Bostwick, A. organization: Advanced Light Source (ALS), Lawrence Berkeley National Laboratory, Berkeley, CA 94720, USA – sequence: 13 givenname: O.V. surname: Yazyev fullname: Yazyev, O.V. organization: Institute of Theoretical Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland – sequence: 14 givenname: M. surname: Grioni fullname: Grioni, M. organization: Institute of Condensed Matter Physics, Ecole Polytechnique Fédérale de Lausanne (EPFL), CH-1015 Lausanne, Switzerland |
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| Copyright | 2014 Elsevier B.V. |
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| Keywords | Angle-resolved photoemission Spin–orbit splitting Tellurohalides Rashba states |
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| SubjectTerms | Angle-resolved photoemission Rashba states Spin–orbit splitting Tellurohalides |
| Title | Bulk and surface band structure of the new family of semiconductors BiTeX (X=I, Br, Cl) |
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