Nanovolume positron traps in glassy-like As2Se3

A meaningful interpretation of positron lifetime characteristics for glassy-like g-As2Se3 is developed taking into account theoretical calculations of Jensen et al. [J. Non-Cryst. Solids 170 (1994) 57] for positrons trapped by so-called free-volume vacancy-type defects (vacancies and vacancy-type cl...

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Published in:Journal of non-crystalline solids Vol. 351; no. 12-13; pp. 1077 - 1081
Main Authors: Kozdras, A., Filipecki, J., Hyla, M., Shpotyuk, O., Kovalskiy, A., Szymura, S.
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Published: Amsterdam Elsevier B.V 01-05-2005
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Abstract A meaningful interpretation of positron lifetime characteristics for glassy-like g-As2Se3 is developed taking into account theoretical calculations of Jensen et al. [J. Non-Cryst. Solids 170 (1994) 57] for positrons trapped by so-called free-volume vacancy-type defects (vacancies and vacancy-type clusters) in orthorhombic As2Se3 and void volume distribution for 146-atoms layer-biased and random computer models of amorphous As2Se3 performed by Popescu yet in 1980. It is concluded that the obtained experimental data can be divided into two groups with close lifetime characteristics but different positron trapping coefficients. This feature can be well explained in terms of average positron lifetime by applying two-state positron trapping model for mathematical treatment of the experimental data.
AbstractList A meaningful interpretation of positron lifetime characteristics for glassy--like g--As2Se3 is developed taking into account theoretical calculations of Jensen et al. [J. Non--Cryst. Solids 170 (1994) 57] for positrons trapped by so--called free--volume vacancy--type defects (vacancies and vacancy--type clusters) in orthorhombic As2Se3 and void volume distribution for 146--atoms layer--biased and random computer models of amorphous As2Se3 performed by Popescu yet in 1980. It is concluded that the obtained experimental data can be divided into two groups with close lifetime characteristics but different positron trapping coefficients. This feature can be well explained in terms of average positron lifetime by applying two--state positron trapping model for mathematical treatment of the experimental data.
Author Filipecki, J.
Shpotyuk, O.
Szymura, S.
Kovalskiy, A.
Hyla, M.
Kozdras, A.
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  surname: Szymura
  fullname: Szymura, S.
  organization: Physics Laboratory of Opole Technical University, 75, ul. Ozimska, Opole, 45370, Poland
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Cites_doi 10.1103/PhysRevB.7.5237
10.1002/pssa.2210480261
10.1016/0022-3093(80)90652-3
10.1016/0168-9002(96)00075-7
10.1016/0022-3093(94)90103-1
10.1002/pssa.2210600258
10.1103/PhysRevB.41.9980
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Issue 12-13
Keywords C145
61.80.Ed
78.70.Bj
S440
61.82.Ms
P305
Vacancies
Glass
Free volume
Vacancy cluster
Positron annihilation
Amorphous state
Defects
Voids
Lifetime
Trapping
Positron attachment
Mathematical models
Positron states
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Snippet A meaningful interpretation of positron lifetime characteristics for glassy-like g-As2Se3 is developed taking into account theoretical calculations of Jensen...
A meaningful interpretation of positron lifetime characteristics for glassy--like g--As2Se3 is developed taking into account theoretical calculations of Jensen...
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SubjectTerms Condensed matter: electronic structure, electrical, magnetic, and optical properties
Exact sciences and technology
Optical properties and condensed-matter spectroscopy and other interactions of matter with particles and radiation
Other interactions of matter with particles and radiation
Physics
Positron annihilation
Title Nanovolume positron traps in glassy-like As2Se3
URI https://dx.doi.org/10.1016/j.jnoncrysol.2005.01.031
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