An improved model for the corrosion of used nuclear fuel inside a failed waste container under permanent disposal conditions
[Display omitted] •The corrosion of spent nuclear fuel in a failed waste container is modelled.•Alpha-radiolysis process is simulated using a full reaction set.•Corrosion of UO2 is largely influenced by steel corrosion products, Fe2+ and H2.•H2 concentrations required to completely suppress fuel cor...
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| Published in: | Corrosion science Vol. 84; pp. 85 - 95 |
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| Abstract | [Display omitted]
•The corrosion of spent nuclear fuel in a failed waste container is modelled.•Alpha-radiolysis process is simulated using a full reaction set.•Corrosion of UO2 is largely influenced by steel corrosion products, Fe2+ and H2.•H2 concentrations required to completely suppress fuel corrosion are calculated.•Influences of burnup and fuel age are examined.
An improved model for nuclear fuel corrosion inside a failed waste container has been developed. The model considers the influence of the α-radiolysis products using a full radiolytic reaction set, and demonstrates that H2O2 is the dominant oxidant. Corrosion of the fuel is modelled considering both the direct oxidation of UO2 by H2O2 and the galvanically-coupled oxidation by H2O2 reduction on noble metal (ε) particles. Corrosion has been found to be very sensitive to the corrosion products of steel container, Fe2+ and H2. The surface coverage of ε-particles can significantly influence the dissolution rate. |
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| AbstractList | [Display omitted]
•The corrosion of spent nuclear fuel in a failed waste container is modelled.•Alpha-radiolysis process is simulated using a full reaction set.•Corrosion of UO2 is largely influenced by steel corrosion products, Fe2+ and H2.•H2 concentrations required to completely suppress fuel corrosion are calculated.•Influences of burnup and fuel age are examined.
An improved model for nuclear fuel corrosion inside a failed waste container has been developed. The model considers the influence of the α-radiolysis products using a full radiolytic reaction set, and demonstrates that H2O2 is the dominant oxidant. Corrosion of the fuel is modelled considering both the direct oxidation of UO2 by H2O2 and the galvanically-coupled oxidation by H2O2 reduction on noble metal (ε) particles. Corrosion has been found to be very sensitive to the corrosion products of steel container, Fe2+ and H2. The surface coverage of ε-particles can significantly influence the dissolution rate. |
| Author | Wu, Linda Shoesmith, David W. Qin, Zack |
| Author_xml | – sequence: 1 givenname: Linda surname: Wu fullname: Wu, Linda organization: Department of Chemistry, The University of Western Ontario, London, ON N6A 5B7, Canada – sequence: 2 givenname: Zack surname: Qin fullname: Qin, Zack organization: Department of Chemistry, The University of Western Ontario, London, ON N6A 5B7, Canada – sequence: 3 givenname: David W. surname: Shoesmith fullname: Shoesmith, David W. email: dwshoesm@uwo.ca organization: Department of Chemistry, The University of Western Ontario, London, ON N6A 5B7, Canada |
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| Keywords | A. Carbon steel C. Interfaces B. Modelling studies C. Anodic dissolution Radioactive waste Electrochemical corrosion Nuclear fuel Waste disposal Modeling Container Storage Anodic dissolution Carbon steel Application Interface |
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| SubjectTerms | A. Carbon steel Applied sciences B. Modelling studies C. Anodic dissolution C. Interfaces Corrosion Corrosion environments Exact sciences and technology Metals. Metallurgy |
| Title | An improved model for the corrosion of used nuclear fuel inside a failed waste container under permanent disposal conditions |
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