Initiation of copper dissolution in sodium chloride electrolytes
Initial stages of copper activation in chloride-ion containing neutral aqueous solution were studied. The results point that activation of copper passivity is initiated once the potential exceeds the breakdown value, occurring with well-defined incubation period, similar to that of other passive met...
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| Published in: | Electrochimica acta Vol. 51; no. 26; pp. 5660 - 5668 |
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| Language: | English |
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15-08-2006
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| Abstract | Initial stages of copper activation in chloride-ion containing neutral aqueous solution were studied. The results point that activation of copper passivity is initiated once the potential exceeds the breakdown value, occurring with well-defined incubation period, similar to that of other passive metals in chloride environments. The effect of applied potential and Cl
− ion concentration on the incubation period is presented. The results indicate that an incubation period for copper activation in chloride containing solutions can be associated with the formation of a two-dimensional CuCl layer on the metal surface. The incubation period is relatively long at negative potentials and it is decreases with a positive shift in the potential. At a certain potential, the incubation period is sharply decreased. The time-frame of incubation period is attributed to the formation rate of two-dimensional CuCl layer and its reduction rate. The formation of a stable salt film on the metal surface facilitates localized rapid dissolution of the copper. |
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| AbstractList | Initial stages of copper activation in chloride-ion containing neutral aqueous solution were studied. The results point that activation of copper passivity is initiated once the potential exceeds the breakdown value, occurring with well-defined incubation period, similar to that of other passive metals in chloride environments. The effect of applied potential and Cl
− ion concentration on the incubation period is presented. The results indicate that an incubation period for copper activation in chloride containing solutions can be associated with the formation of a two-dimensional CuCl layer on the metal surface. The incubation period is relatively long at negative potentials and it is decreases with a positive shift in the potential. At a certain potential, the incubation period is sharply decreased. The time-frame of incubation period is attributed to the formation rate of two-dimensional CuCl layer and its reduction rate. The formation of a stable salt film on the metal surface facilitates localized rapid dissolution of the copper. Initial stages of copper activation in chloride-ion containing neutral aqueous solution were studied. The results point that activation of copper passivity is initiated once the potential exceeds the breakdown value, occurring with well-defined incubation period, similar to that of other passive metals in chloride environments. The effect of applied potential and Cl- ion concentration on the incubation period is presented. The results indicate that an incubation period for copper activation in chloride containing solutions can be associated with the formation of a two-dimensional CuCl layer on the metal surface. The incubation period is relatively long at negative potentials and it is decreases with a positive shift in the potential. At a certain potential, the incubation period is sharply decreased. The time-frame of incubation period is attributed to the formation rate of two-dimensional CuCl layer and its reduction rate. The formation of a stable salt film on the metal surface facilitates localized rapid dissolution of the copper. |
| Author | Khaselev, O. Auinat, M. Ein-Eli, Y. Starosvetsky, D. |
| Author_xml | – sequence: 1 givenname: D. surname: Starosvetsky fullname: Starosvetsky, D. email: davstar@tx.technion.ac.il – sequence: 2 givenname: O. surname: Khaselev fullname: Khaselev, O. – sequence: 3 givenname: M. surname: Auinat fullname: Auinat, M. – sequence: 4 givenname: Y. surname: Ein-Eli fullname: Ein-Eli, Y. email: eineli@tx.technion.ac.il |
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| Cites_doi | 10.1007/BF01093751 10.1149/1.2108335 10.1023/B:JACH.0000021873.30314.eb 10.1016/S0039-6028(00)00442-8 10.1149/1.2085397 10.1149/1.1391638 10.1149/1.2408204 10.1016/0010-938X(94)90041-8 10.1016/S0022-0728(03)00115-3 10.1007/BF01007815 10.1149/1.2403477 10.1007/3-540-44817-9_6 10.1016/S0039-6028(96)01461-6 10.1016/0013-4686(95)00108-Q 10.1016/S0010-938X(03)00140-9 10.5006/1.3280429 10.1007/BF01093752 10.1149/1.2127344 10.1016/0013-4686(88)80192-0 10.1016/0013-4686(88)85008-4 10.1016/S0013-4686(97)10121-9 10.1007/s003390051199 10.1021/jp004012i 10.1016/S0010-938X(71)80118-X 10.1016/0010-938X(92)90191-5 10.1016/S0927-7757(97)00315-4 |
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| Keywords | Localized corrosion Incubation period Copper activation Chlorides Passivity breakdown Atomic force microscopy Corrosion mechanism Passivation potential Electrochemical corrosion Sodium chloride Surface structure Corrosion current Electrodissolution Aqueous solution Copper |
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| Snippet | Initial stages of copper activation in chloride-ion containing neutral aqueous solution were studied. The results point that activation of copper passivity is... |
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| SubjectTerms | Applied sciences Chlorides Copper activation Corrosion Corrosion mechanisms Exact sciences and technology Incubation period Localized corrosion Metals. Metallurgy Passivity breakdown |
| Title | Initiation of copper dissolution in sodium chloride electrolytes |
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