Study of inverted planar CH3NH3PbI3 perovskite solar cells fabricated under environmental conditions

•An efficiency of 10% was obtained with the inverted perovskite configuration under ambient condition.•The anti-solvent method was used to fabricated the perovskite film for solar cells.•The morphological, optic and photovoltaic analyses indicate that the right combination of these two parameters. O...

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Published in:	Solar energy Vol. 180; pp. 594 - 600
Main Authors:	Montoya, Marco Polo, Sidhik, Siraj, Esparza, Diego, López-Luke, Tzarara, Zarazua, Isaac, Rivas, Jesús Manuel, De la Rosa, Elder
Format:	Journal Article
Language:	English
Published:	New York Elsevier Ltd 01-03-2019 Pergamon Press Inc
Subjects:	Circuits Crystal growth Crystal structure Current carriers Electronics industry Environmental conditions Fabrication Inverted structure Organic semiconductors Perovskite Perovskites Photovoltaic cells Photovoltaics Pinholes Relative humidity Short circuit currents Solar cells Solar energy Solvents Titanium dioxide Solar cells Perovskite Inverted structure
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Abstract	•An efficiency of 10% was obtained with the inverted perovskite configuration under ambient condition.•The anti-solvent method was used to fabricated the perovskite film for solar cells.•The morphological, optic and photovoltaic analyses indicate that the right combination of these two parameters. Organic-inorganic inverted perovskite solar cells have been analyzed. This structure uses organic semiconductors as electron and hole selective electrodes and the perovskite as light harvesting layer. The anti-solvent deposition method is a frequently used techniques in the elaboration of conventional perovskite solar cells (FTO/TiO2/CH3NH3PbI3/Spiro-OMetad/Au). However, the anti-solvent method is seldom used in the inverted structure. In this work, we use the anti-solvent method to fabricate the perovskite film for solar cells in the ITO/PEDOT:PSS/CH3NH3PbI3/PC61BM/Ag configuration, systematically studying the effect of the anti-solvent dripping time and the relative humidity in cell fabrication and performance. The morphological, optical and photovoltaic analyses indicate that the right combination of these two parameters will result in a preferential crystal growth in the (1 1 0) orientation. This allows the formation of homogeneous pinhole-free films that enhance light harvesting and reduce charge-carrier leakage, hence increasing short circuit current and fill factor to obtain a photo-conversion efficiency of about ∼10%.
AbstractList	Organic-inorganic inverted perovskite solar cells have been analyzed. This structure uses organic semiconductors as electron and hole selective electrodes and the perovskite as light harvesting layer. The anti-solvent deposition method is a frequently used techniques in the elaboration of conventional perovskite solar cells (FTO/TiO2/CH3NH3PbI3/Spiro-OMetad/Au). However, the anti-solvent method is seldom used in the inverted structure. In this work, we use the anti-solvent method to fabricate the perovskite film for solar cells in the ITO/PEDOT:PSS/CH3NH3PbI3/PC61BM/Ag configuration, systematically studying the effect of the anti-solvent dripping time and the relative humidity in cell fabrication and performance. The morphological, optical and photovoltaic analyses indicate that the right combination of these two parameters will result in a preferential crystal growth in the (1 1 0) orientation. This allows the formation of homogeneous pinhole-free films that enhance light harvesting and reduce charge-carrier leakage, hence increasing short circuit current and fill factor to obtain a photo-conversion efficiency of about ∼10%. •An efficiency of 10% was obtained with the inverted perovskite configuration under ambient condition.•The anti-solvent method was used to fabricated the perovskite film for solar cells.•The morphological, optic and photovoltaic analyses indicate that the right combination of these two parameters. Organic-inorganic inverted perovskite solar cells have been analyzed. This structure uses organic semiconductors as electron and hole selective electrodes and the perovskite as light harvesting layer. The anti-solvent deposition method is a frequently used techniques in the elaboration of conventional perovskite solar cells (FTO/TiO2/CH3NH3PbI3/Spiro-OMetad/Au). However, the anti-solvent method is seldom used in the inverted structure. In this work, we use the anti-solvent method to fabricate the perovskite film for solar cells in the ITO/PEDOT:PSS/CH3NH3PbI3/PC61BM/Ag configuration, systematically studying the effect of the anti-solvent dripping time and the relative humidity in cell fabrication and performance. The morphological, optical and photovoltaic analyses indicate that the right combination of these two parameters will result in a preferential crystal growth in the (1 1 0) orientation. This allows the formation of homogeneous pinhole-free films that enhance light harvesting and reduce charge-carrier leakage, hence increasing short circuit current and fill factor to obtain a photo-conversion efficiency of about ∼10%.
Author	Montoya, Marco Polo Sidhik, Siraj De la Rosa, Elder Zarazua, Isaac Esparza, Diego Rivas, Jesús Manuel López-Luke, Tzarara
Author_xml	– sequence: 1 givenname: Marco Polo surname: Montoya fullname: Montoya, Marco Polo organization: Unidad Académica de Ingeniería Eléctrica, Universidad Autónoma de Zacatecas, Av. Ramón López Velarde 801, Zacatecas C.P. 98060, Mexico – sequence: 2 givenname: Siraj surname: Sidhik fullname: Sidhik, Siraj organization: Nanophotonics and Advanced Materials Group, Centro de Investigaciones en Óptica, A.P. 1-948, León, Gunajuato C.P. 37150, Mexico – sequence: 3 givenname: Diego orcidid: 0000-0002-2097-2830 surname: Esparza fullname: Esparza, Diego email: desparza@uaz.edu.mx organization: Unidad Académica de Ingeniería Eléctrica, Universidad Autónoma de Zacatecas, Av. Ramón López Velarde 801, Zacatecas C.P. 98060, Mexico – sequence: 4 givenname: Tzarara surname: López-Luke fullname: López-Luke, Tzarara organization: Nanophotonics and Advanced Materials Group, Centro de Investigaciones en Óptica, A.P. 1-948, León, Gunajuato C.P. 37150, Mexico – sequence: 5 givenname: Isaac surname: Zarazua fullname: Zarazua, Isaac organization: Departamento de Ciencias Exactas y Tecnología, Universidad de Guadalajara, Centro Universitario de Los Lagos, Lagos de Moreno, Jalisco 47460, Mexico – sequence: 6 givenname: Jesús Manuel surname: Rivas fullname: Rivas, Jesús Manuel organization: Unidad Académica de Ingeniería Eléctrica, Universidad Autónoma de Zacatecas, Av. Ramón López Velarde 801, Zacatecas C.P. 98060, Mexico – sequence: 7 givenname: Elder surname: De la Rosa fullname: De la Rosa, Elder organization: Universidad De La Salle Bajio Campus Campestre, León Gto 37150, Mexico
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Snippet	•An efficiency of 10% was obtained with the inverted perovskite configuration under ambient condition.•The anti-solvent method was used to fabricated the... Organic-inorganic inverted perovskite solar cells have been analyzed. This structure uses organic semiconductors as electron and hole selective electrodes and...
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SubjectTerms	Circuits Crystal growth Crystal structure Current carriers Electronics industry Environmental conditions Fabrication Inverted structure Organic semiconductors Perovskite Perovskites Photovoltaic cells Photovoltaics Pinholes Relative humidity Short circuit currents Solar cells Solar energy Solvents Titanium dioxide
Title	Study of inverted planar CH3NH3PbI3 perovskite solar cells fabricated under environmental conditions
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