Application of Binary PdSb/C as an Anode in a Polymeric Electrolyte Reactor-Fuel Cell Type for Electrosynthesis of Methanol from Methane

Application of Binary PdSb/C as an Anode in a Polymeric Electrolyte Reactor-Fuel Cell Type for Electrosynthesis of Methanol from Methane

PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert methane into oxygenated products and energy in mild conditions. The PER-FC polarization curves for Pd90Sb10/C presented maximum current density about 0.92...

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Published in:Materials research (São Carlos, São Paulo, Brazil) Vol. 25; p. 1
Main Authors: Godoi, Camila M., Santos, Monique C.L., Nunes, Livia C., Silva, Araceli J., Ramos, Andrezza S., Souza, Rodrigo F.B. de, O. Neto, Almir
Format: Journal Article
Language:English
Published: Sao Carlos Universidade Federal do Sao Carlos, Departamento de Engenharia de Materiais 01-01-2022
ABM, ABC, ABPol
Associação Brasileira de Metalurgia e Materiais (ABM); Associação Brasileira de Cerâmica (ABC); Associação Brasileira de Polímeros (ABPol)
Subjects:
Anodes
chemical and energy co-generation
Electrode polarization
Electrolytes
ENGINEERING, CHEMICAL
Fuel cells
MATERIALS SCIENCE, MULTIDISCIPLINARY
METALLURGY & METALLURGICAL ENGINEERING
Methane
Methane into methanol
Methanol
Nuclear fuels
Oxidation
polymeric electrolyte reactor - fuel cell type
Qualitative analysis
chemical and energy co-generation
Methane into methanol
polymeric electrolyte reactor - fuel cell type
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Abstract PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert methane into oxygenated products and energy in mild conditions. The PER-FC polarization curves for Pd90Sb10/C presented maximum current density about 0.92 mW cm-2 about 15% higher than PdSb materials. However, the material Pd50Sb50/C showed higher reaction rate for methanol generation than the other materials occurring close to the OCV (r ~ 7 mol L-1 h-1). The qualitative analyses of PER-FC effluent by FT-IR identified products as methanol, carbonate and formate ions from the partial oxidation of methane for all materials.
AbstractList Abstract PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert methane into oxygenated products and energy in mild conditions. The PER-FC polarization curves for Pd90Sb10/C presented maximum current density about 0.92 mW cm-2 about 15% higher than PdSb materials. However, the material Pd50Sb50/C showed higher reaction rate for methanol generation than the other materials occurring close to the OCV (r ~ 7 mol L-1 h-1). The qualitative analyses of PER-FC effluent by FT-IR identified products as methanol, carbonate and formate ions from the partial oxidation of methane for all materials.
PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert methane into oxygenated products and energy in mild conditions. The PER-FC polarization curves for Pd90Sb10/C presented maximum current density about 0.92 mW cm-2 about 15% higher than PdSb materials. However, the material Pd50Sb50/C showed higher reaction rate for methanol generation than the other materials occurring close to the OCV (r ~ 7 mol L-1 h-1). The qualitative analyses of PER-FC effluent by FT-IR identified products as methanol, carbonate and formate ions from the partial oxidation of methane for all materials.
Author Souza, Rodrigo F.B. de
Santos, Monique C.L.
Ramos, Andrezza S.
O. Neto, Almir
Silva, Araceli J.
Nunes, Livia C.
Godoi, Camila M.
AuthorAffiliation Instituto de Pesquisas Energéticas e Nucleares
AuthorAffiliation_xml – name: Instituto de Pesquisas Energéticas e Nucleares
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  givenname: Monique C.L.
  surname: Santos
  fullname: Santos, Monique C.L.
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  givenname: Livia C.
  surname: Nunes
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  givenname: Araceli J.
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  surname: Silva
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  surname: O. Neto
  fullname: O. Neto, Almir
  organization: Instituto de Pesquisas Energéticas e Nucleares, Brasil
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Keywords chemical and energy co-generation
Methane into methanol
polymeric electrolyte reactor - fuel cell type
Language English
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Snippet PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert methane into...
Abstract PdSb catalyst prepared in different compositions were applied as an anode in a polymeric electrolyte reactor - fuel cell type (PER-FC) to convert...
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SubjectTerms Anodes
chemical and energy co-generation
Electrode polarization
Electrolytes
ENGINEERING, CHEMICAL
Fuel cells
MATERIALS SCIENCE, MULTIDISCIPLINARY
METALLURGY & METALLURGICAL ENGINEERING
Methane
Methane into methanol
Methanol
Nuclear fuels
Oxidation
polymeric electrolyte reactor - fuel cell type
Qualitative analysis
Title Application of Binary PdSb/C as an Anode in a Polymeric Electrolyte Reactor-Fuel Cell Type for Electrosynthesis of Methanol from Methane
URI https://www.proquest.com/docview/2666962077
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https://doaj.org/article/fb5b0c1d311944f8b383db86f4d1bc37
Volume 25
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