Crystallization-driven tuneable lasing of perylene doped into the nematic liquid crystal

Crystallization-driven tuneable lasing of perylene doped into the nematic liquid crystal

Versatile devices with tunable capabilities for controlling lasing wavelength and intensity are in high demand. Liquid crystals (LCs) exhibit immense potential for such applications, offering fine-tuning possibilities through external factors. On the other hand, laser technology is currently a resea...

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Published in:Giant (Oxford, England) Vol. 18; p. 100279
Main Authors: Szukalska, Alina, Zak, Andrzej, Chrzumnicka, Ewa, Gibas, Anna, Baszczuk, Agnieszka, Mysliwiec, Jaroslaw
Format: Journal Article
Language:English
Published: Elsevier Ltd 01-06-2024
Elsevier
Subjects:
Crystals
Lasing
Liquid crystals
Organic materials
Perylene
Self-assembly
TEM
Tuneability
Self-assembly
Organic materials
Crystals
Tuneability
Lasing
Perylene
TEM
Liquid crystals
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Abstract Versatile devices with tunable capabilities for controlling lasing wavelength and intensity are in high demand. Liquid crystals (LCs) exhibit immense potential for such applications, offering fine-tuning possibilities through external factors. On the other hand, laser technology is currently a research hotspot in optoelectronics, and also in practical applications. The recent market introduction of laser television marks a significant stride toward making such advanced technology accessible in every household. In synergy with laser pumping, the LCs unquestionably can be rediscovered. This study presents a comprehensive investigation into the crystallization phenomenon within a host-guest device, compact in size, free from moving parts, and integrating the liquid crystalline (LC) matrix doped with 3,4,9,10-tetra-(3-alcoxy-carbonyl)-perylene (THCP) dye. The focus lies in examining the influence of varying dye concentrations on multicolor fluorescence, lasing behavior, and device morphology. The systematic analysis of Random Lasing (RL) energy thresholds and the impact of DC voltage on light intensity modulation is demonstrated. Morphological changes were monitored in real-time using optical microscopy techniques, including crossed polarizer, and fluorescence imaging under 450 nm excitation. Utilizing advanced Transmission Electron Microscopy (TEM) techniques, we explore exceptional insights into our set of devices, providing novel information about the THCP crystallization process for the first time in the literature. To gain a comprehensive understanding of the crystal forming and molecular geometry we examined additionally the THCP dye, using X-ray diffraction and Raman spectroscopy. Furthermore, we showcase that varying the pumping energy enables multicolor tuning in the fabricated systems, presenting an attractive feature in the context of laser display technologies. [Display omitted]
AbstractList Versatile devices with tunable capabilities for controlling lasing wavelength and intensity are in high demand. Liquid crystals (LCs) exhibit immense potential for such applications, offering fine-tuning possibilities through external factors. On the other hand, laser technology is currently a research hotspot in optoelectronics, and also in practical applications. The recent market introduction of laser television marks a significant stride toward making such advanced technology accessible in every household. In synergy with laser pumping, the LCs unquestionably can be rediscovered. This study presents a comprehensive investigation into the crystallization phenomenon within a host-guest device, compact in size, free from moving parts, and integrating the liquid crystalline (LC) matrix doped with 3,4,9,10-tetra-(3-alcoxy-carbonyl)-perylene (THCP) dye. The focus lies in examining the influence of varying dye concentrations on multicolor fluorescence, lasing behavior, and device morphology. The systematic analysis of Random Lasing (RL) energy thresholds and the impact of DC voltage on light intensity modulation is demonstrated. Morphological changes were monitored in real-time using optical microscopy techniques, including crossed polarizer, and fluorescence imaging under 450 nm excitation. Utilizing advanced Transmission Electron Microscopy (TEM) techniques, we explore exceptional insights into our set of devices, providing novel information about the THCP crystallization process for the first time in the literature. To gain a comprehensive understanding of the crystal forming and molecular geometry we examined additionally the THCP dye, using X-ray diffraction and Raman spectroscopy. Furthermore, we showcase that varying the pumping energy enables multicolor tuning in the fabricated systems, presenting an attractive feature in the context of laser display technologies. [Display omitted]
Versatile devices with tunable capabilities for controlling lasing wavelength and intensity are in high demand. Liquid crystals (LCs) exhibit immense potential for such applications, offering fine-tuning possibilities through external factors. On the other hand, laser technology is currently a research hotspot in optoelectronics, and also in practical applications. The recent market introduction of laser television marks a significant stride toward making such advanced technology accessible in every household. In synergy with laser pumping, the LCs unquestionably can be rediscovered. This study presents a comprehensive investigation into the crystallization phenomenon within a host-guest device, compact in size, free from moving parts, and integrating the liquid crystalline (LC) matrix doped with 3,4,9,10-tetra-(3-alcoxy-carbonyl)-perylene (THCP) dye. The focus lies in examining the influence of varying dye concentrations on multicolor fluorescence, lasing behavior, and device morphology. The systematic analysis of Random Lasing (RL) energy thresholds and the impact of DC voltage on light intensity modulation is demonstrated. Morphological changes were monitored in real-time using optical microscopy techniques, including crossed polarizer, and fluorescence imaging under 450 nm excitation. Utilizing advanced Transmission Electron Microscopy (TEM) techniques, we explore exceptional insights into our set of devices, providing novel information about the THCP crystallization process for the first time in the literature. To gain a comprehensive understanding of the crystal forming and molecular geometry we examined additionally the THCP dye, using X-ray diffraction and Raman spectroscopy. Furthermore, we showcase that varying the pumping energy enables multicolor tuning in the fabricated systems, presenting an attractive feature in the context of laser display technologies.
ArticleNumber 100279
Author Baszczuk, Agnieszka
Mysliwiec, Jaroslaw
Szukalska, Alina
Gibas, Anna
Zak, Andrzej
Chrzumnicka, Ewa
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  email: alina.szukalska@pwr.edu.pl
  organization: Wroclaw University of Science and Technology, Faculty of Chemistry, Institute of Advanced Materials, Wyb. Wyspianskiego 27, 50-370 Wroclaw, Poland
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  givenname: Andrzej
  surname: Zak
  fullname: Zak, Andrzej
  organization: Wroclaw University of Science and Technology, Faculty of Chemistry, Institute of Advanced Materials, Wyb. Wyspianskiego 27, 50-370 Wroclaw, Poland
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  givenname: Ewa
  surname: Chrzumnicka
  fullname: Chrzumnicka, Ewa
  organization: Poznan University of Technology, Faculty of Materials Engineering and Technical Physics, Institute of Materials Research and Quantum Engineering, Piotrowo 3, 60-965 Poznan, Poland
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  givenname: Anna
  surname: Gibas
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– sequence: 6
  givenname: Jaroslaw
  surname: Mysliwiec
  fullname: Mysliwiec, Jaroslaw
  organization: Wroclaw University of Science and Technology, Faculty of Chemistry, Institute of Advanced Materials, Wyb. Wyspianskiego 27, 50-370 Wroclaw, Poland
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Keywords Self-assembly
Organic materials
Crystals
Tuneability
Lasing
Perylene
TEM
Liquid crystals
Language English
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SSID ssj0002810812
Score 2.3088937
Snippet Versatile devices with tunable capabilities for controlling lasing wavelength and intensity are in high demand. Liquid crystals (LCs) exhibit immense potential...
SourceID doaj
crossref
elsevier
SourceType Open Website
Aggregation Database
Publisher
StartPage 100279
SubjectTerms Crystals
Lasing
Liquid crystals
Organic materials
Perylene
Self-assembly
TEM
Tuneability
Title Crystallization-driven tuneable lasing of perylene doped into the nematic liquid crystal
URI https://dx.doi.org/10.1016/j.giant.2024.100279
https://doaj.org/article/a8ef152a5e1446c3b84f12db61009c6c
Volume 18
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