Comparative study of the heat capacity of icosahedral quasicrystals in solid and liquid states
The heat capacity of icosahedral quasicrystals Al 63 Cu 25 Fe 12 and Al 62 Cu 25.5 Fe 12.5 has been studied at high temperatures up to 1700 K, which is by almost 400 K higher than the melting point of the material. It has been shown that the melt exhibits an excess heat capacity with respect to that...
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| Published in: | Physics of the solid state Vol. 53; no. 10; pp. 1987 - 1990 |
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| Format: | Journal Article |
| Language: | English |
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| Abstract | The heat capacity of icosahedral quasicrystals Al
63
Cu
25
Fe
12
and Al
62
Cu
25.5
Fe
12.5
has been studied at high temperatures up to 1700 K, which is by almost 400 K higher than the melting point of the material. It has been shown that the melt exhibits an excess heat capacity with respect to that determined by the Dulong-Petit law and that is a direct extension of the excess heat capacity of the solid state. It has been concluded that the excess heat capacity is related, as a whole, to the short-range order in the quasicrystal structure. This circumstance allows the identification of the orbital hybridization as the most probable mechanism of formation of the pseudogap in the electronic structure of the quasicrystals. |
|---|---|
| AbstractList | The heat capacity of icosahedral quasicrystals [Al.sub.63][Cu.sub.25][Fe.sub.12] and [Al.sub.62][Cu.sub.25.5][Fe.sub.12.5] has been studied at high temperatures up to 1700 K, which is by almost 400 K higher than the melting point of the material. It has been shown that the melt exhibits an excess heat capacity with respect to that determined by the Dulong-Petit law and that is a direct extension of the excess heat capacity of the solid state. It has been concluded that the excess heat capacity is related, as a whole, to the short-range order in the quasicrystal structure. This circumstance allows the identification of the orbital hybridization as the most probable mechanism of formation of the pseudogap in the electronic structure of the quasicrystals. The heat capacity of icosahedral quasicrystals [Al.sub.63][Cu.sub.25][Fe.sub.12] and [Al.sub.62][Cu.sub.25.5][Fe.sub.12.5] has been studied at high temperatures up to 1700 K, which is by almost 400 K higher than the melting point of the material. It has been shown that the melt exhibits an excess heat capacity with respect to that determined by the Dulong-Petit law and that is a direct extension of the excess heat capacity of the solid state. It has been concluded that the excess heat capacity is related, as a whole, to the short-range order in the quasicrystal structure. This circumstance allows the identification of the orbital hybridization as the most probable mechanism of formation of the pseudogap in the electronic structure of the quasicrystals. DOI: 10.1134/S1063783411100246 The heat capacity of icosahedral quasicrystals Al 63 Cu 25 Fe 12 and Al 62 Cu 25.5 Fe 12.5 has been studied at high temperatures up to 1700 K, which is by almost 400 K higher than the melting point of the material. It has been shown that the melt exhibits an excess heat capacity with respect to that determined by the Dulong-Petit law and that is a direct extension of the excess heat capacity of the solid state. It has been concluded that the excess heat capacity is related, as a whole, to the short-range order in the quasicrystal structure. This circumstance allows the identification of the orbital hybridization as the most probable mechanism of formation of the pseudogap in the electronic structure of the quasicrystals. |
| Audience | Academic |
| Author | Grushevskii, K. I. Gaiduchenko, A. B. Shchegolikhina, N. I. Prekul, A. F. |
| Author_xml | – sequence: 1 givenname: A. F. surname: Prekul fullname: Prekul, A. F. email: prekul@imp.uran.ru organization: Institute of Metal Physics, Ural Branch, Russian Academy of Sciences – sequence: 2 givenname: N. I. surname: Shchegolikhina fullname: Shchegolikhina, N. I. organization: Institute of Metal Physics, Ural Branch, Russian Academy of Sciences – sequence: 3 givenname: A. B. surname: Gaiduchenko fullname: Gaiduchenko, A. B. organization: Institute of Reactor Materials, Russian Research Centre Kurchatov Institute – sequence: 4 givenname: K. I. surname: Grushevskii fullname: Grushevskii, K. I. organization: Ural State Pedagogical University |
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| Cites_doi | 10.1080/14786430801958372 10.1080/095008300176452 10.1134/S0031918X09080031 10.1080/14786435.2010.508758 10.1134/S1063783408110024 10.1134/S1063783410090027 10.1088/0953-8984/18/49/L03 10.1080/14786430500253893 10.1016/S0921-5093(00)01132-1 10.1080/14786430701361347 10.1103/PhysRevB.65.024203 |
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| Keywords | Linear Thermal Expansion Coefficient Debye Model Heat Capacity Excess Heat Capacity Beryllium Oxide |
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| References | ZhangL. M.LuckR.Philos. Mag.2006863292006PMag...86..329Z10.1080/14786430500253893 PrekulA. F.ShalaevaE. V.ShchegolikhinaN. I.Phys. Solid State201052917972010PhSS...52.1797P10.1134/S1063783410090027 FaudotF.Ann. Chim. (Fr.)199318445 IshikawaR.IshikawaT.OkadaJ.T.MaskiT.WatanabeY.NanaoS.Philos. Mag.20078729652007PMag...87.2965I10.1080/14786430701361347 OkadaJ. T.InuiM.IshikawaD.BaronA. Q. R.MatsudaK.TsutsuiS.WatanabeY.NanaoS.IshikawaT.J. Phys.: Condens. Matter200618L6132006JPCM...18L.613O10.1088/0953-8984/18/49/L03 PrekulA. F.ShchegolikhinaN. I.NazarovaS. Z.EdagawaK.Phys. Met. Metallogr.200910821202009PMM...108..120P10.1134/S0031918X09080031 KajimaK.EdagawaK.SuzukiT.Philos. Mag. Lett.200080492000PMagL..80...49K10.1080/095008300176452 ShulyatevD. A.NigmatulinA. S.LobanovaA. V.GasparyanT. A.Philos. Mag.20088823192008PMag...88.2319S10.1080/14786430801958372 SwalinR. A.Thermodynamics of Solids19722nd ed.New YorkWiley PrekulA. F.KazantsevV. A.ShchegolikhinaN. I.GulyaevaR. I.EdagavaL.Phys. Solid State2008501120132008PhSS...50.2013P10.1134/S1063783408110024 MizutaniU.InukaiM.SatoH.Philos. Mag.20119119–2125362011PMag...91.2536M10.1080/14786435.2010.508758 KeesomW. H.PearlmanN.Handbook der Physik1956BerlinSpringer SimonetV.HippertF.AudierM.BellissentR.Phys. Rev. B: Condens. Matter2001650242032002PhRvB..65b4203S10.1103/PhysRevB.65.024203 EdagawaK.KajiyamaK.Mater. Sci. Eng., A2000294–296646 K. Kajima (9964_CR10) 2000; 80 A. F. Prekul (9964_CR11) 2010; 52 F. Faudot (9964_CR6) 1993; 18 R. A. Swalin (9964_CR9) 1972 W. H. Keesom (9964_CR14) 1956 L. M. Zhang (9964_CR7) 2006; 86 A. F. Prekul (9964_CR4) 2009; 108 R. Ishikawa (9964_CR8) 2007; 87 U. Mizutani (9964_CR5) 2011; 91 K. Edagawa (9964_CR1) 2000; 294–296 V. Simonet (9964_CR12) 2001; 65 D. A. Shulyatev (9964_CR3) 2008; 88 J. T. Okada (9964_CR13) 2006; 18 A. F. Prekul (9964_CR2) 2008; 50 |
| References_xml | – volume-title: Handbook der Physik year: 1956 ident: 9964_CR14 contributor: fullname: W. H. Keesom – volume: 88 start-page: 2319 year: 2008 ident: 9964_CR3 publication-title: Philos. Mag. doi: 10.1080/14786430801958372 contributor: fullname: D. A. Shulyatev – volume-title: Thermodynamics of Solids year: 1972 ident: 9964_CR9 contributor: fullname: R. A. Swalin – volume: 80 start-page: 49 year: 2000 ident: 9964_CR10 publication-title: Philos. Mag. Lett. doi: 10.1080/095008300176452 contributor: fullname: K. Kajima – volume: 108 start-page: 120 issue: 2 year: 2009 ident: 9964_CR4 publication-title: Phys. Met. Metallogr. doi: 10.1134/S0031918X09080031 contributor: fullname: A. F. Prekul – volume: 18 start-page: 445 year: 1993 ident: 9964_CR6 publication-title: Ann. Chim. (Fr.) contributor: fullname: F. Faudot – volume: 91 start-page: 2536 issue: 19–21 year: 2011 ident: 9964_CR5 publication-title: Philos. Mag. doi: 10.1080/14786435.2010.508758 contributor: fullname: U. Mizutani – volume: 50 start-page: 2013 issue: 11 year: 2008 ident: 9964_CR2 publication-title: Phys. Solid State doi: 10.1134/S1063783408110024 contributor: fullname: A. F. Prekul – volume: 52 start-page: 1797 issue: 9 year: 2010 ident: 9964_CR11 publication-title: Phys. Solid State doi: 10.1134/S1063783410090027 contributor: fullname: A. F. Prekul – volume: 18 start-page: L613 year: 2006 ident: 9964_CR13 publication-title: J. Phys.: Condens. Matter doi: 10.1088/0953-8984/18/49/L03 contributor: fullname: J. T. Okada – volume: 86 start-page: 329 year: 2006 ident: 9964_CR7 publication-title: Philos. Mag. doi: 10.1080/14786430500253893 contributor: fullname: L. M. Zhang – volume: 294–296 start-page: 646 year: 2000 ident: 9964_CR1 publication-title: Mater. Sci. Eng., A doi: 10.1016/S0921-5093(00)01132-1 contributor: fullname: K. Edagawa – volume: 87 start-page: 2965 year: 2007 ident: 9964_CR8 publication-title: Philos. Mag. doi: 10.1080/14786430701361347 contributor: fullname: R. Ishikawa – volume: 65 start-page: 024203 year: 2001 ident: 9964_CR12 publication-title: Phys. Rev. B: Condens. Matter doi: 10.1103/PhysRevB.65.024203 contributor: fullname: V. Simonet |
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| Snippet | The heat capacity of icosahedral quasicrystals Al
63
Cu
25
Fe
12
and Al
62
Cu
25.5
Fe
12.5
has been studied at high temperatures up to 1700 K, which is by... The heat capacity of icosahedral quasicrystals [Al.sub.63][Cu.sub.25][Fe.sub.12] and [Al.sub.62][Cu.sub.25.5][Fe.sub.12.5] has been studied at high... |
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| Title | Comparative study of the heat capacity of icosahedral quasicrystals in solid and liquid states |
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