Synthesis and characterizations of novel spindle-like terphenyl-type chromophores for non-linear optical materials
A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene π-conjugating bridge, N, N-dimethyl and triphenyl amino donors, and Tricyanovinyldihydrofuran(TCF), 1,3,3-trimethyl-5-dicyanovinyl-1-cyclohexene (TDC) acceptors, have been synthesized successfully f...
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| Published in: | Tetrahedron Vol. 67; no. 22; pp. 4110 - 4117 |
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| Language: | English |
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03-06-2011
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| Abstract | A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene π-conjugating bridge,
N,
N-dimethyl and triphenyl amino donors, and Tricyanovinyldihydrofuran(TCF), 1,3,3-trimethyl-5-dicyanovinyl-1-cyclohexene (TDC) acceptors, have been synthesized successfully for the first time. And the non-linear optical properties were evaluated by using the finite-field (FF) method. The results show that, the first-order hyperpolarizability of the chromophores increase with the increase of the withdraw ability of the substituent group on the π-conjugating bridge.
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| AbstractList | A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene [pi]-conjugating bridge, N,N-dimethyl and triphenyl amino donors, and Tricyanovinyldihydrofuran(TCF), 1,3,3-trimethyl-5-dicyanovinyl-1-cyclohexene (TDC) acceptors, have been synthesized successfully for the first time. And the non-linear optical properties were evaluated by using the finite-field (FF) method. The results show that, the first-order hyperpolarizability of the chromophores increase with the increase of the withdraw ability of the substituent group on the [pi]-conjugating bridge. A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene π-conjugating bridge, N, N-dimethyl and triphenyl amino donors, and Tricyanovinyldihydrofuran(TCF), 1,3,3-trimethyl-5-dicyanovinyl-1-cyclohexene (TDC) acceptors, have been synthesized successfully for the first time. And the non-linear optical properties were evaluated by using the finite-field (FF) method. The results show that, the first-order hyperpolarizability of the chromophores increase with the increase of the withdraw ability of the substituent group on the π-conjugating bridge. [Display omitted] |
| Author | Zhang, Xiaolong Shi, Zuosen Yang, Guochun Su, Zhongmin Cui, Zhanchen |
| Author_xml | – sequence: 1 givenname: Zuosen surname: Shi fullname: Shi, Zuosen organization: State Key Lab for Supramolecular Structure and Materials, College of Chemistry, Jilin University, 2699# Qianjin Road, Changchun 130012, PR China – sequence: 2 givenname: Xiaolong surname: Zhang fullname: Zhang, Xiaolong organization: State Key Lab for Supramolecular Structure and Materials, College of Chemistry, Jilin University, 2699# Qianjin Road, Changchun 130012, PR China – sequence: 3 givenname: Guochun surname: Yang fullname: Yang, Guochun organization: Institute of Functional Material Chemistry, Faculty of Chemistry, Northeast Normal University, Changchun 130024, PR China – sequence: 4 givenname: Zhongmin surname: Su fullname: Su, Zhongmin organization: Institute of Functional Material Chemistry, Faculty of Chemistry, Northeast Normal University, Changchun 130024, PR China – sequence: 5 givenname: Zhanchen surname: Cui fullname: Cui, Zhanchen email: cuizc@jlu.edu.cn organization: State Key Lab for Supramolecular Structure and Materials, College of Chemistry, Jilin University, 2699# Qianjin Road, Changchun 130012, PR China |
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| CitedBy_id | crossref_primary_10_1016_j_dyepig_2018_11_001 crossref_primary_10_1039_C6TC02964G crossref_primary_10_1002_ange_201403509 crossref_primary_10_1002_anie_201403509 crossref_primary_10_1134_S1070428022070077 crossref_primary_10_1016_j_polymer_2019_121987 crossref_primary_10_1002_tcr_202300262 crossref_primary_10_1039_C5RA27783C crossref_primary_10_1080_00304948_2017_1336052 crossref_primary_10_1039_C6TC02016J crossref_primary_10_1039_C7TC00713B crossref_primary_10_1007_s11172_022_3417_2 crossref_primary_10_1039_C9CP05827C crossref_primary_10_1021_acs_jpca_2c02204 |
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| Keywords | NLO Terphenyl Optical Chromophore Terphenyl derivatives Furan derivatives Non linear optics Oxygen heterocycle Characterization Amine Styrene derivatives Optical properties Vinylic compound Benzenic compound Optical material Chemical synthesis Electron acceptor Hyperpolarization |
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| Snippet | A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene π-conjugating bridge,
N,
N-dimethyl and triphenyl amino... A series of novel spindle-like terphenyl-type chromophores, based on 2,5-diphenyl-1,4-distyrylbenzene [pi]-conjugating bridge, N,N-dimethyl and triphenyl amino... |
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| SubjectTerms | Alicyclic compounds Alicyclic compounds, terpenoids, prostaglandins, steroids Bridges (structures) Chemistry Chromophore Chromophores Exact sciences and technology Fundamental areas of phenomenology (including applications) NLO Noncondensed benzenic compounds Nonlinearity Optical Optical materials Optical properties Optics Organic chemistry Other nonlinear optical materials; photorefractive and semiconductor materials Physics Preparations and properties Synthesis (chemistry) Terphenyl Tetrahedrons Triphenyls |
| Title | Synthesis and characterizations of novel spindle-like terphenyl-type chromophores for non-linear optical materials |
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