Atomically thin superfluid helium films on solid hydrogen
We have measured both adsorption isotherms and third-sound resonance of atomically thin {sup 4}He films on solid hydrogen. We find helium more weakly bound to a hydrogen surface than to other rare-gas surfaces, with a van der Waals cofficient of 4.6{plus minus}0.4 K (layers){sup 3}. We have also mea...
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| Published in: | Physical review letters Vol. 67; no. 9; pp. 1118 - 1121 |
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| Format: | Journal Article |
| Language: | English |
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Ridge, NY
American Physical Society
26-08-1991
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| Abstract | We have measured both adsorption isotherms and third-sound resonance of atomically thin {sup 4}He films on solid hydrogen. We find helium more weakly bound to a hydrogen surface than to other rare-gas surfaces, with a van der Waals cofficient of 4.6{plus minus}0.4 K (layers){sup 3}. We have also measured third sound, at 0.18 K, down to a total helium coverage of 0.45{plus minus}0.01 atomic layer, indicating an inert coverage at {ital T}=0 K of 0.29 atomic layer or less. In common with other weak-binding substrates we also see depressions in third-sound velocity near half-layer intervals. |
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| AbstractList | We have measured both adsorption isotherms and third-sound resonance of atomically thin {sup 4}He films on solid hydrogen. We find helium more weakly bound to a hydrogen surface than to other rare-gas surfaces, with a van der Waals cofficient of 4.6{plus minus}0.4 K (layers){sup 3}. We have also measured third sound, at 0.18 K, down to a total helium coverage of 0.45{plus minus}0.01 atomic layer, indicating an inert coverage at {ital T}=0 K of 0.29 atomic layer or less. In common with other weak-binding substrates we also see depressions in third-sound velocity near half-layer intervals. |
| Author | SHIRRON, P. J MOCHEL, J. M |
| Author_xml | – sequence: 1 givenname: P. J surname: SHIRRON fullname: SHIRRON, P. J organization: Univ. Illinois at Urbana-Champaign, dep. physics, Urbana IL 61801, United States – sequence: 2 givenname: J. M surname: MOCHEL fullname: MOCHEL, J. M organization: Univ. Illinois at Urbana-Champaign, dep. physics, Urbana IL 61801, United States |
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| Cites_doi | 10.1007/BF00681551 10.1103/PhysRevLett.58.1751 10.1007/BF00686097 10.1103/PhysRevLett.55.1761 10.1063/1.1746689 10.1063/1.1743130 10.1103/PhysRevLett.39.1201 10.1103/PhysRevLett.44.333 10.1103/PhysRev.183.327 10.1103/PhysRevB.32.5713 10.1007/BF00683712 10.1103/RevModPhys.53.199 10.1021/ja01269a023 10.1103/PhysRevA.7.790 10.1103/PhysRevB.31.2713 10.1063/1.1138320 10.1103/PhysRevB.39.8934 10.1103/PhysRevLett.52.2375 10.1007/BF00682673 |
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| Issue | 9 |
| Keywords | Liquid solid interface Support Hydrogen Chemical bond Crystals Superfluid Kosterlitz Thouless transition Coverage rate Experimental study Helium Thin film Sound velocity Adsorption Van der Waals interaction Isotherm Chemical potential Third sound |
| Language | English |
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| References | E. S. Sabisky (PhysRevLett.67.1118Cc10R1) 1973; 7 G. Agnolet (PhysRevLett.67.1118Cc13R1) 1989; 39 P. J. Shirron (PhysRevLett.67.1118Cc1R1) 1990; 78 S. Ramesh (PhysRevLett.67.1118Cc14R2) 1984; 52 M. W. Cole (PhysRevLett.67.1118Cc3R1) 1981; 53 L. V. Mikheev (PhysRevLett.67.1118Cc15R1) 1987; 65 E. Cheng (PhysRevLett.67.1118Cc4R1) 1991; 82 M. A. Paalanen (PhysRevLett.67.1118Cc19R1) 1985; 55 S. Volz (PhysRevLett.67.1118Cc6R1) 1985; 56 T. L. Hill (PhysRevLett.67.1118Cc9R3) 1949; 17 D. R. Nelson (PhysRevLett.67.1118Cc12R3) 1977; 39 E. Cheng (PhysRevLett.67.1118Cc2R1) 1989; 74 J. Frenkel (PhysRevLett.67.1118Cc9R1) 1946 J. A. Roth (PhysRevLett.67.1118Cc14R1) 1980; 44 D. Goodstein (PhysRevLett.67.1118Cc17R1) 1969; 183 R. A. Guyer (PhysRevLett.67.1118Cc21R1) 1985; 31 J. M. Kosterlitz (PhysRevLett.67.1118Cc12R1) 1973; 6 W. A. Steele (PhysRevLett.67.1118Cc8R1) 1956; 25 P. J. Shirron (PhysRevLett.67.1118Cc5R1) 1989; 75 S. Brunauer (PhysRevLett.67.1118Cc8R2) 1938; 60 D. Cieslikowski (PhysRevLett.67.1118Cc20R1) 1987; 58 E. Krotscheck (PhysRevLett.67.1118Cc16R1) 1985; 32 G. D. Halsey (PhysRevLett.67.1118Cc9R2) 1948; 16 J. M. Kosterlitz (PhysRevLett.67.1118Cc12R2) 1974; 7 |
| References_xml | – volume: 82 start-page: 49 year: 1991 ident: PhysRevLett.67.1118Cc4R1 publication-title: J. Low Temp. Phys. doi: 10.1007/BF00681551 contributor: fullname: E. Cheng – volume-title: Kinetic Theory of Liquids year: 1946 ident: PhysRevLett.67.1118Cc9R1 contributor: fullname: J. Frenkel – volume: 58 start-page: 1751 year: 1987 ident: PhysRevLett.67.1118Cc20R1 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.58.1751 contributor: fullname: D. Cieslikowski – volume: 78 start-page: 157 year: 1990 ident: PhysRevLett.67.1118Cc1R1 publication-title: J. Low Temp. Phys. doi: 10.1007/BF00686097 contributor: fullname: P. J. Shirron – volume: 55 start-page: 1761 year: 1985 ident: PhysRevLett.67.1118Cc19R1 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.55.1761 contributor: fullname: M. A. Paalanen – volume: 16 start-page: 931 year: 1948 ident: PhysRevLett.67.1118Cc9R2 publication-title: J. Chem. Phys. doi: 10.1063/1.1746689 contributor: fullname: G. D. Halsey – volume: 25 start-page: 819 year: 1956 ident: PhysRevLett.67.1118Cc8R1 publication-title: J. Chem. Phys. doi: 10.1063/1.1743130 contributor: fullname: W. A. Steele – volume: 39 start-page: 1201 year: 1977 ident: PhysRevLett.67.1118Cc12R3 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.39.1201 contributor: fullname: D. R. Nelson – volume: 44 start-page: 333 year: 1980 ident: PhysRevLett.67.1118Cc14R1 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.44.333 contributor: fullname: J. A. Roth – volume: 183 start-page: 327 year: 1969 ident: PhysRevLett.67.1118Cc17R1 publication-title: Phys. Rev. doi: 10.1103/PhysRev.183.327 contributor: fullname: D. Goodstein – volume: 32 start-page: 5713 year: 1985 ident: PhysRevLett.67.1118Cc16R1 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.32.5713 contributor: fullname: E. Krotscheck – volume: 75 start-page: 349 year: 1989 ident: PhysRevLett.67.1118Cc5R1 publication-title: J. Low Temp. Phys. doi: 10.1007/BF00683712 contributor: fullname: P. J. Shirron – volume: 53 start-page: 199 year: 1981 ident: PhysRevLett.67.1118Cc3R1 publication-title: Rev. Mod. Phys. doi: 10.1103/RevModPhys.53.199 contributor: fullname: M. W. Cole – volume: 60 start-page: 309 year: 1938 ident: PhysRevLett.67.1118Cc8R2 publication-title: J. Am. Chem. Soc. doi: 10.1021/ja01269a023 contributor: fullname: S. Brunauer – volume: 7 start-page: 1046 year: 1974 ident: PhysRevLett.67.1118Cc12R2 publication-title: J. Phys. Chem. contributor: fullname: J. M. Kosterlitz – volume: 17 start-page: 580 year: 1949 ident: PhysRevLett.67.1118Cc9R3 publication-title: J. Chem. Phys. contributor: fullname: T. L. Hill – volume: 65 start-page: 971 year: 1987 ident: PhysRevLett.67.1118Cc15R1 publication-title: Sov. Phys. JETP contributor: fullname: L. V. Mikheev – volume: 7 start-page: 790 year: 1973 ident: PhysRevLett.67.1118Cc10R1 publication-title: Phys. Rev. A doi: 10.1103/PhysRevA.7.790 contributor: fullname: E. S. Sabisky – volume: 31 start-page: 2713 year: 1985 ident: PhysRevLett.67.1118Cc21R1 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.31.2713 contributor: fullname: R. A. Guyer – volume: 56 start-page: 444 year: 1985 ident: PhysRevLett.67.1118Cc6R1 publication-title: Rev. Sci. Instrum. doi: 10.1063/1.1138320 contributor: fullname: S. Volz – volume: 6 start-page: 1181 year: 1973 ident: PhysRevLett.67.1118Cc12R1 publication-title: J. Phys. Chem. contributor: fullname: J. M. Kosterlitz – volume: 39 start-page: 8934 year: 1989 ident: PhysRevLett.67.1118Cc13R1 publication-title: Phys. Rev. B doi: 10.1103/PhysRevB.39.8934 contributor: fullname: G. Agnolet – volume: 52 start-page: 2375 year: 1984 ident: PhysRevLett.67.1118Cc14R2 publication-title: Phys. Rev. Lett. doi: 10.1103/PhysRevLett.52.2375 contributor: fullname: S. Ramesh – volume: 74 start-page: 519 year: 1989 ident: PhysRevLett.67.1118Cc2R1 publication-title: J. Low Temp. Phys. doi: 10.1007/BF00682673 contributor: fullname: E. Cheng |
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| Snippet | We have measured both adsorption isotherms and third-sound resonance of atomically thin {sup 4}He films on solid hydrogen. We find helium more weakly bound to... |
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| SubjectTerms | 08 HYDROGEN 080800 - Hydrogen- Properties & Composition 640450 - Fluid Physics- Superfluidity ADSORPTION ISOTHERMS CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY Condensed matter: structure, mechanical and thermal properties ELEMENTS EVEN-EVEN NUCLEI Exact sciences and technology Films (including physical adsorption) FLUIDS HELIUM 4 HELIUM II HELIUM ISOTOPES HYDROGEN ISOTHERMS ISOTOPES LIGHT NUCLEI NONMETALS NUCLEI Physics QUANTUM FLUIDS Quantum fluids and solids; liquid and solid helium SORPTIVE PROPERTIES STABLE ISOTOPES SURFACE PROPERTIES THIN FILMS THIRD SOUND VAN DER WAALS FORCES WETTABILITY |
| Title | Atomically thin superfluid helium films on solid hydrogen |
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