Valley polarization in MoS2 monolayers by optical pumping

Most electronic devices exploit the electric charge of electrons, but it is also possible to build devices that rely on other properties of electrons. Spintronic devices, for example, make use of the spin of electrons 1 , 2 . Valleytronics is a more recent development that relies on the fact that th...

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Published in:	Nature nanotechnology Vol. 7; no. 8; pp. 490 - 493
Main Authors:	Zeng, Hualing, Dai, Junfeng, Yao, Wang, Xiao, Di, Cui, Xiaodong
Format:	Journal Article
Language:	English
Published:	London Nature Publishing Group UK 01-08-2012 Nature Publishing Group
Subjects:	639/624/400 639/925/357/995 Chemistry and Materials Science Electronics Electrons letter Light Luminescence Materials Science Molybdenum - chemistry Nanotechnology Nanotechnology and Microengineering Optical Phenomena Polarization Semiconductors Symmetry Hong Kong China China
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Abstract	Most electronic devices exploit the electric charge of electrons, but it is also possible to build devices that rely on other properties of electrons. Spintronic devices, for example, make use of the spin of electrons 1 , 2 . Valleytronics is a more recent development that relies on the fact that the conduction bands of some materials have two or more minima at equal energies but at different positions in momentum space 3 , 4 , 5 . To make a valleytronic device it is necessary to control the number of electrons in these valleys, thereby producing a valley polarization 6 , 7 , 8 , 9 , 10 , 11 . Single-layer MoS 2 is a promising material for valleytronics because both the conduction and valence band edges have two energy-degenerate valleys at the corners of the first Brillouin zone 12 . Here, we demonstrate that optical pumping with circularly polarized light can achieve a valley polarization of 30% in pristine monolayer MoS 2 . Our results, and similar results by Mak et al. 13 , demonstrate the viability of optical valley control and valley-based electronic and optoelectronic applications in MoS 2 monolayers. Circularly polarized light has been used to achieve a valley polarization of 30% in single-layer molybdenum disulphide.
AbstractList	Most electronic devices exploit the electric charge of electrons, but it is also possible to build devices that rely on other properties of electrons. Spintronic devices, for example, make use of the spin of electrons. Valleytronics is a more recent development that relies on the fact that the conduction bands of some materials have two or more minima at equal energies but at different positions in momentum space. To make a valleytronic device it is necessary to control the number of electrons in these valleys, thereby producing a valley polarization. Single-layer MoS(2) is a promising material for valleytronics because both the conduction and valence band edges have two energy-degenerate valleys at the corners of the first Brillouin zone. Here, we demonstrate that optical pumping with circularly polarized light can achieve a valley polarization of 30% in pristine monolayer MoS(2). Our results, and similar results by Mak et al., demonstrate the viability of optical valley control and valley-based electronic and optoelectronic applications in MoS(2) monolayers. Most electronic devices exploit the electric charge of electrons, but it is also possible to build devices that rely on other properties of electrons. Spintronic devices, for example, make use of the spin of electrons 1 , 2 . Valleytronics is a more recent development that relies on the fact that the conduction bands of some materials have two or more minima at equal energies but at different positions in momentum space 3 , 4 , 5 . To make a valleytronic device it is necessary to control the number of electrons in these valleys, thereby producing a valley polarization 6 , 7 , 8 , 9 , 10 , 11 . Single-layer MoS 2 is a promising material for valleytronics because both the conduction and valence band edges have two energy-degenerate valleys at the corners of the first Brillouin zone 12 . Here, we demonstrate that optical pumping with circularly polarized light can achieve a valley polarization of 30% in pristine monolayer MoS 2 . Our results, and similar results by Mak et al. 13 , demonstrate the viability of optical valley control and valley-based electronic and optoelectronic applications in MoS 2 monolayers. Circularly polarized light has been used to achieve a valley polarization of 30% in single-layer molybdenum disulphide.
Author	Dai, Junfeng Zeng, Hualing Cui, Xiaodong Xiao, Di Yao, Wang
Author_xml	– sequence: 1 givenname: Hualing surname: Zeng fullname: Zeng, Hualing organization: Physics Department, The University of Hong Kong – sequence: 2 givenname: Junfeng surname: Dai fullname: Dai, Junfeng organization: Physics Department, The University of Hong Kong, Department of Physics, South University of Science and Technology of China – sequence: 3 givenname: Wang surname: Yao fullname: Yao, Wang organization: Physics Department, The University of Hong Kong, Center of Theoretical and Computational Physics, The University of Hong Kong – sequence: 4 givenname: Di surname: Xiao fullname: Xiao, Di organization: Materials Science and Technology Division, Oak Ridge National Laboratory – sequence: 5 givenname: Xiaodong surname: Cui fullname: Cui, Xiaodong email: xdcui@hku.hk organization: Physics Department, The University of Hong Kong
BackLink	https://www.ncbi.nlm.nih.gov/pubmed/22706701$$D View this record in MEDLINE/PubMed
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Snippet	Most electronic devices exploit the electric charge of electrons, but it is also possible to build devices that rely on other properties of electrons....
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SubjectTerms	639/624/400 639/925/357/995 Chemistry and Materials Science Electronics Electrons letter Light Luminescence Materials Science Molybdenum - chemistry Nanotechnology Nanotechnology and Microengineering Optical Phenomena Polarization Semiconductors Symmetry
Title	Valley polarization in MoS2 monolayers by optical pumping
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