Spectral narrowing in coherent rayleigh scattering
Spectral narrowing of the coherent Rayleigh scattering line shape in a room temperature CO(2) gas (2.5 x 10(23) m(-3)) with intense fields in the 10(15) W m(-2) range is observed. The line shape saturates to a width of approximately half that observed at low pump intensities and indicates a transiti...
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Published in: | Physical review letters Vol. 99; no. 13; p. 133001 |
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Main Authors: | , , |
Format: | Journal Article |
Language: | English |
Published: |
United States
28-09-2007
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Online Access: | Get full text |
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Summary: | Spectral narrowing of the coherent Rayleigh scattering line shape in a room temperature CO(2) gas (2.5 x 10(23) m(-3)) with intense fields in the 10(15) W m(-2) range is observed. The line shape saturates to a width of approximately half that observed at low pump intensities and indicates a transition from scattering primarily from untrapped molecules to that from both trapped and untrapped molecules that are localized by the deep (60 K) optical potentials produced by the pump beams. At higher densities (5 x 10(24) m(-3)), collisions between the trapped and untrapped molecules broaden the spectral profile. |
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Bibliography: | ObjectType-Article-1 SourceType-Scholarly Journals-1 ObjectType-Feature-2 content type line 23 |
ISSN: | 0031-9007 1079-7114 |
DOI: | 10.1103/PhysRevLett.99.133001 |