Spectral narrowing in coherent rayleigh scattering

Spectral narrowing of the coherent Rayleigh scattering line shape in a room temperature CO(2) gas (2.5 x 10(23) m(-3)) with intense fields in the 10(15) W m(-2) range is observed. The line shape saturates to a width of approximately half that observed at low pump intensities and indicates a transiti...

Full description

Saved in:
Bibliographic Details
Published in:Physical review letters Vol. 99; no. 13; p. 133001
Main Authors: Bookey, H T, Shneider, M N, Barker, P F
Format: Journal Article
Language:English
Published: United States 28-09-2007
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Spectral narrowing of the coherent Rayleigh scattering line shape in a room temperature CO(2) gas (2.5 x 10(23) m(-3)) with intense fields in the 10(15) W m(-2) range is observed. The line shape saturates to a width of approximately half that observed at low pump intensities and indicates a transition from scattering primarily from untrapped molecules to that from both trapped and untrapped molecules that are localized by the deep (60 K) optical potentials produced by the pump beams. At higher densities (5 x 10(24) m(-3)), collisions between the trapped and untrapped molecules broaden the spectral profile.
Bibliography:ObjectType-Article-1
SourceType-Scholarly Journals-1
ObjectType-Feature-2
content type line 23
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.99.133001