Enhancing antifouling characteristics and performance against protein macromolecule foulant on PVDF membrane ultrafiltration with eco-friendly Arabic gum additive

This study investigated the effects of Arabic gum (AG) on the separation performance of polyvinylidene fluoride (PVDF) membranes. The membrane properties were characterized using scanning electron microscope energy dispersive X-ray (SEM-EDX), Fourier transforms infrared (FTIR), tensile strength test...

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Published in:	Journal of macromolecular science. Part A, Pure and applied chemistry Vol. 60; no. 4; pp. 255 - 269
Main Authors:	Putri, Radenrara Dewi Artanti, Abriyanto, Herlambang, Desiriani, Ria, Filardli, Abdullah Malik Islam, Bahlawan, Zuhriyan Ash Shiddieqy, Kusumaningrum, Maharani, Prastiwi, Gita Putri, Raihana, Rica, Siami, Desy Hikmatul, Aswar, Randi
Format:	Journal Article
Language:	English
Published:	New York Taylor & Francis 03-04-2023 Marcel Dekker, Inc
Subjects:	Antifouling Arabic gum Contact angle Fourier transforms Infrared spectroscopy Membranes Polyvinylidene fluorides PVDF Scanning electron microscopy Serum albumin Tensile strength Ultrafiltration ultrafiltration membrane
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Abstract	This study investigated the effects of Arabic gum (AG) on the separation performance of polyvinylidene fluoride (PVDF) membranes. The membrane properties were characterized using scanning electron microscope energy dispersive X-ray (SEM-EDX), Fourier transforms infrared (FTIR), tensile strength tester, and contact angle. Results showed that incorporating AG from 0.5 wt% to 1.5 wt% into PVDF membrane could increase pure water flux from 47.46 L/m 2 h to 66.04 L/m 2 h and porosity from 53% to 58%. Moreover, the highest flux recovery was obtained by PVDF/AG-1.5 membrane, revealing the improvement in fouling resistance against bovine serum albumin (BSA). However, the addition of AG from 0.5 wt% to 1.5 wt% did not affect to increase of membrane mechanical strength and the efficiency of the membranes for BSA rejection. SEM, XRD and FTIR analyses confirmed the successful incorporation of AG, which improved membrane surface hydrophilicity compared to the pristine PVDF membrane. Overall, the obtained result showed that incorporating AG could attain synergy benefits in enhancing the membrane properties and performance.
AbstractList	This study investigated the effects of Arabic gum (AG) on the separation performance of polyvinylidene fluoride (PVDF) membranes. The membrane properties were characterized using scanning electron microscope energy dispersive X-ray (SEM-EDX), Fourier transforms infrared (FTIR), tensile strength tester, and contact angle. Results showed that incorporating AG from 0.5 wt% to 1.5 wt% into PVDF membrane could increase pure water flux from 47.46 L/m 2 h to 66.04 L/m 2 h and porosity from 53% to 58%. Moreover, the highest flux recovery was obtained by PVDF/AG-1.5 membrane, revealing the improvement in fouling resistance against bovine serum albumin (BSA). However, the addition of AG from 0.5 wt% to 1.5 wt% did not affect to increase of membrane mechanical strength and the efficiency of the membranes for BSA rejection. SEM, XRD and FTIR analyses confirmed the successful incorporation of AG, which improved membrane surface hydrophilicity compared to the pristine PVDF membrane. Overall, the obtained result showed that incorporating AG could attain synergy benefits in enhancing the membrane properties and performance. This study investigated the effects of Arabic gum (AG) on the separation performance of polyvinylidene fluoride (PVDF) membranes. The membrane properties were characterized using scanning electron microscope energy dispersive X-ray (SEM–EDX), Fourier transforms infrared (FTIR), tensile strength tester, and contact angle. Results showed that incorporating AG from 0.5 wt% to 1.5 wt% into PVDF membrane could increase pure water flux from 47.46 L/m2 h to 66.04 L/m2 h and porosity from 53% to 58%. Moreover, the highest flux recovery was obtained by PVDF/AG-1.5 membrane, revealing the improvement in fouling resistance against bovine serum albumin (BSA). However, the addition of AG from 0.5 wt% to 1.5 wt% did not affect to increase of membrane mechanical strength and the efficiency of the membranes for BSA rejection. SEM, XRD and FTIR analyses confirmed the successful incorporation of AG, which improved membrane surface hydrophilicity compared to the pristine PVDF membrane. Overall, the obtained result showed that incorporating AG could attain synergy benefits in enhancing the membrane properties and performance.
Author	Bahlawan, Zuhriyan Ash Shiddieqy Filardli, Abdullah Malik Islam Putri, Radenrara Dewi Artanti Prastiwi, Gita Putri Aswar, Randi Raihana, Rica Desiriani, Ria Kusumaningrum, Maharani Abriyanto, Herlambang Siami, Desy Hikmatul
Author_xml	– sequence: 1 givenname: Radenrara Dewi Artanti orcidid: 0000-0002-8990-3091 surname: Putri fullname: Putri, Radenrara Dewi Artanti organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 2 givenname: Herlambang orcidid: 0000-0003-4760-4082 surname: Abriyanto fullname: Abriyanto, Herlambang organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 3 givenname: Ria orcidid: 0000-0001-6940-1767 surname: Desiriani fullname: Desiriani, Ria organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 4 givenname: Abdullah Malik Islam orcidid: 0000-0003-2490-6782 surname: Filardli fullname: Filardli, Abdullah Malik Islam organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 5 givenname: Zuhriyan Ash Shiddieqy orcidid: 0000-0003-3872-4402 surname: Bahlawan fullname: Bahlawan, Zuhriyan Ash Shiddieqy organization: Department of Chemical Engineering, Faculty of Engineering, Universitas Negeri Semarang – sequence: 6 givenname: Maharani orcidid: 0000-0002-3879-6644 surname: Kusumaningrum fullname: Kusumaningrum, Maharani organization: Department of Chemical Engineering, Faculty of Engineering, Universitas Negeri Semarang – sequence: 7 givenname: Gita Putri surname: Prastiwi fullname: Prastiwi, Gita Putri organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 8 givenname: Rica surname: Raihana fullname: Raihana, Rica organization: Membrane Research Center (MeR-C), Integrated Laboratory for Research and Services, Diponegoro University – sequence: 9 givenname: Desy Hikmatul surname: Siami fullname: Siami, Desy Hikmatul organization: Department of Chemical Engineering, Faculty of Engineering, Universitas Negeri Semarang – sequence: 10 givenname: Randi orcidid: 0000-0003-3687-9275 surname: Aswar fullname: Aswar, Randi organization: Department of Chemical Engineering, Faculty of Engineering, Universitas Negeri Semarang
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SubjectTerms	Antifouling Arabic gum Contact angle Fourier transforms Infrared spectroscopy Membranes Polyvinylidene fluorides PVDF Scanning electron microscopy Serum albumin Tensile strength Ultrafiltration ultrafiltration membrane
Title	Enhancing antifouling characteristics and performance against protein macromolecule foulant on PVDF membrane ultrafiltration with eco-friendly Arabic gum additive
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