Luminescence quenching of Ru(II) complexes in polydimethylsiloxane sensors for oxygen
The luminescence quenching of ruthenium(II)-tris(1,10-phenanthroline) and ruthenium(II)-tris(4,7-diphenyl-1,10-phenanthroline) by oxygen in films of commercial polydimethylsiloxane was studied by steady state and time-resolved methods. The decay kinetics is not monoexponential in the absence and in...
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| Published in: | Journal of photochemistry and photobiology. A, Chemistry. Vol. 120; no. 1; pp. 15 - 21 |
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| Main Authors: | , , |
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| Language: | English |
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Lausanne
Elsevier B.V
04-01-1999
Elsevier Science |
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| Abstract | The luminescence quenching of ruthenium(II)-tris(1,10-phenanthroline) and ruthenium(II)-tris(4,7-diphenyl-1,10-phenanthroline) by oxygen in films of commercial polydimethylsiloxane was studied by steady state and time-resolved methods. The decay kinetics is not monoexponential in the absence and in the presence of oxygen. It can be accurately described in all cases by the function exp(−
Bt
1/2), a particular case of the stretched exponential behaviour often found in solid media. The steady state and integrated time-resolved quenching efficiency coincide and show a downward curvature as a function of oxygen partial pressure. This dependence is explained by assuming a Freundlich type adsorption of oxygen in the dopants of the polymer. Both complexes render the same dependence of adsorbed oxygen on its partial pressure. |
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| AbstractList | The luminescence quenching of ruthenium(II)-tris(1,10-phenanthroline) and ruthenium(II)-tris(4,7-diphenyl-1,10-phenanthroline) by oxygen in films of commercial polydimethylsiloxane was studied by steady state and time-resolved methods. The decay kinetics is not monoexponential in the absence and in the presence of oxygen. It can be accurately described in all cases by the function exp(−
Bt
1/2), a particular case of the stretched exponential behaviour often found in solid media. The steady state and integrated time-resolved quenching efficiency coincide and show a downward curvature as a function of oxygen partial pressure. This dependence is explained by assuming a Freundlich type adsorption of oxygen in the dopants of the polymer. Both complexes render the same dependence of adsorbed oxygen on its partial pressure. |
| Author | Daraio, Marta E. Bossi, Mariano L. F. Aramendı́a, Pedro |
| Author_xml | – sequence: 1 givenname: Mariano L. surname: Bossi fullname: Bossi, Mariano L. – sequence: 2 givenname: Marta E. surname: Daraio fullname: Daraio, Marta E. – sequence: 3 givenname: Pedro surname: F. Aramendı́a fullname: F. Aramendı́a, Pedro |
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| Cites_doi | 10.1021/ac00095a004 10.1021/ac00111a024 10.1021/ac00051a012 10.1021/ac00004a006 10.1002/bbpc.198800075 10.1021/ac00097a015 10.1007/BFb0017965 10.1021/j100010a029 10.1021/jp963132g 10.1021/ac970430g 10.1021/ac00150a012 10.1063/1.1697063 10.1021/ac960008k 10.1021/ed060p834 10.1002/bbpc.19790830403 10.1016/0009-2614(85)80438-3 10.1021/ac9507092 10.1364/AO.35.004117 10.1007/978-1-4615-7658-7 10.1021/ac960083v 10.1021/ac00118a013 10.1021/ac00114a012 10.1021/la00060a015 10.1016/0009-2614(85)85348-3 10.1021/ac00114a010 |
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| Keywords | Polymer Oxygen Ruthenium(II) diimines Luminescence Quenching Performance evaluation Dimethylsiloxane polymer Fluorescence detector Organic ligand Transition metal Complexes Chemical sensor Luminescence decay Matrix isolation Luminescence quenching Ruthenium Complexes Platinoid Complexes Gas detector |
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| Snippet | The luminescence quenching of ruthenium(II)-tris(1,10-phenanthroline) and ruthenium(II)-tris(4,7-diphenyl-1,10-phenanthroline) by oxygen in films of commercial... |
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| SubjectTerms | Analytical chemistry Chemistry Exact sciences and technology General, instrumentation Luminescence Oxygen Polymer Quenching Ruthenium(II) diimines |
| Title | Luminescence quenching of Ru(II) complexes in polydimethylsiloxane sensors for oxygen |
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