Controlled growth of Co9S8 nanoparticle-embedded carbon nanosheets/carbon nanofibers toward high-performance sodium storage
[Display omitted] •Multifunctional Co9S8@CNSs/CNFs flexible self-supporting electrode is designed for Sodium-ion batteries.•The advantages of multi-stage structural synergistic composites are illustrated at the electrode scale.•In-depth analysis of electrode electrochemical reaction kinetics and de-...
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| Published in: | Journal of colloid and interface science Vol. 648; pp. 644 - 653 |
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| Main Authors: | , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Inc
15-10-2023
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| Abstract | [Display omitted]
•Multifunctional Co9S8@CNSs/CNFs flexible self-supporting electrode is designed for Sodium-ion batteries.•The advantages of multi-stage structural synergistic composites are illustrated at the electrode scale.•In-depth analysis of electrode electrochemical reaction kinetics and de-/sodiation mechanism.•High sodium storage half-cells and stable full cell capacity with self-supporting electrodes are achieved.
Transition metal sulfides (TMSs) are considered as promising anodes for sodium-ion batteries (SIBs) due to their high theoretical capacity and low cost. However, TMSs suffer from massive volume expansion, slow sodium-ion diffusion kinetics, and poor electrical conductivity, which severely restrict their practical application. Herein, we design self-supporting Co9S8 nanoparticles embedded carbon nanosheets/carbon nanofibers (Co9S8@CNSs/CNFs) as anode materials for SIBs. The electrospun carbon nanofibers (CNFs) provide continuous conductive networks to accelerate the ion and electron diffusion/transport kinetics, while MOFs-derived carbon nanosheets (CNSs) buffer the volume variation of Co9S8, consequently improving the cycle stability. Benefitting from the unique design and pseudocapacitive features, Co9S8@CNSs/CNFs deliver a stable capacity of 516 mAh g−1 at 200 mA g−1 and a reversible capacity of 313 mAh g−1 after 1500 cycles at 2 A g−1. Note that, it also displays excellent sodium storage performance when assembled into a full cell. The rational design and excellent electrochemical properties endow Co9S8@CNSs/CNFs with the potential stepping into commercial SIBs. |
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| AbstractList | [Display omitted]
•Multifunctional Co9S8@CNSs/CNFs flexible self-supporting electrode is designed for Sodium-ion batteries.•The advantages of multi-stage structural synergistic composites are illustrated at the electrode scale.•In-depth analysis of electrode electrochemical reaction kinetics and de-/sodiation mechanism.•High sodium storage half-cells and stable full cell capacity with self-supporting electrodes are achieved.
Transition metal sulfides (TMSs) are considered as promising anodes for sodium-ion batteries (SIBs) due to their high theoretical capacity and low cost. However, TMSs suffer from massive volume expansion, slow sodium-ion diffusion kinetics, and poor electrical conductivity, which severely restrict their practical application. Herein, we design self-supporting Co9S8 nanoparticles embedded carbon nanosheets/carbon nanofibers (Co9S8@CNSs/CNFs) as anode materials for SIBs. The electrospun carbon nanofibers (CNFs) provide continuous conductive networks to accelerate the ion and electron diffusion/transport kinetics, while MOFs-derived carbon nanosheets (CNSs) buffer the volume variation of Co9S8, consequently improving the cycle stability. Benefitting from the unique design and pseudocapacitive features, Co9S8@CNSs/CNFs deliver a stable capacity of 516 mAh g−1 at 200 mA g−1 and a reversible capacity of 313 mAh g−1 after 1500 cycles at 2 A g−1. Note that, it also displays excellent sodium storage performance when assembled into a full cell. The rational design and excellent electrochemical properties endow Co9S8@CNSs/CNFs with the potential stepping into commercial SIBs. |
| Author | Wang, Silan Zhou, Ziyi Yang, Guorui Wen, Bo Yan, Wei Zhang, Zhijie |
| Author_xml | – sequence: 1 givenname: Silan surname: Wang fullname: Wang, Silan organization: Xi'an Key Laboratory of Solid Waste Recycling and Resource Recovery, State Key Laboratory of Multiphase Flow in Power Engineering, Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an 710049, China – sequence: 2 givenname: Ziyi surname: Zhou fullname: Zhou, Ziyi organization: Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, “Four Joint Subjects One Union” School-Enterprise Joint Research Center for Power Battery Recycling & Circulation Utilization Technology, Department of Applied Chemistry, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, China – sequence: 3 givenname: Bo surname: Wen fullname: Wen, Bo organization: Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, “Four Joint Subjects One Union” School-Enterprise Joint Research Center for Power Battery Recycling & Circulation Utilization Technology, Department of Applied Chemistry, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, China – sequence: 4 givenname: Zhijie surname: Zhang fullname: Zhang, Zhijie organization: Xi'an Key Laboratory of Solid Waste Recycling and Resource Recovery, State Key Laboratory of Multiphase Flow in Power Engineering, Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an 710049, China – sequence: 5 givenname: Guorui surname: Yang fullname: Yang, Guorui email: yangguorui@xjtu.edu.cn organization: Engineering Research Center of Energy Storage Materials and Devices, Ministry of Education, “Four Joint Subjects One Union” School-Enterprise Joint Research Center for Power Battery Recycling & Circulation Utilization Technology, Department of Applied Chemistry, School of Chemistry, Xi’an Jiaotong University, Xi’an 710049, China – sequence: 6 givenname: Wei surname: Yan fullname: Yan, Wei email: yanwei@xjtu.edu.cn organization: Xi'an Key Laboratory of Solid Waste Recycling and Resource Recovery, State Key Laboratory of Multiphase Flow in Power Engineering, Department of Environmental Science and Engineering, Xi'an Jiaotong University, Xi'an 710049, China |
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