Improved boundary lubrication of perfluoropolyether using fluoropolymer-grafted cellulose nanocrystal

As the thickener for fluorine greases, polytetrafluoroethylene (PTFE) powder performs insufficient load-carrying capacity and limited assistance for friction reduction and wear resistance in the boundary lubrication regime. The present work aims to explore novel nanoparticles with higher mechanical...

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Published in:	Cellulose (London) Vol. 30; no. 6; pp. 3757 - 3771
Main Authors:	Ge, Yue, Lin, Ning, Du, Chen, Amann, Tobias, Feng, Hao, Yuan, Chengqing, Li, Ke
Format:	Journal Article
Language:	English
Published:	Dordrecht Springer Netherlands 01-04-2023 Springer Nature B.V
Subjects:	Antiwear additives Bearing strength Bioorganic Chemistry Boundary lubrication Cellulose Ceramics Chemistry Chemistry and Materials Science Composites Engineering Fluorine Fluoropolymers Fourier transforms Friction Friction reduction Glass Grafting Graphene Greases Hydrocarbons Load carrying capacity Lubricants & lubrication Lubrication Nanocrystals Nanoparticles Natural Materials Organic Chemistry Original Research Physical Chemistry Polymer Sciences Polytetrafluoroethylene Sustainable Development Wear resistance Polytetrafluoroethylene powder Boundary lubrication Cellulose nanocrystals Perfluoropolyether lubricant
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Abstract	As the thickener for fluorine greases, polytetrafluoroethylene (PTFE) powder performs insufficient load-carrying capacity and limited assistance for friction reduction and wear resistance in the boundary lubrication regime. The present work aims to explore novel nanoparticles with higher mechanical strength as an alternative to PTFE. Cellulose nanocrystals (CNCs) were surface modified by grafting (or partially adsorbing) fluoropolymer chains and introduced into perfluoropolyether PFPE base oil. The obtained polyhexafuorobutyl methacrylate grafted CNC (CNC-g-PHFMA) powder exhibited good compatibility with the PFPE oil. The friction test and wear analysis showed that CNC-g-PHFMA formed a more intensive and stable tribo-film than PTFE on the sliding surface, resulting in more effective friction reduction (11%) and wear resistance (19%). This study demonstrates that fluoropolymer-grafted CNCs have a good application prospect in fluorine greases.
AbstractList	As the thickener for fluorine greases, polytetrafluoroethylene (PTFE) powder performs insufficient load-carrying capacity and limited assistance for friction reduction and wear resistance in the boundary lubrication regime. The present work aims to explore novel nanoparticles with higher mechanical strength as an alternative to PTFE. Cellulose nanocrystals (CNCs) were surface modified by grafting (or partially adsorbing) fluoropolymer chains and introduced into perfluoropolyether PFPE base oil. The obtained polyhexafuorobutyl methacrylate grafted CNC (CNC-g-PHFMA) powder exhibited good compatibility with the PFPE oil. The friction test and wear analysis showed that CNC-g-PHFMA formed a more intensive and stable tribo-film than PTFE on the sliding surface, resulting in more effective friction reduction (11%) and wear resistance (19%). This study demonstrates that fluoropolymer-grafted CNCs have a good application prospect in fluorine greases.
Author	Du, Chen Feng, Hao Yuan, Chengqing Li, Ke Ge, Yue Lin, Ning Amann, Tobias
Author_xml	– sequence: 1 givenname: Yue surname: Ge fullname: Ge, Yue organization: School of Transportation and Logistics Engineering, Wuhan University of Technology, Reliability Engineering Institute, National Engineering Research Center for Water Transport Safety, MOST – sequence: 2 givenname: Ning surname: Lin fullname: Lin, Ning organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology – sequence: 3 givenname: Chen surname: Du fullname: Du, Chen organization: School of Chemistry, Chemical Engineering and Life Sciences, Wuhan University of Technology – sequence: 4 givenname: Tobias surname: Amann fullname: Amann, Tobias organization: Fraunhofer Institute for Mechanics of Materials IWM – sequence: 5 givenname: Hao surname: Feng fullname: Feng, Hao organization: Shenzhen Volyke Technology Co., Ltd – sequence: 6 givenname: Chengqing surname: Yuan fullname: Yuan, Chengqing organization: School of Transportation and Logistics Engineering, Wuhan University of Technology, Reliability Engineering Institute, National Engineering Research Center for Water Transport Safety, MOST – sequence: 7 givenname: Ke surname: Li fullname: Li, Ke email: li_ke@whut.edu.cn organization: School of Transportation and Logistics Engineering, Wuhan University of Technology, Reliability Engineering Institute, National Engineering Research Center for Water Transport Safety, MOST
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Keywords	Polytetrafluoroethylene powder Boundary lubrication Cellulose nanocrystals Perfluoropolyether lubricant
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Snippet	As the thickener for fluorine greases, polytetrafluoroethylene (PTFE) powder performs insufficient load-carrying capacity and limited assistance for friction...
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SubjectTerms	Antiwear additives Bearing strength Bioorganic Chemistry Boundary lubrication Cellulose Ceramics Chemistry Chemistry and Materials Science Composites Engineering Fluorine Fluoropolymers Fourier transforms Friction Friction reduction Glass Grafting Graphene Greases Hydrocarbons Load carrying capacity Lubricants & lubrication Lubrication Nanocrystals Nanoparticles Natural Materials Organic Chemistry Original Research Physical Chemistry Polymer Sciences Polytetrafluoroethylene Sustainable Development Wear resistance
Title	Improved boundary lubrication of perfluoropolyether using fluoropolymer-grafted cellulose nanocrystal
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