Target-to-substrate distance influenced linear and nonlinear optical properties of a-plane oriented ZnO:Al thin films
This manuscript deals with the investigation of the impact of target-to-substrate distance on the linear and nonlinear optical properties of a -plane oriented aluminum-doped ZnO (ZnO:Al) thin films synthesized by the pulsed laser deposition (PLD) technique. X-ray diffraction studies proclaim an incr...
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| Published in: | Journal of materials science. Materials in electronics Vol. 32; no. 17; pp. 22214 - 22231 |
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| Abstract | This manuscript deals with the investigation of the impact of target-to-substrate distance on the linear and nonlinear optical properties of
a
-plane oriented aluminum-doped ZnO (ZnO:Al) thin films synthesized by the pulsed laser deposition (PLD) technique. X-ray diffraction studies proclaim an increment in the crystallinity with a decrement in target-to-substrate distance from 6 to 3 cm, attributed to increased thickness, decrease in stress, and defect levels in the thin films. A relaxation in the stress induces a decrease in the energy gap (3.47–3.37 eV) with a reduction in target–substrate distance from 6 to 3 cm is observed from UV–visible spectroscopic analysis. Spectroscopic ellipsometry confirms an increment in the refractive index and extinction coefficient with a decrease in target-to-substrate distance. From the Photoluminescence spectrum, the presence of low defect levels in the ZnO:Al thin films prepared at a shorter target-to-substrate distance is observed. The induced absorption (RSA) and self-defocusing process of ZnO:Al thin films are revealed by open aperture and closed aperture
Z
-scan measurements at 532 nm wavelength. The optical limiting behavior of all the thin films strongly suggests their applicability in optical power limiting. Thus, the present study emphasizes the optimization of the target-to-substrate distance to tailor the structural, linear, and nonlinear optical properties of the
a
-plane oriented ZnO:Al thin films. |
|---|---|
| AbstractList | This manuscript deals with the investigation of the impact of target-to-substrate distance on the linear and nonlinear optical properties of a-plane oriented aluminum-doped ZnO (ZnO:Al) thin films synthesized by the pulsed laser deposition (PLD) technique. X-ray diffraction studies proclaim an increment in the crystallinity with a decrement in target-to-substrate distance from 6 to 3 cm, attributed to increased thickness, decrease in stress, and defect levels in the thin films. A relaxation in the stress induces a decrease in the energy gap (3.47–3.37 eV) with a reduction in target–substrate distance from 6 to 3 cm is observed from UV–visible spectroscopic analysis. Spectroscopic ellipsometry confirms an increment in the refractive index and extinction coefficient with a decrease in target-to-substrate distance. From the Photoluminescence spectrum, the presence of low defect levels in the ZnO:Al thin films prepared at a shorter target-to-substrate distance is observed. The induced absorption (RSA) and self-defocusing process of ZnO:Al thin films are revealed by open aperture and closed aperture Z-scan measurements at 532 nm wavelength. The optical limiting behavior of all the thin films strongly suggests their applicability in optical power limiting. Thus, the present study emphasizes the optimization of the target-to-substrate distance to tailor the structural, linear, and nonlinear optical properties of the a-plane oriented ZnO:Al thin films. This manuscript deals with the investigation of the impact of target-to-substrate distance on the linear and nonlinear optical properties of a -plane oriented aluminum-doped ZnO (ZnO:Al) thin films synthesized by the pulsed laser deposition (PLD) technique. X-ray diffraction studies proclaim an increment in the crystallinity with a decrement in target-to-substrate distance from 6 to 3 cm, attributed to increased thickness, decrease in stress, and defect levels in the thin films. A relaxation in the stress induces a decrease in the energy gap (3.47–3.37 eV) with a reduction in target–substrate distance from 6 to 3 cm is observed from UV–visible spectroscopic analysis. Spectroscopic ellipsometry confirms an increment in the refractive index and extinction coefficient with a decrease in target-to-substrate distance. From the Photoluminescence spectrum, the presence of low defect levels in the ZnO:Al thin films prepared at a shorter target-to-substrate distance is observed. The induced absorption (RSA) and self-defocusing process of ZnO:Al thin films are revealed by open aperture and closed aperture Z -scan measurements at 532 nm wavelength. The optical limiting behavior of all the thin films strongly suggests their applicability in optical power limiting. Thus, the present study emphasizes the optimization of the target-to-substrate distance to tailor the structural, linear, and nonlinear optical properties of the a -plane oriented ZnO:Al thin films. |
| Author | Ananya Kote, M. Kumar, Prasad Bhajantri, R. F. Dharmaprakash, S. M. Sandeep, K. M. Patil, Parutagouda Shankaragouda |
| Author_xml | – sequence: 1 givenname: Prasad orcidid: 0000-0001-7488-4126 surname: Kumar fullname: Kumar, Prasad email: prasadkumarkulal@gmail.com organization: Department of Physics, Mangalore University – sequence: 2 givenname: S. M. surname: Dharmaprakash fullname: Dharmaprakash, S. M. organization: Department of Physics, Mangalore University – sequence: 3 givenname: M. surname: Ananya Kote fullname: Ananya Kote, M. organization: Department of Physics, Mangalore University – sequence: 4 givenname: K. M. surname: Sandeep fullname: Sandeep, K. M. organization: Department of Physics, Sri Jayachamarajendra College of Engineering, JSS Science and Technology University – sequence: 5 givenname: Parutagouda Shankaragouda surname: Patil fullname: Patil, Parutagouda Shankaragouda organization: Department of Physics, BLDEA’s Commerce, BHS Arts and TGP Science College – sequence: 6 givenname: R. F. surname: Bhajantri fullname: Bhajantri, R. F. organization: Department of Physics, Karnatak University |
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a
-plane oriented... This manuscript deals with the investigation of the impact of target-to-substrate distance on the linear and nonlinear optical properties of a-plane oriented... |
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| SubjectTerms | Aluminum Apertures Characterization and Evaluation of Materials Chemistry and Materials Science Constraining Defocusing Energy gap Materials Science Nonlinear optics Optical and Electronic Materials Optical properties Optimization Photoluminescence Pulsed laser deposition Pulsed lasers Refractivity Spectroellipsometry Stress relaxation Substrates Thin films Zinc oxide |
| Title | Target-to-substrate distance influenced linear and nonlinear optical properties of a-plane oriented ZnO:Al thin films |
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