Insights from the combined bulk chemical and surface characterization of airborne PM10 on source contributions and health risk: the case of three Mexican cities

Insights from the combined bulk chemical and surface characterization of airborne PM10 on source contributions and health risk: the case of three Mexican cities

The composition profiles of PM 10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was conducted to collect filter samples using high-volume instruments. The samples were analyzed by X-ray photoelectron spectroscopy (XPS), inductively...

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Published in:Air quality, atmosphere and health Vol. 16; no. 7; pp. 1455 - 1477
Main Authors: González, Lucy T., Pérez-Rodríguez, Michael, Rodríguez, F.E. Longoria, Mancilla, Yasmany, Acuña-Askar, Karim, Campos, Alfredo, Peña González, Luis A., Silva Vidaurri, Luis G., Zapata, Alejandro Arizpe, Nucamendi, Andrea, Karissova, Oxana, Mendoza, Alberto
Format: Journal Article
Language:English
Published: Dordrecht Springer Netherlands 01-07-2023
Springer Nature B.V
Subjects:
Air pollution
Air quality
Airborne particulates
Aromatic hydrocarbons
Atmospheric models
Atmospheric Protection/Air Quality Control/Air Pollution
Cancer
Chemical behavior
Chromium
Cities
Composition
Copper
Diffraction
Earth and Environmental Science
Earth crust
Electron microscopy
Environment
Environmental Health
Health Promotion and Disease Prevention
Health risk assessment
Health risks
Hydrocarbons
Inductively coupled plasma mass spectrometry
Iron
Lead
Mass spectrometry
Mass spectroscopy
Microscopy
Morphology
Outdoor air quality
Particulate matter
Particulate matter sources
Photoelectron spectroscopy
Photoelectrons
Raman spectroscopy
Scanning electron microscopy
Surface properties
Urban air quality
X ray photoelectron spectroscopy
X-ray diffraction
X-ray spectroscopy
X-rays
Mexico
Air pollution
Health risk assessment
PM
Source apportionment
Trace metals
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Abstract The composition profiles of PM 10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was conducted to collect filter samples using high-volume instruments. The samples were analyzed by X-ray photoelectron spectroscopy (XPS), inductively coupled plasma mass spectrometry (ICP-MS), scanning electron microscopy-energy dispersive X-ray spectroscopy (SEM-EDS), micro-Raman spectroscopy (MRS), and X-ray diffraction (XRD). The hazard quotient and incremental lifetime cancer risks were calculated to assess the health risks. The PM 10 concentrations ranged from 29.80 to 78.86 μg/m 3 . Fe, Zn, and Cu were the most abundant elements with average contents of 737.8 ± 258.69, 164.33 ± 64.73, and 83.31± 68.65 ng/m 3 , respectively. The highly toxic elements As, Cr, and Pb were found at concentrations that suggest potential health risks. The XPS revealed C, O, and Si to be the major elements in the PM 10 surface composition associated with aliphatic and aromatic hydrocarbons. The morphological analysis and PCA showed that the Fe-rich particles exhibited spheroidal morphologies, while the Pb-rich particles exhibited irregular and prismatic-type morphologies. These results suggest metal-work, lead-battery manufacturing, and the earth’s crust as emission sources. The cumulative risk of cancer suggests a moderate potential health risk that implies the need for preventive and corrective actions to improve air quality in urban cities. The combination of analytical techniques can be used to obtain better insights into the physical and chemical behavior of airborne particles in the atmosphere and potential tools to complement receptor models for source apportionment.
AbstractList The composition profiles of PM 10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was conducted to collect filter samples using high-volume instruments. The samples were analyzed by X-ray photoelectron spectroscopy (XPS), inductively coupled plasma mass spectrometry (ICP-MS), scanning electron microscopy-energy dispersive X-ray spectroscopy (SEM-EDS), micro-Raman spectroscopy (MRS), and X-ray diffraction (XRD). The hazard quotient and incremental lifetime cancer risks were calculated to assess the health risks. The PM 10 concentrations ranged from 29.80 to 78.86 μg/m 3 . Fe, Zn, and Cu were the most abundant elements with average contents of 737.8 ± 258.69, 164.33 ± 64.73, and 83.31± 68.65 ng/m 3 , respectively. The highly toxic elements As, Cr, and Pb were found at concentrations that suggest potential health risks. The XPS revealed C, O, and Si to be the major elements in the PM 10 surface composition associated with aliphatic and aromatic hydrocarbons. The morphological analysis and PCA showed that the Fe-rich particles exhibited spheroidal morphologies, while the Pb-rich particles exhibited irregular and prismatic-type morphologies. These results suggest metal-work, lead-battery manufacturing, and the earth’s crust as emission sources. The cumulative risk of cancer suggests a moderate potential health risk that implies the need for preventive and corrective actions to improve air quality in urban cities. The combination of analytical techniques can be used to obtain better insights into the physical and chemical behavior of airborne particles in the atmosphere and potential tools to complement receptor models for source apportionment.
The composition profiles of PM10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was conducted to collect filter samples using high-volume instruments. The samples were analyzed by X-ray photoelectron spectroscopy (XPS), inductively coupled plasma mass spectrometry (ICP-MS), scanning electron microscopy-energy dispersive X-ray spectroscopy (SEM-EDS), micro-Raman spectroscopy (MRS), and X-ray diffraction (XRD). The hazard quotient and incremental lifetime cancer risks were calculated to assess the health risks. The PM10 concentrations ranged from 29.80 to 78.86 μg/m3. Fe, Zn, and Cu were the most abundant elements with average contents of 737.8 ± 258.69, 164.33 ± 64.73, and 83.31± 68.65 ng/m3, respectively. The highly toxic elements As, Cr, and Pb were found at concentrations that suggest potential health risks. The XPS revealed C, O, and Si to be the major elements in the PM10 surface composition associated with aliphatic and aromatic hydrocarbons. The morphological analysis and PCA showed that the Fe-rich particles exhibited spheroidal morphologies, while the Pb-rich particles exhibited irregular and prismatic-type morphologies. These results suggest metal-work, lead-battery manufacturing, and the earth’s crust as emission sources. The cumulative risk of cancer suggests a moderate potential health risk that implies the need for preventive and corrective actions to improve air quality in urban cities. The combination of analytical techniques can be used to obtain better insights into the physical and chemical behavior of airborne particles in the atmosphere and potential tools to complement receptor models for source apportionment.
Author Mendoza, Alberto
Acuña-Askar, Karim
Karissova, Oxana
Pérez-Rodríguez, Michael
Rodríguez, F.E. Longoria
Nucamendi, Andrea
Silva Vidaurri, Luis G.
Campos, Alfredo
Zapata, Alejandro Arizpe
Mancilla, Yasmany
González, Lucy T.
Peña González, Luis A.
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  organization: Tecnologico de Monterrey, Escuela de Ingeniería y Ciencias
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  givenname: Luis G.
  surname: Silva Vidaurri
  fullname: Silva Vidaurri, Luis G.
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  fullname: Nucamendi, Andrea
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  givenname: Oxana
  surname: Karissova
  fullname: Karissova, Oxana
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  givenname: Alberto
  surname: Mendoza
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CitedBy_id crossref_primary_10_1007_s13762_024_05544_5
crossref_primary_10_1021_acsomega_3c08402
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Snippet The composition profiles of PM 10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was...
The composition profiles of PM10 were investigated using microscopy and spectroscopy techniques. A 24-h intensive, wintertime measurement campaign was...
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StartPage 1455
SubjectTerms Air pollution
Air quality
Airborne particulates
Aromatic hydrocarbons
Atmospheric models
Atmospheric Protection/Air Quality Control/Air Pollution
Cancer
Chemical behavior
Chromium
Cities
Composition
Copper
Diffraction
Earth and Environmental Science
Earth crust
Electron microscopy
Environment
Environmental Health
Health Promotion and Disease Prevention
Health risk assessment
Health risks
Hydrocarbons
Inductively coupled plasma mass spectrometry
Iron
Lead
Mass spectrometry
Mass spectroscopy
Microscopy
Morphology
Outdoor air quality
Particulate matter
Particulate matter sources
Photoelectron spectroscopy
Photoelectrons
Raman spectroscopy
Scanning electron microscopy
Surface properties
Urban air quality
X ray photoelectron spectroscopy
X-ray diffraction
X-ray spectroscopy
X-rays
Title Insights from the combined bulk chemical and surface characterization of airborne PM10 on source contributions and health risk: the case of three Mexican cities
URI https://link.springer.com/article/10.1007/s11869-023-01353-w
https://www.proquest.com/docview/2840417282
Volume 16
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