Regulating Intercalation of Layered Compounds for Electrochemical Energy Storage and Electrocatalysis

Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to their fast ion diffusion, exfoliative feature, superior mechanical flexibility, tunable bandgap structure, etc. The presence of large interlaye...

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Published in:	Advanced functional materials Vol. 31; no. 52
Main Authors:	Yang, Beibei, Tamirat, Andebet Gedamu, Bin, Duan, Yao, Yong, Lu, Hongbin, Xia, Yongyao
Format:	Journal Article
Language:	English
Published:	Hoboken Wiley Subscription Services, Inc 01-12-2021
Subjects:	Catalysis Charge transport Chemical reactions Conversion Diffusion layers Diffusion rate electrochemical performance Energy storage guest species Intercalation Interlayers Ion diffusion Ion transport Layered materials Materials science
Online Access:	Get full text
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Abstract	Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to their fast ion diffusion, exfoliative feature, superior mechanical flexibility, tunable bandgap structure, etc. The presence of large interlayer space between each layer enhances intercalation of the guest ion or molecule, which is beneficial for fast ion diffusion and charge transport along the channels. This intercalation reaction of layered compounds with guest species results in material with improved mechanical and electronic properties for efficient energy storage and conversion, catalysis, ion transport, and other applications. This review extensively discusses the intercalation of guest ionic or molecular species into layered materials used for various types of applications. It assesses the intercalation strategies, mechanism of ionic or molecular intercalation reactions, and highlights recent advancements. The electrochemical performances of several typical intercalated materials in batteries, supercapacitors, and electrocatalytic systems have been thoroughly discussed. Moreover, the challenges in the design and intercalation of layered materials, as well as prospects of future development are highlighted. This review systematically discusses the intercalation mechanism and method of guest species into layered materials, highlights their recent application such as lithium ion batteries, sodium ion batteries, aqueous zinc batteries, supercapacitors, hydrogen evolution reaction and oxygen evolution reaction, and emphasizes the strategies to enhance their properties and fundamental issues of the intercalated layered materials.
AbstractList	Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to their fast ion diffusion, exfoliative feature, superior mechanical flexibility, tunable bandgap structure, etc. The presence of large interlayer space between each layer enhances intercalation of the guest ion or molecule, which is beneficial for fast ion diffusion and charge transport along the channels. This intercalation reaction of layered compounds with guest species results in material with improved mechanical and electronic properties for efficient energy storage and conversion, catalysis, ion transport, and other applications. This review extensively discusses the intercalation of guest ionic or molecular species into layered materials used for various types of applications. It assesses the intercalation strategies, mechanism of ionic or molecular intercalation reactions, and highlights recent advancements. The electrochemical performances of several typical intercalated materials in batteries, supercapacitors, and electrocatalytic systems have been thoroughly discussed. Moreover, the challenges in the design and intercalation of layered materials, as well as prospects of future development are highlighted. This review systematically discusses the intercalation mechanism and method of guest species into layered materials, highlights their recent application such as lithium ion batteries, sodium ion batteries, aqueous zinc batteries, supercapacitors, hydrogen evolution reaction and oxygen evolution reaction, and emphasizes the strategies to enhance their properties and fundamental issues of the intercalated layered materials. Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to their fast ion diffusion, exfoliative feature, superior mechanical flexibility, tunable bandgap structure, etc. The presence of large interlayer space between each layer enhances intercalation of the guest ion or molecule, which is beneficial for fast ion diffusion and charge transport along the channels. This intercalation reaction of layered compounds with guest species results in material with improved mechanical and electronic properties for efficient energy storage and conversion, catalysis, ion transport, and other applications. This review extensively discusses the intercalation of guest ionic or molecular species into layered materials used for various types of applications. It assesses the intercalation strategies, mechanism of ionic or molecular intercalation reactions, and highlights recent advancements. The electrochemical performances of several typical intercalated materials in batteries, supercapacitors, and electrocatalytic systems have been thoroughly discussed. Moreover, the challenges in the design and intercalation of layered materials, as well as prospects of future development are highlighted. Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to their fast ion diffusion, exfoliative feature, superior mechanical flexibility, tunable bandgap structure, etc. The presence of large interlayer space between each layer enhances intercalation of the guest ion or molecule, which is beneficial for fast ion diffusion and charge transport along the channels. This intercalation reaction of layered compounds with guest species results in material with improved mechanical and electronic properties for efficient energy storage and conversion, catalysis, ion transport, and other applications. This review extensively discusses the intercalation of guest ionic or molecular species into layered materials used for various types of applications. It assesses the intercalation strategies, mechanism of ionic or molecular intercalation reactions, and highlights recent advancements. The electrochemical performances of several typical intercalated materials in batteries, supercapacitors, and electrocatalytic systems have been thoroughly discussed. Moreover, the challenges in the design and intercalation of layered materials, as well as prospects of future development are highlighted.
Author	Tamirat, Andebet Gedamu Yao, Yong Yang, Beibei Xia, Yongyao Lu, Hongbin Bin, Duan
Author_xml	– sequence: 1 givenname: Beibei surname: Yang fullname: Yang, Beibei organization: Nantong University – sequence: 2 givenname: Andebet Gedamu surname: Tamirat fullname: Tamirat, Andebet Gedamu organization: Kotebe Metropolitan University – sequence: 3 givenname: Duan orcidid: 0000-0002-4142-9052 surname: Bin fullname: Bin, Duan email: dbin17@fudan.edu.cn organization: Nantong University – sequence: 4 givenname: Yong surname: Yao fullname: Yao, Yong organization: Nantong University – sequence: 5 givenname: Hongbin surname: Lu fullname: Lu, Hongbin email: luhb@nju.edu.cn organization: Nantong University – sequence: 6 givenname: Yongyao surname: Xia fullname: Xia, Yongyao email: yyxia@fudan.edu.cn organization: Fudan University
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Snippet	Layered materials have received extensive attention for widespread applications such as energy storage and conversion, catalysis, and ion transport owing to...
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SubjectTerms	Catalysis Charge transport Chemical reactions Conversion Diffusion layers Diffusion rate electrochemical performance Energy storage guest species Intercalation Interlayers Ion diffusion Ion transport Layered materials Materials science
Title	Regulating Intercalation of Layered Compounds for Electrochemical Energy Storage and Electrocatalysis
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