Origin of poor photovoltaic performance of bis(tetracyanoantrathiophene) non-fullerene acceptor
Light-induced EPR and out-of-phase electron spin echo techniques were applied to identify the origin of low photovoltaic performance of novel non-fullerene antrathiophene-based acceptor 2,2′-[2,2′-(9,9-dioctyl-9H-fluorene-2,7-diyl)bis(anthra[2,3-b]thiophene-5,10-diylidene)]tetrapropanedinitrile (AT1...
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| Published in: | Chemical physics Vol. 546; p. 111162 |
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| Main Authors: | , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier B.V
01-06-2021
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| Abstract | Light-induced EPR and out-of-phase electron spin echo techniques were applied to identify the origin of low photovoltaic performance of novel non-fullerene antrathiophene-based acceptor 2,2′-[2,2′-(9,9-dioctyl-9H-fluorene-2,7-diyl)bis(anthra[2,3-b]thiophene-5,10-diylidene)]tetrapropanedinitrile (AT1), compared to conventional fullerene acceptors. These techniques revealed that average trapping energy of electrons in PCDTBT/AT1 blend is higher than that in the blends of PCDTBT with fullerene acceptors, while the distance of the initial photo-induced electron transfer is decreased. These two effects are suggested to enhance the efficiency of geminate recombination in PCDTBT/AT1 blend and reduce the yield of free charges, which is supposed to be the main reason for poor OPV performance of AT1-containing blends. Low electron mobility μe = 3.5 *10-6 cm2V-1s−1 is estimated for AT1 from photo-CELIV experiment. Strong localization of the electrons on terminal acceptor units of AT1 consistently explains both efficient geminate recombination in blends of antrathiophene-based acceptor with polymer donors and low electron mobility in AT1. |
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| AbstractList | Light-induced EPR and out-of-phase electron spin echo techniques were applied to identify the origin of low photovoltaic performance of novel non-fullerene antrathiophene-based acceptor 2,2′-[2,2′-(9,9-dioctyl-9H-fluorene-2,7-diyl)bis(anthra[2,3-b]thiophene-5,10-diylidene)]tetrapropanedinitrile (AT1), compared to conventional fullerene acceptors. These techniques revealed that average trapping energy of electrons in PCDTBT/AT1 blend is higher than that in the blends of PCDTBT with fullerene acceptors, while the distance of the initial photo-induced electron transfer is decreased. These two effects are suggested to enhance the efficiency of geminate recombination in PCDTBT/AT1 blend and reduce the yield of free charges, which is supposed to be the main reason for poor OPV performance of AT1-containing blends. Low electron mobility μe = 3.5 *10-6 cm2V-1s−1 is estimated for AT1 from photo-CELIV experiment. Strong localization of the electrons on terminal acceptor units of AT1 consistently explains both efficient geminate recombination in blends of antrathiophene-based acceptor with polymer donors and low electron mobility in AT1. |
| ArticleNumber | 111162 |
| Author | Kobeleva, E.S. Kulik, L.V. Baranov, D.S. Nevostruev, D.A. Degtyarenko, K.M. Sukhikh, A.S. Popov, A.A. Gadirov, R.M. Uvarov, M.N. |
| Author_xml | – sequence: 1 givenname: E.S. surname: Kobeleva fullname: Kobeleva, E.S. organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation – sequence: 2 givenname: A.A. surname: Popov fullname: Popov, A.A. organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation – sequence: 3 givenname: D.S. surname: Baranov fullname: Baranov, D.S. organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation – sequence: 4 givenname: M.N. surname: Uvarov fullname: Uvarov, M.N. organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation – sequence: 5 givenname: D.A. surname: Nevostruev fullname: Nevostruev, D.A. organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation – sequence: 6 givenname: K.M. surname: Degtyarenko fullname: Degtyarenko, K.M. organization: Tomsk State University, Tomsk, Russian Federation – sequence: 7 givenname: R.M. surname: Gadirov fullname: Gadirov, R.M. organization: Tomsk State University, Tomsk, Russian Federation – sequence: 8 givenname: A.S. surname: Sukhikh fullname: Sukhikh, A.S. organization: Nikolaev Institute of Inorganic Chemistry, Siberian Branch of Russian Academy of Sciences, Novosibirsk, Russian Federation – sequence: 9 givenname: L.V. surname: Kulik fullname: Kulik, L.V. email: chemphy@kinetics.nsc.ru organization: Voevodsky Institute of Chemical Kinetics and Combustion, Siberian Branch of the Russian Academy of Science, Novosibirsk, Russian Federation |
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| Keywords | Fullerenes Mobility Recombination Organic photovoltaics EPR spectroscopy Electron spin echo |
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| SubjectTerms | Electron spin echo EPR spectroscopy Fullerenes Mobility Organic photovoltaics Recombination |
| Title | Origin of poor photovoltaic performance of bis(tetracyanoantrathiophene) non-fullerene acceptor |
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