H2 production from ammonia decomposition with Mo2N catalyst driven by dielectric barrier discharge plasma
Dielectric barrier discharge (DBD) plasma-assisted ammonia decomposition reaction was investigated to produce carbon-free hydrogen for fuel cell applications. Mo2N catalyst was synthesized and applied for catalytic ammonia decomposition in different reaction modes. The synergistic effect of using Mo...
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| Published in: | International journal of hydrogen energy Vol. 49; pp. 1375 - 1385 |
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| Main Authors: | , , , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Ltd
02-01-2024
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| Abstract | Dielectric barrier discharge (DBD) plasma-assisted ammonia decomposition reaction was investigated to produce carbon-free hydrogen for fuel cell applications. Mo2N catalyst was synthesized and applied for catalytic ammonia decomposition in different reaction modes. The synergistic effect of using Mo2N catalyst in combination with DBD plasma resulted in near complete conversion of NH3 decomposition at specific energy input (SEI) of 39.6 kJ L−1, giving an energy efficiency of 6.1 mol·kWh−1 for H2 production. The particle size of Mo2N catalyst was discovered to affect the plasma-catalytic performance for NH3 decomposition, with Mo2N-powder catalyst showing higher reactivity compared with Mo2N-particle catalyst. The plasma diagnostic results showed that, compared to the filamentary discharge with Mo2N-particle catalyst, the Mo2N-powder catalyst packing lead to a predominant surface discharge; such localized surface discharges might contribute to a facile transportation of reactive species from the plasma phase to the catalyst surface, thus leading to higher plasma-catalytic performance.
•Plasma driven NH3 decomposition with Mo2N catalyst to produce hydrogen.•Plasma reduces NH3 full conversion temperature by > 100 °C compared to catalysis.•Mo2N catalyst size affects the plasma-catalytic performance. |
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| AbstractList | Dielectric barrier discharge (DBD) plasma-assisted ammonia decomposition reaction was investigated to produce carbon-free hydrogen for fuel cell applications. Mo2N catalyst was synthesized and applied for catalytic ammonia decomposition in different reaction modes. The synergistic effect of using Mo2N catalyst in combination with DBD plasma resulted in near complete conversion of NH3 decomposition at specific energy input (SEI) of 39.6 kJ L−1, giving an energy efficiency of 6.1 mol·kWh−1 for H2 production. The particle size of Mo2N catalyst was discovered to affect the plasma-catalytic performance for NH3 decomposition, with Mo2N-powder catalyst showing higher reactivity compared with Mo2N-particle catalyst. The plasma diagnostic results showed that, compared to the filamentary discharge with Mo2N-particle catalyst, the Mo2N-powder catalyst packing lead to a predominant surface discharge; such localized surface discharges might contribute to a facile transportation of reactive species from the plasma phase to the catalyst surface, thus leading to higher plasma-catalytic performance.
•Plasma driven NH3 decomposition with Mo2N catalyst to produce hydrogen.•Plasma reduces NH3 full conversion temperature by > 100 °C compared to catalysis.•Mo2N catalyst size affects the plasma-catalytic performance. |
| Author | Gou, Fujun Ye, Zongbiao Wang, Zhijun Deng, Jiyou Lei, Guangjiu Zhang, Kun Mao, Xinchun Zhang, Huazhou He, Ge Liao, Che Zheng, Guoyao |
| Author_xml | – sequence: 1 givenname: Zhijun orcidid: 0000-0003-1758-1430 surname: Wang fullname: Wang, Zhijun email: wangzhijun@cdu.edu.cn organization: Institute for Advanced Study, Chengdu University, Chengdu, 610106, China – sequence: 2 givenname: Huazhou surname: Zhang fullname: Zhang, Huazhou organization: School of Mechanical Engineering, Chengdu University, Chengdu, 610106, China – sequence: 3 givenname: Zongbiao surname: Ye fullname: Ye, Zongbiao email: zongbiaoye@scu.edu.cn organization: Institute of Nuclear Science and Technology, Sichuan University, Chengdu, 610064, China – sequence: 4 givenname: Ge surname: He fullname: He, Ge organization: School of Mechanical Engineering, Chengdu University, Chengdu, 610106, China – sequence: 5 givenname: Che surname: Liao fullname: Liao, Che organization: School of Mechanical Engineering, Chengdu University, Chengdu, 610106, China – sequence: 6 givenname: Jiyou surname: Deng fullname: Deng, Jiyou organization: School of Mechanical Engineering, Chengdu University, Chengdu, 610106, China – sequence: 7 givenname: Guangjiu surname: Lei fullname: Lei, Guangjiu organization: Southwestern Institute of Physics (SWIP), Chengdu, Sichuan, 610225, China – sequence: 8 givenname: Guoyao surname: Zheng fullname: Zheng, Guoyao organization: Southwestern Institute of Physics (SWIP), Chengdu, Sichuan, 610225, China – sequence: 9 givenname: Kun orcidid: 0000-0002-5484-1441 surname: Zhang fullname: Zhang, Kun organization: Institute of Nuclear Science and Technology, Sichuan University, Chengdu, 610064, China – sequence: 10 givenname: Fujun surname: Gou fullname: Gou, Fujun organization: Institute of Nuclear Science and Technology, Sichuan University, Chengdu, 610064, China – sequence: 11 givenname: Xinchun surname: Mao fullname: Mao, Xinchun email: mxch@caep.cn organization: Institute of Materials, China Academy of Engineering Physics, Jiangyou, 621908, China |
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| Keywords | Molybdenum nitride Ammonia decomposition Dielectric barrier discharge plasma Plasma catalysis Hydrogen production |
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