A novel Li3Mg3NbO7 microwave dielectric ceramic with ultra-low loss
Novel ultra-low-loss Li3Mg3NbO7 ceramics were synthesized using solid-state reaction method. The microstructure, bond characteristics, and microwave dielectric properties (MDPs) of the Li3Mg3NbO7 ceramics were explored. Furthermore, the Li3Mg3NbO7 ceramics crystallized in the orthorhombic rock-salt...
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| Published in: | Ceramics international Vol. 49; no. 15; pp. 25495 - 25503 |
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| Main Authors: | , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Ltd
01-08-2023
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| Abstract | Novel ultra-low-loss Li3Mg3NbO7 ceramics were synthesized using solid-state reaction method. The microstructure, bond characteristics, and microwave dielectric properties (MDPs) of the Li3Mg3NbO7 ceramics were explored. Furthermore, the Li3Mg3NbO7 ceramics crystallized in the orthorhombic rock-salt structure and the optimized density (97.7%) was obtained at 1200 °C. Utilizing complex chemical bond theory (P–V-L theory) and Raman spectra, the connection between structure and properties was constructed. εr value was mainly affected by the ρrel and average ionic polarization. The UNb–O and packing fraction were the key internal factors influencing the Q × f value. The τf was intimately relevant to Nb–O bond and τε. Notably, the Li3Mg3NbO7 ceramics sintered at 1200 °C exhibited excellent MDPs (εr = 14.7, Q × f = 121,047 GHz, τf = −24.8 ppm/°C), offering enormous prospects for 5G/6G communication applications. |
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| AbstractList | Novel ultra-low-loss Li3Mg3NbO7 ceramics were synthesized using solid-state reaction method. The microstructure, bond characteristics, and microwave dielectric properties (MDPs) of the Li3Mg3NbO7 ceramics were explored. Furthermore, the Li3Mg3NbO7 ceramics crystallized in the orthorhombic rock-salt structure and the optimized density (97.7%) was obtained at 1200 °C. Utilizing complex chemical bond theory (P–V-L theory) and Raman spectra, the connection between structure and properties was constructed. εr value was mainly affected by the ρrel and average ionic polarization. The UNb–O and packing fraction were the key internal factors influencing the Q × f value. The τf was intimately relevant to Nb–O bond and τε. Notably, the Li3Mg3NbO7 ceramics sintered at 1200 °C exhibited excellent MDPs (εr = 14.7, Q × f = 121,047 GHz, τf = −24.8 ppm/°C), offering enormous prospects for 5G/6G communication applications. |
| Author | Xiao, Hanning Xie, Jiawei Ma, Jingjing Guo, Wenming Cai, Chaoyang Qin, Hang Li, Hao Gao, Pengzhao |
| Author_xml | – sequence: 1 givenname: Chaoyang surname: Cai fullname: Cai, Chaoyang organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 2 givenname: Jingjing surname: Ma fullname: Ma, Jingjing organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 3 givenname: Jiawei surname: Xie fullname: Xie, Jiawei organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 4 givenname: Hao surname: Li fullname: Li, Hao organization: College of Electrical and Information Engineering, Hunan University, Changsha, 410082, China – sequence: 5 givenname: Wenming surname: Guo fullname: Guo, Wenming email: ggwwmm1234@163.com organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 6 givenname: Hang surname: Qin fullname: Qin, Hang organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 7 givenname: Pengzhao orcidid: 0000-0003-2119-6041 surname: Gao fullname: Gao, Pengzhao organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China – sequence: 8 givenname: Hanning orcidid: 0000-0001-8521-4443 surname: Xiao fullname: Xiao, Hanning email: hnxiao@hnu.edu.cn organization: College of Materials Science and Engineering, Hunan University, Changsha, 410082, China |
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| Title | A novel Li3Mg3NbO7 microwave dielectric ceramic with ultra-low loss |
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