Influence of surface plasmon polaritons on laser energy absorption and structuring of surfaces

• Published in: Applied surface science Vol. 512; p. 144420
• Main Authors: Terekhin, P.N., Benhayoun, O., Weber, S.T., Ivanov, D.S., Garcia, M.E., Rethfeld, B.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 15-05-2020
• Subjects: Laser energy absorption; LIPSS; Plasmonics; Surface plasmon polaritons; Ultrashort laser pulses; Surface plasmon polaritons; LIPSS; Plasmonics; Laser energy absorption; Ultrashort laser pulses
• ISSN: 0169-4332; 1873-5584
• DOI: 10.1016/j.apsusc.2019.144420

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•Analytical energy density rate for laser energy absorption is derived.•Interference of the excited SPP with the laser light is considered.•The interference pattern coexists along long distances.•The modulation of the laser deposited energy is close to the laser wavelength.•The results are applicable for the description of LIPSS as well as plasmonics.
The accurate calculation of laser energy absorption during femto- or picosecond laser pulse experiments is very important for the description of the formation of periodic surface structures. On a rough material surface, a crack or a step edge, ultrashort laser pulses can excite surface plasmon polaritons (SPP), i.e. surface plasmons coupled to a laser-electromagnetic wave. The interference of such plasmon wave and the incoming pulse leads to a periodic modulation of the deposited laser energy on the surface of the sample. In the present work, within the frames of a Two Temperature Model we propose the analytical form of the source term, which takes into account SPP excited at a step edge of a dielectric-metal interface upon irradiation of an ultrashort laser pulse at normal incidence. The influence of the laser pulse parameters on energy absorption is quantified for the example of gold. This result can be used for nanophotonic applications and for the theoretical investigation of the evolution of electronic and lattice temperatures and, therefore, of the formation of surfaces with predestined properties under controlled conditions.