Self-assembly and desulfurization mediated Turn-ON mercury sensing in aqueous media by tripodal synthetic amphiphile chemosensors
A water-soluble substituted thiourea amphiphile detects mercury with a Turn-On emission signal. Desulfurization-directed mercury sensing in water has been resolved with spectral studies. The amphiphilic thiourea shows appreciable selectivity and sensitivity among other cations and heavy metals, cont...
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| Published in: | Dyes and pigments Vol. 195; p. 109659 |
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| Language: | English |
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01-11-2021
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| Abstract | A water-soluble substituted thiourea amphiphile detects mercury with a Turn-On emission signal. Desulfurization-directed mercury sensing in water has been resolved with spectral studies. The amphiphilic thiourea shows appreciable selectivity and sensitivity among other cations and heavy metals, contrary to its control compound in aqueous media. The asymmetric tripodal can self-assemble into ribbon-like morphology in aqueous media, which has been outlined by microscopic analysis. The analytical utility of the tripodal has been probed through real water samples and soil testing. Moreover, the Hg-ensemble selectively recognizes H2S viz; sulphide ion in water and rendering a substantially low detection limit of 0.5 ppm. Realistically, paper strips are set for the fluorimetric visualization of both the analytes.
Desulfurization mediated “Turn-On” mercury sensing in water has been reported by an asymmetric tripodal amphiphile, which exhibits self-assembling properties. [Display omitted]
•Tripodal “Turn On” mercury chemosensor in aqueous media•Self-assembly studies of the substituted thiourea amphiphile•Desulfurization mediated mercury sensing•Anion sensing in water via ensemble viz; sulfide ion•Analytical utilities paper strips, real water sample, soil testing; etc.•Substantially low detection limit for both the toxins |
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| AbstractList | A water-soluble substituted thiourea amphiphile detects mercury with a Turn-On emission signal. Desulfurization-directed mercury sensing in water has been resolved with spectral studies. The amphiphilic thiourea shows appreciable selectivity and sensitivity among other cations and heavy metals, contrary to its control compound in aqueous media. The asymmetric tripodal can self-assemble into ribbon-like morphology in aqueous media, which has been outlined by microscopic analysis. The analytical utility of the tripodal has been probed through real water samples and soil testing. Moreover, the Hg-ensemble selectively recognizes H2S viz; sulphide ion in water and rendering a substantially low detection limit of 0.5 ppm. Realistically, paper strips are set for the fluorimetric visualization of both the analytes.
Desulfurization mediated “Turn-On” mercury sensing in water has been reported by an asymmetric tripodal amphiphile, which exhibits self-assembling properties. [Display omitted]
•Tripodal “Turn On” mercury chemosensor in aqueous media•Self-assembly studies of the substituted thiourea amphiphile•Desulfurization mediated mercury sensing•Anion sensing in water via ensemble viz; sulfide ion•Analytical utilities paper strips, real water sample, soil testing; etc.•Substantially low detection limit for both the toxins |
| ArticleNumber | 109659 |
| Author | Das, Gopal De, Sagnik |
| Author_xml | – sequence: 1 givenname: Sagnik surname: De fullname: De, Sagnik – sequence: 2 givenname: Gopal surname: Das fullname: Das, Gopal email: gdas@iitg.ac.in |
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| CitedBy_id | crossref_primary_10_1039_D3SD00146F crossref_primary_10_1016_j_ymeth_2024_01_002 crossref_primary_10_1021_acs_langmuir_2c00517 crossref_primary_10_1016_j_jlumin_2021_118668 crossref_primary_10_1002_slct_202400920 crossref_primary_10_1016_j_dyepig_2023_111502 crossref_primary_10_1039_D2NR01524B crossref_primary_10_1039_D2RA04093J crossref_primary_10_1016_j_jphotochem_2022_114491 crossref_primary_10_1021_acs_inorgchem_2c03152 crossref_primary_10_1016_j_molstruc_2024_138035 crossref_primary_10_1021_acs_langmuir_2c03357 crossref_primary_10_1016_j_jphotochem_2022_114431 |
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| Keywords | Desulfurization Self-assembly Tripodal amphiphile Mercury sensing H2S sensing |
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| Title | Self-assembly and desulfurization mediated Turn-ON mercury sensing in aqueous media by tripodal synthetic amphiphile chemosensors |
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