Receptor properties of nanoporous structures based on β-cyclodextrin
A columnar modification of β-cyclodextrin (β-CD col ) has been synthesized using self-assembly and self-organization processes. It is shown that the obtained macrocycle assemblies in the solid state are highly ordered structures with through cylindrical pores with an average diameter of ∼0.7 nm and...
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| Published in: | Nanotechnologies in Russia Vol. 5; no. 5-6; pp. 304 - 312 |
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| Abstract | A columnar modification of β-cyclodextrin (β-CD
col
) has been synthesized using self-assembly and self-organization processes. It is shown that the obtained macrocycle assemblies in the solid state are highly ordered structures with through cylindrical pores with an average diameter of ∼0.7 nm and a length of about 60 nm. These structures can be of interest as a new type of macroreceptors for the inclusion of molecules with diameters not exceeding 0.7 nm belonging to various chemical classes. The abilities of the common cage structure of β-CD and the β-CD
col
modification to bind low-molecular-weight volatile organic compounds have been compared. The dependence of the composition, structure, and thermal stability of the inclusion complexes on the ligand nature and geometry is analyzed. The absence of any specificity in the adsorption of ligands on β-CD
col
and the possibility of using this structure as a stable nanocontainter for the storage of volatile compounds is demonstrated. |
|---|---|
| AbstractList | A columnar modification of β-cyclodextrin (β-CD
col
) has been synthesized using self-assembly and self-organization processes. It is shown that the obtained macrocycle assemblies in the solid state are highly ordered structures with through cylindrical pores with an average diameter of ∼0.7 nm and a length of about 60 nm. These structures can be of interest as a new type of macroreceptors for the inclusion of molecules with diameters not exceeding 0.7 nm belonging to various chemical classes. The abilities of the common cage structure of β-CD and the β-CD
col
modification to bind low-molecular-weight volatile organic compounds have been compared. The dependence of the composition, structure, and thermal stability of the inclusion complexes on the ligand nature and geometry is analyzed. The absence of any specificity in the adsorption of ligands on β-CD
col
and the possibility of using this structure as a stable nanocontainter for the storage of volatile compounds is demonstrated. |
| Author | Panova, I. G. Matukhina, E. V. Topchieva, I. N. Zhukova, E. K. |
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| Cites_doi | 10.1002/masy.200450630 10.1126/science.1072252 10.1002/1521-3773(20000616)39:12<2081::AID-ANIE2081>3.0.CO;2-A 10.1021/jp0102217 10.1021/ac071509g 10.1002/(SICI)1521-3773(19990115)38:1/2<56::AID-ANIE56>3.0.CO;2-E 10.1016/S0040-4020(01)87780-2 10.1007/s00289-006-0697-x 10.1021/jp014352j 10.1021/la0262452 10.1021/cr9700181 10.1126/science.1062711 10.1038/386377a0 10.1126/science.286.5442.1127 10.1126/science.1067208 10.1021/nl015692j 10.1021/ja054119p 10.1002/anie.200462356 10.1063/1.881603 10.1021/ja0436289 |
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| Keywords | Cyclodextrin Guest Molecule Columnar Structure Inclusion Complex Macrocycle |
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| Title | Receptor properties of nanoporous structures based on β-cyclodextrin |
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