Desorption of U(VI) from montmorillonite with aluminum and iron hydroxides deposited on its surface
Decontamination of uranium-containing samples based on montmorillonite from the Cherkassy deposit, with Al(III) and Fe(III) hydroxides (weight fraction with respect to metal 0 and 5%: M-0, MAl-5, and MFe-5) deposited on its surface, by desorption with complexing agents (EDTA, citric acid, oxalic aci...
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| Published in: | Radiochemistry (New York, N.Y.) Vol. 51; no. 3; pp. 301 - 307 |
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01-06-2009
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| Abstract | Decontamination of uranium-containing samples based on montmorillonite from the Cherkassy deposit, with Al(III) and Fe(III) hydroxides (weight fraction with respect to metal 0 and 5%: M-0, MAl-5, and MFe-5) deposited on its surface, by desorption with complexing agents (EDTA, citric acid, oxalic acid, sodium carbonate) was studied. With respect to efficiency of U(VI) desorption from the sample surface, the ligands can be ranked in the following order: citric acid > oxalic acid > ETDA ≥ sodium carbonate. In neutral solutions, citric acid is the most effective and environmentally suitable. From M-0 and MAl-5 samples, U(VI) is desorbed completely, whereas in the case of MFe-5 about 15% of U is irreversibly bound to the surface. |
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| AbstractList | Decontamination of uranium-containing samples based on montmorillonite from the Cherkassy deposit, with Al(III) and Fe(III) hydroxides (weight fraction with respect to metal 0 and 5%: M-0, MAl-5, and MFe-5) deposited on its surface, by desorption with complexing agents (EDTA, citric acid, oxalic acid, sodium carbonate) was studied. With respect to efficiency of U(VI) desorption from the sample surface, the ligands can be ranked in the following order: citric acid > oxalic acid > ETDA ≥ sodium carbonate. In neutral solutions, citric acid is the most effective and environmentally suitable. From M-0 and MAl-5 samples, U(VI) is desorbed completely, whereas in the case of MFe-5 about 15% of U is irreversibly bound to the surface. |
| Author | Kobets, S. A. Pshinko, G. N. Bogolepov, A. A. |
| Author_xml | – sequence: 1 givenname: A. A. surname: Bogolepov fullname: Bogolepov, A. A. organization: Dumanskii Institute of Colloid and Water Chemistry, National Academy of Science of Ukraine – sequence: 2 givenname: S. A. surname: Kobets fullname: Kobets, S. A. organization: Dumanskii Institute of Colloid and Water Chemistry, National Academy of Science of Ukraine – sequence: 3 givenname: G. N. surname: Pshinko fullname: Pshinko, G. N. organization: Dumanskii Institute of Colloid and Water Chemistry, National Academy of Science of Ukraine |
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| Title | Desorption of U(VI) from montmorillonite with aluminum and iron hydroxides deposited on its surface |
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