Reversible evolution of ferroelectric-antiferroelectric phase transition in lanthanum-modified NaNbO3-based ceramics
Sodium niobate (NN) lead-free perovskites have been concentrated on due to high performance and abundant phase structure. The complex structure evolution has become a hot topic of research for this kind of materials. In this work, antiferroelectric phase is recovered by introducing La3+ dopant from...
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| Published in: | Journal of the European Ceramic Society Vol. 44; no. 1; pp. 233 - 241 |
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| Main Authors: | , , , , , , |
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01-01-2024
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| Abstract | Sodium niobate (NN) lead-free perovskites have been concentrated on due to high performance and abundant phase structure. The complex structure evolution has become a hot topic of research for this kind of materials. In this work, antiferroelectric phase is recovered by introducing La3+ dopant from modified ferroelectric states, indicating reversible composition-induced antiferroelectric-ferroelectric (AFE-FE) phase transition in NN-based ceramics. Significantly, change tendency of decreasing first and then increasing appears for phase transition temperature with increasing La3+, which is different from general phenomenon for ions dopant. Antiferroelectric orthorhombic (Pbma) is induced from ferroelectric tetragonal (P4mm) with a transient state of paraelectric cubic (Pm3m) via enhancing La3+. Further, substitution on A-site and A/B-sites are revealed with low and high content of La3+, respectively, accompanied by decreased first and then increased oxygen vacancy. Moreover, obviously deteriorated piezoelectric response is observed along with poor domain switching due to the vanishing ferroelectric domain for FE-PE-AFE phase transition. Meanwhile, weak strain, piezoelectric and dielectric properties are observed for antiferroelectric phase with antiparallel dipoles, while enhanced strain and dielectric permittivity are gained around ferroelectric-paraelectric coexistence or paraelectric region originating from electric field-induced ferroelectric state from polar nanoregions. Thus, this work demonstrated an abnormal phase transition in NN-based ceramics, promoting the understanding of antiferroelectrics. |
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| AbstractList | Sodium niobate (NN) lead-free perovskites have been concentrated on due to high performance and abundant phase structure. The complex structure evolution has become a hot topic of research for this kind of materials. In this work, antiferroelectric phase is recovered by introducing La3+ dopant from modified ferroelectric states, indicating reversible composition-induced antiferroelectric-ferroelectric (AFE-FE) phase transition in NN-based ceramics. Significantly, change tendency of decreasing first and then increasing appears for phase transition temperature with increasing La3+, which is different from general phenomenon for ions dopant. Antiferroelectric orthorhombic (Pbma) is induced from ferroelectric tetragonal (P4mm) with a transient state of paraelectric cubic (Pm3m) via enhancing La3+. Further, substitution on A-site and A/B-sites are revealed with low and high content of La3+, respectively, accompanied by decreased first and then increased oxygen vacancy. Moreover, obviously deteriorated piezoelectric response is observed along with poor domain switching due to the vanishing ferroelectric domain for FE-PE-AFE phase transition. Meanwhile, weak strain, piezoelectric and dielectric properties are observed for antiferroelectric phase with antiparallel dipoles, while enhanced strain and dielectric permittivity are gained around ferroelectric-paraelectric coexistence or paraelectric region originating from electric field-induced ferroelectric state from polar nanoregions. Thus, this work demonstrated an abnormal phase transition in NN-based ceramics, promoting the understanding of antiferroelectrics. |
| Author | Tao, Hong Zhao, Chunlin Yin, Jie Ergu, Daji Wu, Bo Ma, Jian Zhao, Lin |
| Author_xml | – sequence: 1 givenname: Hong orcidid: 0000-0002-1005-2336 surname: Tao fullname: Tao, Hong email: taohongscu@163.com organization: Sichuan Zoige Alpine Wetland Ecosystem National Observation and Research Station, Southwest Minzu University, 610041 Chengdu, China – sequence: 2 givenname: Jie surname: Yin fullname: Yin, Jie organization: Department of Materials Science, Sichuan University, Chengdu 610064, China – sequence: 3 givenname: Chunlin surname: Zhao fullname: Zhao, Chunlin organization: Department of Materials Science, Fuzhou, Fuzhou 310002, China – sequence: 4 givenname: Lin surname: Zhao fullname: Zhao, Lin organization: Sichuan Prov Key Lab Informat Mat, Southwest Minzu University, Chengdu 610041, China – sequence: 5 givenname: Bo surname: Wu fullname: Wu, Bo organization: Sichuan Zoige Alpine Wetland Ecosystem National Observation and Research Station, Southwest Minzu University, 610041 Chengdu, China – sequence: 6 givenname: Jian surname: Ma fullname: Ma, Jian organization: Sichuan Zoige Alpine Wetland Ecosystem National Observation and Research Station, Southwest Minzu University, 610041 Chengdu, China – sequence: 7 givenname: Daji surname: Ergu fullname: Ergu, Daji email: ergudaji@163.com organization: Sichuan Prov Key Lab Informat Mat, Southwest Minzu University, Chengdu 610041, China |
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| Keywords | Ferroelectric-antiferroelectric phase transition Sodium niobate ceramics Ions substitution |
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| Title | Reversible evolution of ferroelectric-antiferroelectric phase transition in lanthanum-modified NaNbO3-based ceramics |
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