Excellent thermal stability and high quantum efficiency orange-red-emitting AlPO4:Eu3+ phosphors for WLED application

Excellent thermal stability and high quantum efficiency orange-red-emitting AlPO4:Eu3+ phosphors for WLED application

Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows strong orange-red emissions with the strongest peaks at 588, 594, 685 and 700 nm. The highest PL intensity is achieved at the dopant concent...

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Published in:Journal of alloys and compounds Vol. 853; p. 156941
Main Authors: Tran, M.T., Tu, Nguyen, Quang, N.V., Nguyen, D.H, Thu, L.T.H., Trung, D.Q., Huy, P.T.
Format: Journal Article
Language:English
Published: Lausanne Elsevier B.V 05-02-2021
Elsevier BV
Subjects:
AlPO4:Eu3
Aluminum phosphate
Chromaticity
Color
Dopants
Europium
Judd-Ofelt intensity parameters
Orange-red-emitting phosphors
Phosphors
Quantum efficiency
Room temperature
Stability analysis
Symmetry
Thermal stability
Warm white LED
Orange-red-emitting phosphors
Warm white LED
Judd-Ofelt intensity parameters
AlPO4:Eu3
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Abstract Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows strong orange-red emissions with the strongest peaks at 588, 594, 685 and 700 nm. The highest PL intensity is achieved at the dopant concentration of 3 mol% and the annealing temperature of 1000 °C. Additionally, 84% of the room-temperature emission intensity is still maintained at 160 °C, indicating a good thermal stability and practicality. By a Judd-Ofelt (JO) analysis, it is demonstrated that the symmetry sites surrounding Eu3+ ions are influenced by the dopant level. The lowest value of Ω2/Ω4 ratio of 0.27 reveals the highest symmetry site at the Eu3+ concentration of 3 mol%. The CIE 1931 color chromaticity coordinates (x, y) and the activation energy of the AlPO4:3%Eu3+ phosphor are (0.5602; 0.3862) and 0.28 eV, respectively. The color coordinates of the phosphor coated on NUV LED chip and its quantum efficiency (QE) are (0.5573, 0.3253) and 38.7%, respectively. To the best of our knowledge, this is the first time that a calculated QE of AlPO4:Eu3+-based orange-red-emitting LED is reported. The obtained results show a great potential of using orange-red-emitting AlPO4:Eu3+ phosphor for WLED application. [Display omitted] •Orange-red-emitting AlPO4:Eu3+ phosphor is synthesized by a co-precipitation method.•The highest PL intensity is obtained at the annealing temperature of 1000 °C and the Eu3+ ions concentration of 3 mol%.•The highest symmetry site is found at the Eu3+ concentration of 3 mol% by a modified Judd-Ofelt analysis.•The color coordinates and quantum efficiency of phosphor-coated LED chip are (0.5573; 0.3253) and 38.7%, respectively.
AbstractList Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows strong orange-red emissions with the strongest peaks at 588, 594, 685 and 700 nm. The highest PL intensity is achieved at the dopant concentration of 3 mol% and the annealing temperature of 1000 °C. Additionally, 84% of the room-temperature emission intensity is still maintained at 160 °C, indicating a good thermal stability and practicality. By a Judd-Ofelt (JO) analysis, it is demonstrated that the symmetry sites surrounding Eu3+ ions are influenced by the dopant level. The lowest value of Ω2/Ω4 ratio of 0.27 reveals the highest symmetry site at the Eu3+ concentration of 3 mol%. The CIE 1931 color chromaticity coordinates (x, y) and the activation energy of the AlPO4:3%Eu3+ phosphor are (0.5602; 0.3862) and 0.28 eV, respectively. The color coordinates of the phosphor coated on NUV LED chip and its quantum efficiency (QE) are (0.5573, 0.3253) and 38.7%, respectively. To the best of our knowledge, this is the first time that a calculated QE of AlPO4:Eu3+-based orange-red-emitting LED is reported. The obtained results show a great potential of using orange-red-emitting AlPO4:Eu3+ phosphor for WLED application. [Display omitted] •Orange-red-emitting AlPO4:Eu3+ phosphor is synthesized by a co-precipitation method.•The highest PL intensity is obtained at the annealing temperature of 1000 °C and the Eu3+ ions concentration of 3 mol%.•The highest symmetry site is found at the Eu3+ concentration of 3 mol% by a modified Judd-Ofelt analysis.•The color coordinates and quantum efficiency of phosphor-coated LED chip are (0.5573; 0.3253) and 38.7%, respectively.
Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows strong orange-red emissions with the strongest peaks at 588, 594, 685 and 700 nm. The highest PL intensity is achieved at the dopant concentration of 3 mol% and the annealing temperature of 1000 °C. Additionally, 84% of the room-temperature emission intensity is still maintained at 160 °C, indicating a good thermal stability and practicality. By a Judd-Ofelt (JO) analysis, it is demonstrated that the symmetry sites surrounding Eu3+ ions are influenced by the dopant level. The lowest value of Ω2/Ω4 ratio of 0.27 reveals the highest symmetry site at the Eu3+ concentration of 3 mol%. The CIE 1931 color chromaticity coordinates (x, y) and the activation energy of the AlPO4:3%Eu3+ phosphor are (0.5602; 0.3862) and 0.28 eV, respectively. The color coordinates of the phosphor coated on NUV LED chip and its quantum efficiency (QE) are (0.5573, 0.3253) and 38.7%, respectively. To the best of our knowledge, this is the first time that a calculated QE of AlPO4:Eu3+-based orange-red-emitting LED is reported. The obtained results show a great potential of using orange-red-emitting AlPO4:Eu3+ phosphor for WLED application.
ArticleNumber 156941
Author Nguyen, D.H
Thu, L.T.H.
Tran, M.T.
Quang, N.V.
Trung, D.Q.
Tu, Nguyen
Huy, P.T.
Author_xml – sequence: 1
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  surname: Tran
  fullname: Tran, M.T.
  email: trung.tranmanh@phenikaa-uni.edu.vn, trungtm89@gmail.com
  organization: Faculty of Materials Science and Engineering, Phenikaa University, Yen Nghia Ha-Dong District, Hanoi, 10000, Viet Nam
– sequence: 2
  givenname: Nguyen
  surname: Tu
  fullname: Tu, Nguyen
  email: tu.nguyen@phenikaa-uni.edu.vn
  organization: Phenikaa Research and Technology Institute (PRATI), Phenikaa University, A&A Green Phoenix Group, 167 Hoang Ngan, Hanoi, 10000, Viet Nam
– sequence: 3
  givenname: N.V.
  surname: Quang
  fullname: Quang, N.V.
  email: nvquang201@gmail.com
  organization: Faculty of Chemistry, Hanoi Pedagogical University 2, Xuan Hoa, Vinh Phuc, Viet Nam
– sequence: 4
  givenname: D.H
  surname: Nguyen
  fullname: Nguyen, D.H
  email: hung.nguyenduy@hust.edu.vn
  organization: Advanced Institute for Science and Technology, Hanoi University of Science and Technology (HUST), 01 Dai Co Viet, Hai Ba Trung, Hanoi, 10000, Viet Nam
– sequence: 5
  givenname: L.T.H.
  surname: Thu
  fullname: Thu, L.T.H.
  email: thu.luuthiha@phenikaa-uni.edu.vn
  organization: Faculty of Materials Science and Engineering, Phenikaa University, Yen Nghia Ha-Dong District, Hanoi, 10000, Viet Nam
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  givenname: D.Q.
  surname: Trung
  fullname: Trung, D.Q.
  email: trung.doquang@phenikaa-uni.edu.vn
  organization: Phenikaa Research and Technology Institute (PRATI), Phenikaa University, A&A Green Phoenix Group, 167 Hoang Ngan, Hanoi, 10000, Viet Nam
– sequence: 7
  givenname: P.T.
  surname: Huy
  fullname: Huy, P.T.
  email: huy.phamthanh@phenikaa-uni.edu.vn
  organization: Faculty of Materials Science and Engineering, Phenikaa University, Yen Nghia Ha-Dong District, Hanoi, 10000, Viet Nam
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Keywords Orange-red-emitting phosphors
Warm white LED
Judd-Ofelt intensity parameters
AlPO4:Eu3
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Snippet Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows...
Orange-red-emitting AlPO4:Eu3+ phosphors have been systematically synthesized by a co-precipitation method. Under the excitation at 394 nm these phosphor shows...
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SubjectTerms AlPO4:Eu3
Aluminum phosphate
Chromaticity
Color
Dopants
Europium
Judd-Ofelt intensity parameters
Orange-red-emitting phosphors
Phosphors
Quantum efficiency
Room temperature
Stability analysis
Symmetry
Thermal stability
Warm white LED
Title Excellent thermal stability and high quantum efficiency orange-red-emitting AlPO4:Eu3+ phosphors for WLED application
URI https://dx.doi.org/10.1016/j.jallcom.2020.156941
https://www.proquest.com/docview/2469842765
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