Mechanisms for Enhancing Luminescence Yield in KBr Crystals under the Influence of Low-Temperature Uniaxial Elastic Deformation

This study investigates the radiative relaxation of electronic excitations through luminescence spectroscopy techniques applied to high-purity KBr crystals subjected to low-temperature (85 K) uniaxial deformation along the and crystallographic directions. Results demonstrate that the most significan...

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Published in:	Crystals (Basel) Vol. 14; no. 8; p. 698
Main Authors:	Shunkeyev, Kuanyshbek, Sagimbayeva, Shynar, Ubaev, Zhiger, Kenzhebayeva, Adelya
Format:	Journal Article
Language:	English
Published:	Basel MDPI AG 01-08-2024
Subjects:	Anion exchanging Charge exchange Crystal lattices Crystallography Crystals Elastic deformation Excitation spectra Excitons high-purity KBr crystal Investigations ionic crystal Low temperature Luminescence Luminescence quenching Radiation Raw materials self-trapped exciton Single crystals Temperature uniaxial deformation X-ray luminescence
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Abstract	This study investigates the radiative relaxation of electronic excitations through luminescence spectroscopy techniques applied to high-purity KBr crystals subjected to low-temperature (85 K) uniaxial deformation along the and crystallographic directions. Results demonstrate that the most significant enhancement in the intensity of σ-(4.42 eV) and π-(2.3 eV) luminescence from self-trapped excitons in KBr crystals occurs with elastic deformation along the direction, aligning with the axis of the hole component of the anion self-trapped exciton. Deformation-induced changes in X-ray, tunneling, and thermally stimulated luminescence spectra reveal a new band, denoted as Ex, peaking at approximately 3.58 eV, attributed to tunneling charge exchange between the F’- and VK-centers in their ground state.
AbstractList	This study investigates the radiative relaxation of electronic excitations through luminescence spectroscopy techniques applied to high-purity KBr crystals subjected to low-temperature (85 K) uniaxial deformation along the and crystallographic directions. Results demonstrate that the most significant enhancement in the intensity of σ-(4.42 eV) and π-(2.3 eV) luminescence from self-trapped excitons in KBr crystals occurs with elastic deformation along the direction, aligning with the axis of the hole component of the anion self-trapped exciton. Deformation-induced changes in X-ray, tunneling, and thermally stimulated luminescence spectra reveal a new band, denoted as Ex, peaking at approximately 3.58 eV, attributed to tunneling charge exchange between the F’- and VK-centers in their ground state.
Audience	Academic
Author	Sagimbayeva, Shynar Kenzhebayeva, Adelya Shunkeyev, Kuanyshbek Ubaev, Zhiger
Author_xml	– sequence: 1 givenname: Kuanyshbek orcidid: 0000-0002-3860-397X surname: Shunkeyev fullname: Shunkeyev, Kuanyshbek – sequence: 2 givenname: Shynar orcidid: 0000-0002-1234-3030 surname: Sagimbayeva fullname: Sagimbayeva, Shynar – sequence: 3 givenname: Zhiger orcidid: 0000-0002-8862-3506 surname: Ubaev fullname: Ubaev, Zhiger – sequence: 4 givenname: Adelya surname: Kenzhebayeva fullname: Kenzhebayeva, Adelya
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Snippet	This study investigates the radiative relaxation of electronic excitations through luminescence spectroscopy techniques applied to high-purity KBr crystals...
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SubjectTerms	Anion exchanging Charge exchange Crystal lattices Crystallography Crystals Elastic deformation Excitation spectra Excitons high-purity KBr crystal Investigations ionic crystal Low temperature Luminescence Luminescence quenching Radiation Raw materials self-trapped exciton Single crystals Temperature uniaxial deformation X-ray luminescence
Title	Mechanisms for Enhancing Luminescence Yield in KBr Crystals under the Influence of Low-Temperature Uniaxial Elastic Deformation
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