Comprehensive understanding of coupled stress characteristics in ytterbium disilicate environmental barrier coatings undergoing corrosion transformation and thermal cycling
Ytterbium disilicate (Yb2Si2O7, YbDS), with good thermal matching ability, is a promising candidate for environmental barrier coatings (EBCs). Nevertheless, cracking and delamination of the YbDS topcoat may occur in a flowing steam environment due to the corrosion transformation from YbDS to ytterbi...
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| Published in: | Ceramics international Vol. 48; no. 17; pp. 25528 - 25537 |
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| Main Authors: | , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Ltd
01-09-2022
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| Abstract | Ytterbium disilicate (Yb2Si2O7, YbDS), with good thermal matching ability, is a promising candidate for environmental barrier coatings (EBCs). Nevertheless, cracking and delamination of the YbDS topcoat may occur in a flowing steam environment due to the corrosion transformation from YbDS to ytterbium monosilicate (Yb2SiO5, YbMS). In this work, a scanning electron microscope (SEM)-based thermo-mechanical model, involving such corrosion transformation, is established to explore the stress characteristics in EBCs under the coupling effect of YbDS corrosion and thermal cycling. The main factors resulting in EBC failure during YbDS corrosion were also investigated. The results showed that compressive stress acted on the YbDS topcoat without a water vapor attack. However, the tensile stress occurred in the corroded YbDS coating after steam cycling. A large stress led to premature cracking of the EBC, thus providing channels for corrosive medium penetration. Volume shrinkage during YbDS corrosion dominated the stress magnitude in the corrosion zone. Furthermore, the increasing porosity caused a decrease in the Young's modulus and shrinkage strain of the corrosion zone, significantly affecting the EBC stress field. These findings not only enhance the comprehensive understanding of coupled stress characteristics in YbDS-EBCs, but also provide theoretical guidance for extending the EBC lifetime. |
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| AbstractList | Ytterbium disilicate (Yb2Si2O7, YbDS), with good thermal matching ability, is a promising candidate for environmental barrier coatings (EBCs). Nevertheless, cracking and delamination of the YbDS topcoat may occur in a flowing steam environment due to the corrosion transformation from YbDS to ytterbium monosilicate (Yb2SiO5, YbMS). In this work, a scanning electron microscope (SEM)-based thermo-mechanical model, involving such corrosion transformation, is established to explore the stress characteristics in EBCs under the coupling effect of YbDS corrosion and thermal cycling. The main factors resulting in EBC failure during YbDS corrosion were also investigated. The results showed that compressive stress acted on the YbDS topcoat without a water vapor attack. However, the tensile stress occurred in the corroded YbDS coating after steam cycling. A large stress led to premature cracking of the EBC, thus providing channels for corrosive medium penetration. Volume shrinkage during YbDS corrosion dominated the stress magnitude in the corrosion zone. Furthermore, the increasing porosity caused a decrease in the Young's modulus and shrinkage strain of the corrosion zone, significantly affecting the EBC stress field. These findings not only enhance the comprehensive understanding of coupled stress characteristics in YbDS-EBCs, but also provide theoretical guidance for extending the EBC lifetime. |
| Author | Han, Xuecheng Dong, Xiaoxue Huang, Yaping Wei, Zhiyuan Cai, Hongneng Zhang, Qiang |
| Author_xml | – sequence: 1 givenname: Yaping surname: Huang fullname: Huang, Yaping organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China – sequence: 2 givenname: Zhiyuan surname: Wei fullname: Wei, Zhiyuan organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China – sequence: 3 givenname: Qiang surname: Zhang fullname: Zhang, Qiang organization: AECC Beijing Institute of Aeronautical Materials, Huanshancun, Haidian District, Beijing, 100095, China – sequence: 4 givenname: Hongneng surname: Cai fullname: Cai, Hongneng email: hntsai@126.com organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China – sequence: 5 givenname: Xuecheng surname: Han fullname: Han, Xuecheng organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China – sequence: 6 givenname: Xiaoxue surname: Dong fullname: Dong, Xiaoxue organization: State Key Laboratory for Mechanical Behavior of Materials, School of Materials Science and Engineering, Xi'an Jiaotong University, Xi'an, 710049, China |
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| Keywords | Environmental barrier coatings YbDS corrosion Water vapor attack Porosity Volume shrinkage |
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| Title | Comprehensive understanding of coupled stress characteristics in ytterbium disilicate environmental barrier coatings undergoing corrosion transformation and thermal cycling |
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