Luminescence and Nonlinear Optical Properties of Borates LnGa3(BO3)4 (Ln = Nd, Sm, Tb, Er, Dy, or Ho)
Luminescence spectra of single crystals of rare-earth gallium borates LnGa 3 (BO 3 ) 4 (Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K) temperatures are presented for the first time. Photoluminescence has been recorded in the wavelength range of 470–5000 nm (2000–21 300 cm –1 )...
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| Published in: | Optics and spectroscopy Vol. 127; no. 1; pp. 107 - 112 |
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| Main Authors: | , , , , |
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| Language: | English |
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| Abstract | Luminescence spectra of single crystals of rare-earth gallium borates LnGa
3
(BO
3
)
4
(Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K) temperatures are presented for the first time. Photoluminescence has been recorded in the wavelength range of 470–5000 nm (2000–21 300 cm
–1
) with a high spectral resolution (down to 0.1 cm
–1
) upon excitation by different diode lasers. The spectra obtained cannot be unambiguously interpreted within one luminescent center, which can be due to the presence of defects and/or inclusions of other crystalline phases. The optical nonlinearity of rare-earth–gallium borates has been estimated using the Kurtz–Perry powder technique. The typical intensities of the second-harmonic generation in gallium borate powders are 30–40 (with respect to quartz), and the optical nonlinearity is as good as the nonlinearity of the efficient rare-earth aluminum borate YAl
3
(BO
3
)
4
. |
|---|---|
| AbstractList | Luminescence spectra of single crystals of rare-earth gallium borates LnGa
3
(BO
3
)
4
(Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K) temperatures are presented for the first time. Photoluminescence has been recorded in the wavelength range of 470–5000 nm (2000–21 300 cm
–1
) with a high spectral resolution (down to 0.1 cm
–1
) upon excitation by different diode lasers. The spectra obtained cannot be unambiguously interpreted within one luminescent center, which can be due to the presence of defects and/or inclusions of other crystalline phases. The optical nonlinearity of rare-earth–gallium borates has been estimated using the Kurtz–Perry powder technique. The typical intensities of the second-harmonic generation in gallium borate powders are 30–40 (with respect to quartz), and the optical nonlinearity is as good as the nonlinearity of the efficient rare-earth aluminum borate YAl
3
(BO
3
)
4
. Luminescence spectra of single crystals of rare-earth gallium borates LnGa3(BO3)4 (Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K) temperatures are presented for the first time. Photoluminescence has been recorded in the wavelength range of 470–5000 nm (2000–21 300 cm–1) with a high spectral resolution (down to 0.1 cm–1) upon excitation by different diode lasers. The spectra obtained cannot be unambiguously interpreted within one luminescent center, which can be due to the presence of defects and/or inclusions of other crystalline phases. The optical nonlinearity of rare-earth–gallium borates has been estimated using the Kurtz–Perry powder technique. The typical intensities of the second-harmonic generation in gallium borate powders are 30–40 (with respect to quartz), and the optical nonlinearity is as good as the nonlinearity of the efficient rare-earth aluminum borate YAl3(BO3)4. |
| Author | Boldyrev, K. N. Popova, M. N. Kuz’min, N. N. Stefanovich, S. Yu Leonyuk, N. I. |
| Author_xml | – sequence: 1 givenname: N. N. surname: Kuz’min fullname: Kuz’min, N. N. organization: Institute of Spectroscopy, Russian Academy of Sciences, Faculty of Geology, Moscow State University – sequence: 2 givenname: K. N. surname: Boldyrev fullname: Boldyrev, K. N. email: kn.boldyrev@gmail.com organization: Institute of Spectroscopy, Russian Academy of Sciences, National Research University Higher School of Economics – sequence: 3 givenname: N. I. surname: Leonyuk fullname: Leonyuk, N. I. organization: Faculty of Geology, Moscow State University – sequence: 4 givenname: S. Yu surname: Stefanovich fullname: Stefanovich, S. Yu organization: Faculty of Chemistry, Moscow State University – sequence: 5 givenname: M. N. surname: Popova fullname: Popova, M. N. organization: Institute of Spectroscopy, Russian Academy of Sciences |
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| Keywords | luminescence spectra rare-earth gallium borate crystals second-harmonic generation |
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| Snippet | Luminescence spectra of single crystals of rare-earth gallium borates LnGa
3
(BO
3
)
4
(Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K)... Luminescence spectra of single crystals of rare-earth gallium borates LnGa3(BO3)4 (Ln = Nd, Sm, Tb, Er, Dy, or Ho) at room (300 K) and cryogenic (10 K)... |
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| SubjectTerms | Aluminum Borates Cryogenic temperature Crystal defects Crystals Dysprosium Erbium Gallium Inclusions Lasers Luminescence Nonlinear optics Nonlinearity Optical Devices Optical Materials Optical properties Optics Photoluminescence Photonics Physics Physics and Astronomy Rare earth elements Second harmonic generation Semiconductor lasers Single crystals Spectra Spectral resolution Terbium |
| Title | Luminescence and Nonlinear Optical Properties of Borates LnGa3(BO3)4 (Ln = Nd, Sm, Tb, Er, Dy, or Ho) |
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