χ (3) measurements and optical limiting in dibenzylideneacetone and its derivatives
We investigated the third order nonlinear optical properties of dibenzylidene acetone (1,5-diphenyl-1, 4-pentadeine-3-one) and its derivatives. The nonlinear measurements were performed by using single beam Z-scan technique with Q-switched Nd:YAG nanosecond laser pulses at 532 nm. Open aperture data...
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| Published in: | Chemical physics Vol. 324; no. 2; pp. 699 - 704 |
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| Language: | English |
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31-05-2006
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| Abstract | We investigated the third order nonlinear optical properties of dibenzylidene acetone (1,5-diphenyl-1, 4-pentadeine-3-one) and its derivatives. The nonlinear measurements were performed by using single beam Z-scan technique with Q-switched Nd:YAG nanosecond laser pulses at 532
nm. Open aperture data for dibenzylidene and its derivatives demonstrate the presence of two-photon absorption at this wavelength. The dependence of
χ
(3) on donor/acceptor type substituents to the basic compound clearly shows the electronic origin of nonlinearity and hence demonstrates that the mechanism by which the third order nonlinear response enhanced is not by the thermal effects, but instead due to the strong nonlinear absorption and nonlinear refraction of the compounds. The derivatives of the basic compound show very good optical limiting behavior. |
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| AbstractList | We investigated the third order nonlinear optical properties of dibenzylidene acetone (1,5-diphenyl-1, 4-pentadeine-3-one) and its derivatives. The nonlinear measurements were performed by using single beam Z-scan technique with Q-switched Nd:YAG nanosecond laser pulses at 532
nm. Open aperture data for dibenzylidene and its derivatives demonstrate the presence of two-photon absorption at this wavelength. The dependence of
χ
(3) on donor/acceptor type substituents to the basic compound clearly shows the electronic origin of nonlinearity and hence demonstrates that the mechanism by which the third order nonlinear response enhanced is not by the thermal effects, but instead due to the strong nonlinear absorption and nonlinear refraction of the compounds. The derivatives of the basic compound show very good optical limiting behavior. |
| Author | Kalluraya, Balakrishna Chandrasekharan, K. Umesh, G. Kiran, A. John Shashikala, H.D. Nooji, Satheesh Rai |
| Author_xml | – sequence: 1 givenname: A. John surname: Kiran fullname: Kiran, A. John email: jk_swe@rediffmail.com organization: Department of Physics, National Institute of Technology Karnataka, Surathkal, Srinivasnagar D.K, Mangalore, Karnataka 575 025, India – sequence: 2 givenname: K. surname: Chandrasekharan fullname: Chandrasekharan, K. organization: Department of Physics, National Institute of Technology Karnataka, Surathkal, Srinivasnagar D.K, Mangalore, Karnataka 575 025, India – sequence: 3 givenname: Satheesh Rai surname: Nooji fullname: Nooji, Satheesh Rai organization: Department of Chemistry, Mangalore University, Karnataka 574 199, India – sequence: 4 givenname: H.D. surname: Shashikala fullname: Shashikala, H.D. email: hds@nitk.ac.in organization: Department of Physics, National Institute of Technology Karnataka, Surathkal, Srinivasnagar D.K, Mangalore, Karnataka 575 025, India – sequence: 5 givenname: G. surname: Umesh fullname: Umesh, G. organization: Department of Physics, National Institute of Technology Karnataka, Surathkal, Srinivasnagar D.K, Mangalore, Karnataka 575 025, India – sequence: 6 givenname: Balakrishna surname: Kalluraya fullname: Kalluraya, Balakrishna organization: Department of Chemistry, Mangalore University, Karnataka 574 199, India |
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| Keywords | Optical limiting Nonlinear absorption Z-scan Nonlinear optics Nonlinear refraction Optical susceptibility |
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| SubjectTerms | Nonlinear absorption Nonlinear optics Nonlinear refraction Optical limiting Optical susceptibility Z-scan |
| Title | χ (3) measurements and optical limiting in dibenzylideneacetone and its derivatives |
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