Tannic acid etching construction of hollow heterogeneous CoSe2-FeSe2@nitrogen-doped carbon rhombic dodecahedron for high-performance sodium storage
[Display omitted] •Tannic acid etching construction of CoSe2-FeSe2@NC with rhombic dodecahedron.•The hollow rhombic dodecahedron can reduce the Na+/electron migration path.•The hollow rhombic dodecahedron can alleviate the volume variations during cycling.•The BIEF at the heterointerfaces can accele...
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| Published in: | Journal of colloid and interface science Vol. 679; no. Pt B; pp. 40 - 49 |
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| Main Authors: | , , , , , , , , |
| Format: | Journal Article |
| Language: | English |
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Elsevier Inc
01-02-2025
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| Abstract | [Display omitted]
•Tannic acid etching construction of CoSe2-FeSe2@NC with rhombic dodecahedron.•The hollow rhombic dodecahedron can reduce the Na+/electron migration path.•The hollow rhombic dodecahedron can alleviate the volume variations during cycling.•The BIEF at the heterointerfaces can accelerate the kinetics of ionic diffusion.•The CoSe2-FeSe2@NC exhibits a remarkable electrochemical performance.
Metal selenides are very promising anode materials for sodium ion batteries (SIBs) due to their rich redox behaviors, low cost, high theoretical capacity, and environmentally benign. However, the poor cycle performance and rate capability greatly hinder their widespread applications. In this paper, we have proposed a tannic acid etching zeolitic imidazolate framework-67 (ZIF-67)-derived selenide strategy to construct hollow heterogeneous CoSe2-FeSe2@N-doped carbon rhombic dodecahedron (CoSe2-FeSe2@NC) as anode for high-performance SIBs. The special microstructural characteristics with hollow rhombic dodecahedron can reduce the Na+/electron migration path and alleviate the volume variations during cycling. The NC can improve conductivity and reduce volume effects during cycling. What’s more, the built-in electric fields (BIEF) at the CoSe2-FeSe2 heterointerfaces can modulate the electronic structure and accelerate the kinetics of ionic diffusion, resulting in the improvement electrochemical properties. When applied as anodes for SIBs, the CoSe2-FeSe2@NC can deliver a remarkable electrochemical performance in terms of sodium storage capacity (648.5 mAh g−1 at 0.2 A/g), initial coulombic efficiency (82.0 %), cycle performance (92.6 % capacity retention after 100 cycles), and rate capability of 450.6 mAh g−1 after 1000 cycles at a high rate of 1 A/g. The kinetic analysis indicates that the discharging-charging process of CoSe2-FeSe2@NC is ascribed to both capacitive behavior and controlled diffusion. |
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| AbstractList | Metal selenides are very promising anode materials for sodium ion batteries (SIBs) due to their rich redox behaviors, low cost, high theoretical capacity, and environmentally benign. However, the poor cycle performance and rate capability greatly hinder their widespread applications. In this paper, we have proposed a tannic acid etching zeolitic imidazolate framework-67 (ZIF-67)-derived selenide strategy to construct hollow heterogeneous CoSe2-FeSe2@N-doped carbon rhombic dodecahedron (CoSe2-FeSe2@NC) as anode for high-performance SIBs. The special microstructural characteristics with hollow rhombic dodecahedron can reduce the Na+/electron migration path and alleviate the volume variations during cycling. The NC can improve conductivity and reduce volume effects during cycling. What's more, the built-in electric fields (BIEF) at the CoSe2-FeSe2 heterointerfaces can modulate the electronic structure and accelerate the kinetics of ionic diffusion, resulting in the improvement electrochemical properties. When applied as anodes for SIBs, the CoSe2-FeSe2@NC can deliver a remarkable electrochemical performance in terms of sodium storage capacity (648.5 mAh g-1 at 0.2 A/g), initial coulombic efficiency (82.0 %), cycle performance (92.6 % capacity retention after 100 cycles), and rate capability of 450.6 mAh g-1 after 1000 cycles at a high rate of 1 A/g. The kinetic analysis indicates that the discharging-charging process of CoSe2-FeSe2@NC is ascribed to both capacitive behavior and controlled diffusion.Metal selenides are very promising anode materials for sodium ion batteries (SIBs) due to their rich redox behaviors, low cost, high theoretical capacity, and environmentally benign. However, the poor cycle performance and rate capability greatly hinder their widespread applications. In this paper, we have proposed a tannic acid etching zeolitic imidazolate framework-67 (ZIF-67)-derived selenide strategy to construct hollow heterogeneous CoSe2-FeSe2@N-doped carbon rhombic dodecahedron (CoSe2-FeSe2@NC) as anode for high-performance SIBs. The special microstructural characteristics with hollow rhombic dodecahedron can reduce the Na+/electron migration path and alleviate the volume variations during cycling. The NC can improve conductivity and reduce volume effects during cycling. What's more, the built-in electric fields (BIEF) at the CoSe2-FeSe2 heterointerfaces can modulate the electronic structure and accelerate the kinetics of ionic diffusion, resulting in the improvement electrochemical properties. When applied as anodes for SIBs, the CoSe2-FeSe2@NC can deliver a remarkable electrochemical performance in terms of sodium storage capacity (648.5 mAh g-1 at 0.2 A/g), initial coulombic efficiency (82.0 %), cycle performance (92.6 % capacity retention after 100 cycles), and rate capability of 450.6 mAh g-1 after 1000 cycles at a high rate of 1 A/g. The kinetic analysis indicates that the discharging-charging process of CoSe2-FeSe2@NC is ascribed to both capacitive behavior and controlled diffusion. [Display omitted] •Tannic acid etching construction of CoSe2-FeSe2@NC with rhombic dodecahedron.•The hollow rhombic dodecahedron can reduce the Na+/electron migration path.•The hollow rhombic dodecahedron can alleviate the volume variations during cycling.•The BIEF at the heterointerfaces can accelerate the kinetics of ionic diffusion.•The CoSe2-FeSe2@NC exhibits a remarkable electrochemical performance. Metal selenides are very promising anode materials for sodium ion batteries (SIBs) due to their rich redox behaviors, low cost, high theoretical capacity, and environmentally benign. However, the poor cycle performance and rate capability greatly hinder their widespread applications. In this paper, we have proposed a tannic acid etching zeolitic imidazolate framework-67 (ZIF-67)-derived selenide strategy to construct hollow heterogeneous CoSe2-FeSe2@N-doped carbon rhombic dodecahedron (CoSe2-FeSe2@NC) as anode for high-performance SIBs. The special microstructural characteristics with hollow rhombic dodecahedron can reduce the Na+/electron migration path and alleviate the volume variations during cycling. The NC can improve conductivity and reduce volume effects during cycling. What’s more, the built-in electric fields (BIEF) at the CoSe2-FeSe2 heterointerfaces can modulate the electronic structure and accelerate the kinetics of ionic diffusion, resulting in the improvement electrochemical properties. When applied as anodes for SIBs, the CoSe2-FeSe2@NC can deliver a remarkable electrochemical performance in terms of sodium storage capacity (648.5 mAh g−1 at 0.2 A/g), initial coulombic efficiency (82.0 %), cycle performance (92.6 % capacity retention after 100 cycles), and rate capability of 450.6 mAh g−1 after 1000 cycles at a high rate of 1 A/g. The kinetic analysis indicates that the discharging-charging process of CoSe2-FeSe2@NC is ascribed to both capacitive behavior and controlled diffusion. |
| Author | Sun, Zhihua Zhou, Bo Chen, Lizhuang Chen, Yingying Fu, Xueying Yang, Hongxun Tian, Hao Sun, Dongya Li, Yanjiao |
| Author_xml | – sequence: 1 givenname: Hao surname: Tian fullname: Tian, Hao organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 2 givenname: Yanjiao surname: Li fullname: Li, Yanjiao organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 3 givenname: Zhihua surname: Sun fullname: Sun, Zhihua organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 4 givenname: Xueying surname: Fu fullname: Fu, Xueying organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 5 givenname: Lizhuang surname: Chen fullname: Chen, Lizhuang organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 6 givenname: Yingying surname: Chen fullname: Chen, Yingying organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China – sequence: 7 givenname: Dongya surname: Sun fullname: Sun, Dongya organization: Key Laboratory of Functional Materials and Applications of Fujian Province, School of Materials Science and Engineering, Xiamen University of Technology, Xiamen 361024, PR China – sequence: 8 givenname: Bo surname: Zhou fullname: Zhou, Bo organization: School of Life Science, Jilin Normal University, Siping 136000, Jilin, PR China – sequence: 9 givenname: Hongxun surname: Yang fullname: Yang, Hongxun email: yhongxun@just.edu.cn organization: School of Environmental & Chemical Engineering, Jiangsu University of Science and Technology, Zhenjiang 212003, Jiangsu, PR China |
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| Keywords | Sodium ion batteries N-doped carbon Anode CoSe2-FeSe2 Metal selenides |
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•Tannic acid etching construction of CoSe2-FeSe2@NC with rhombic dodecahedron.•The hollow rhombic dodecahedron can reduce the Na+/electron... Metal selenides are very promising anode materials for sodium ion batteries (SIBs) due to their rich redox behaviors, low cost, high theoretical capacity, and... |
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| SubjectTerms | Anode CoSe2-FeSe2 Metal selenides N-doped carbon Sodium ion batteries |
| Title | Tannic acid etching construction of hollow heterogeneous CoSe2-FeSe2@nitrogen-doped carbon rhombic dodecahedron for high-performance sodium storage |
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