Measurement of fission products yields in the quasi-mono-energetic neutron-induced fission of 232Th

• Published in: Nuclear physics. A Vol. 952; pp. 100 - 120
• Main Authors: Naik, H., Mukherji, Sadhana, Suryanarayana, S.V., Jagadeesan, K.C., Thakare, S.V., Sharma, S.C.
• Format: Journal Article
• Language: English
• Published: Elsevier B.V 01-08-2016
• Subjects: 232Th(n, F); 7.75, 9.35 and 12.53 MeV; formula omitted; mass yield distributions; measured fission product yields; Nuclear reactions; Off-line γ-ray spectrometric technique; mass yield distributions; measured fission product yields; 7.75, 9.35 and 12.53 MeV; 232Th(n, F); En=5.42; Nuclear reactions; Off-line γ-ray spectrometric technique
• ISSN: 0375-9474
• DOI: 10.1016/j.nuclphysa.2016.04.003

The cumulative yields of various fission products in the 232Th(n, f) reaction at average neutron energies of 5.42, 7.75, 9.35 and 12.53 MeV have been determined by using an off-line γ-ray spectrometric technique. The neutron beam was produced from the 7Li(p, n) reaction by using the proton energies of 7.8, 12, 16 and 20 MeV. The mass chain yields were obtained from the cumulative fission yields by using the charge distribution correction of medium energy fission. The fine structure in the mass yield distribution was interpreted from the point of nuclear structure effect. On the other hand, the higher yield around mass number 133–134 and 143–144 as well as their complementary products were explained based on the standard I and standard II asymmetric mode of fission. From the mass yield data, the average value of light mass (〈AL〉), heavy mass (〈AH〉), the average number of neutrons (〈ν〉) and the peak-to-valley (P/V) ratios at different neutron energies of present work and literature data were obtained in the 232Th(n, f) reaction. The different parameters of the mass yield distribution in the 232Th(n, f) reaction were compared with the similar data in the 232Th(γ, f) reaction at comparable excitation energy and a surprising difference was observed.
•Yields of fission products in 5.42, 7.75, 9.35 and 12.53 MeV neutron induced fission of 232Th.•It is important for decay heat calculation and thus design of AHWR and ADSs.•The mass yields in the 232Th(n, f) reaction are important for nuclear structure effect and see the difference of 232Th(n, f) and 232Th(γ, f) reactions from the point of one neutron difference of the compound nucleus.