Energy and Photoinduced Electron Transfer in a Wheel-Shaped Artificial Photosynthetic Antenna-Reaction Center Complex

Functional mimics of a photosynthetic antenna-reaction center complex comprising five bis(phenylethynyl)anthracene antenna moieties and a porphyrin−fullerene dyad organized by a central hexaphenylbenzene core have been prepared and studied spectroscopically. The molecules successfully integrate sing...

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Bibliographic Details
Published in:	Journal of the American Chemical Society Vol. 128; no. 6; pp. 1818 - 1827
Main Authors:	Kodis, Gerdenis, Terazono, Yuichi, Liddell, Paul A, Andréasson, Joakim, Garg, Vikas, Hambourger, Michael, Moore, Thomas A, Moore, Ana L, Gust, Devens
Format:	Journal Article
Language:	English
Published:	Washington, DC American Chemical Society 15-02-2006
Subjects:	Anthracenes - chemical synthesis Anthracenes - chemistry Atomic and molecular physics Biomimetic Materials - chemical synthesis Biomimetic Materials - chemistry Electrons Exact sciences and technology Fluorescence and phosphorescence; radiationless transitions, quenching (intersystem crossing, internal conversion) Kinetics Molecular properties and interactions with photons Photochemistry Photosynthetic Reaction Center Complex Proteins - chemical synthesis Photosynthetic Reaction Center Complex Proteins - chemistry Physics Porphyrins - chemical synthesis Porphyrins - chemistry Radiationless transitions, quenching Spectrophotometry, Ultraviolet Fluorescence spectroscopy Fullerene compounds Light harvesting system Photosynthetic reaction centers Electron transfer Radiative lifetimes Experimental study Quantum yield Non metal porphyrin Luminescence decay Iron Organic compounds Biomimetic compound Molecular complex Energy transfer Ultraviolet visible spectrometry
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