Enhanced LED Performance by Ion Migration in Multiple Quantum Well Perovskite

Enhanced LED Performance by Ion Migration in Multiple Quantum Well Perovskite

Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in Ruddlesden-Popper and Dion-Jacobson two-dimensional perovskites having multiple quantum well (MQW) structures. PeLED devices were fabricated...

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Published in:The journal of physical chemistry letters Vol. 14; no. 51; pp. 11610 - 11617
Main Authors: Yudco, Shir, Bisquert, Juan, Etgar, Lioz
Format: Journal Article
Language:English
Published: United States American Chemical Society 28-12-2023
Subjects:
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Physical Insights into Materials and Molecular Properties
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Abstract Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in Ruddlesden-Popper and Dion-Jacobson two-dimensional perovskites having multiple quantum well (MQW) structures. PeLED devices were fabricated by using the same conditions and architecture, while their electroluminescence properties and ion migration behavior were investigated. Impedance spectroscopy measurements were used to analyze the PeLEDs, which found a direct link between the barrier molecule type, the device efficiency, and ion migration. The best performing LEDs were based on the aromatic barriers, which present dominant inductive impedance, indicating an earlier onset voltage of radiative recombination. These findings present an approach of how to control radiative emission in perovskite LEDs which opens the way for further improvement in PeLEDs and memristors.
AbstractList Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in Ruddlesden-Popper and Dion-Jacobson two-dimensional perovskites having multiple quantum well (MQW) structures. PeLED devices were fabricated by using the same conditions and architecture, while their electroluminescence properties and ion migration behavior were investigated. Impedance spectroscopy measurements were used to analyze the PeLEDs, which found a direct link between the barrier molecule type, the device efficiency, and ion migration. The best performing LEDs were based on the aromatic barriers, which present dominant inductive impedance, indicating an earlier onset voltage of radiative recombination. These findings present an approach of how to control radiative emission in perovskite LEDs which opens the way for further improvement in PeLEDs and memristors.
Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in Ruddlesden-Popper and Dion-Jacobson two-dimensional perovskites having multiple quantum well (MQW) structures. PeLED devices were fabricated by using the same conditions and architecture, while their electroluminescence properties and ion migration behavior were investigated. Impedance spectroscopy measurements were used to analyze the PeLEDs, which found a direct link between the barrier molecule type, the device efficiency, and ion migration. The best performing LEDs were based on the aromatic barriers, which present dominant inductive impedance, indicating an earlier onset voltage of radiative recombination. These findings present an approach of how to control radiative emission in perovskite LEDs which opens the way for further improvement in PeLEDs and memristors.
Author Etgar, Lioz
Yudco, Shir
Bisquert, Juan
AuthorAffiliation Institute of Chemistry, Casali Center for Applied Chemistry and the Center for Nanoscience and Nanotechnology
Institute of Advanced Materials (INAM)
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  givenname: Shir
  surname: Yudco
  fullname: Yudco, Shir
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  givenname: Juan
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  surname: Bisquert
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  givenname: Lioz
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  surname: Etgar
  fullname: Etgar, Lioz
  email: lioz.etgar@mail.huji.ac.il
  organization: Institute of Chemistry, Casali Center for Applied Chemistry and the Center for Nanoscience and Nanotechnology
BackLink https://www.ncbi.nlm.nih.gov/pubmed/38100371$$D View this record in MEDLINE/PubMed
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Snippet Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in...
Here we study the effect of ion migration on the performance of perovskite light emitting diodes (PeLEDs). We compared aromatic and linear barrier molecules in...
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Physical Insights into Materials and Molecular Properties
Title Enhanced LED Performance by Ion Migration in Multiple Quantum Well Perovskite
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