Local Structure of the Zeolitic Catalytically Active Site during Reaction

The structural changes of the catalytic active site that occur during catalytic reaction in an acidic zeolite are detected. The local structure of the zeolitic Brønsted active site is a distorted tetrahedrally coordinated aluminum that has three short and one long aluminum−oxygen bond. Using in situ...

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Bibliographic Details
Published in:	Journal of the American Chemical Society Vol. 126; no. 14; pp. 4506 - 4507
Main Authors:	van Bokhoven, Jeroen A, van der Eerden, Ad M. J, Prins, Roel
Format:	Journal Article
Language:	English
Published:	Washington, DC American Chemical Society 14-04-2004
Subjects:	Catalysis Catalytic reactions Chemistry Exact sciences and technology General and physical chemistry Theory of reactions, general kinetics. Catalysis. Nomenclature, chemical documentation, computer chemistry Ammonium Catalytic reaction Oligomerization Hydrocarbon Ethylene Aluminosilicates Modified catalyst Experimental study EXAFS spectrometry Molecular sieve Local structure Catalytic site Ion exchange Catalyst activity
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