New Insights into Single-Molecule Junctions Using a Robust, Unsupervised Approach to Data Collection and Analysis
We have applied a new, robust and unsupervised approach to data collection, sorting and analysis that provides fresh insights into the nature of single-molecule junctions. Automation of tunneling current-distance (I(s)) spectroscopy facilitates the collection of very large data sets (up to 100 000 t...
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| Published in: | Journal of the American Chemical Society Vol. 137; no. 31; pp. 9971 - 9981 |
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| Main Authors: | , , , , , , |
| Format: | Journal Article |
| Language: | English |
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American Chemical Society
12-08-2015
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| Abstract | We have applied a new, robust and unsupervised approach to data collection, sorting and analysis that provides fresh insights into the nature of single-molecule junctions. Automation of tunneling current-distance (I(s)) spectroscopy facilitates the collection of very large data sets (up to 100 000 traces for a single experiment), enabling comprehensive statistical interrogations with respect to underlying tunneling characteristics, noise and junction formation probability (JFP). We frequently observe unusual low-to-high through-molecule conductance features with increasing electrode separation, in addition to numerous other “plateau” shapes, which may be related to changes in interfacial or molecular bridge structure. Furthermore, for the first time we use the JFP to characterize the homogeneity of functionalized surfaces at the nanoscale. |
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| AbstractList | We have applied a new, robust and unsupervised approach to data collection, sorting and analysis that provides fresh insights into the nature of single-molecule junctions. Automation of tunneling current-distance (I(s)) spectroscopy facilitates the collection of very large data sets (up to 100,000 traces for a single experiment), enabling comprehensive statistical interrogations with respect to underlying tunneling characteristics, noise and junction formation probability (JFP). We frequently observe unusual low-to-high through-molecule conductance features with increasing electrode separation, in addition to numerous other "plateau" shapes, which may be related to changes in interfacial or molecular bridge structure. Furthermore, for the first time we use the JFP to characterize the homogeneity of functionalized surfaces at the nanoscale. |
| Author | Inkpen, Michael S Lemmer, Mario Long, Nicholas J Milan, David C Fitzpatrick, Nathan Nichols, Richard J Albrecht, Tim |
| AuthorAffiliation | Department of Chemistry University of Liverpool Imperial College London |
| AuthorAffiliation_xml | – name: University of Liverpool – name: Department of Chemistry – name: Imperial College London |
| Author_xml | – sequence: 1 givenname: Michael S surname: Inkpen fullname: Inkpen, Michael S email: michael.inkpen08@imperial.ac.uk – sequence: 2 givenname: Mario surname: Lemmer fullname: Lemmer, Mario – sequence: 3 givenname: Nathan surname: Fitzpatrick fullname: Fitzpatrick, Nathan – sequence: 4 givenname: David C surname: Milan fullname: Milan, David C – sequence: 5 givenname: Richard J surname: Nichols fullname: Nichols, Richard J – sequence: 6 givenname: Nicholas J surname: Long fullname: Long, Nicholas J email: n.long@imperial.ac.uk – sequence: 7 givenname: Tim surname: Albrecht fullname: Albrecht, Tim email: t.albrecht@imperial.ac.uk |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/26181714$$D View this record in MEDLINE/PubMed |
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| Title | New Insights into Single-Molecule Junctions Using a Robust, Unsupervised Approach to Data Collection and Analysis |
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