Graphene-Induced Substrate Decoupling and Ideal Doping of a Self-Assembled Iron-phthalocyanine Single Layer

Iron-phthalocyanine molecules self-assemble on the moiré pattern of graphene/Ir(111) as a flat and weakly interacting layer, as determined by core-level photoemission and absorption spectroscopy. The graphene buffer layer decouples the FePc two-dimensional structure from the underlying metal; the e...

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Published in:	Journal of physical chemistry. C Vol. 117; no. 6; pp. 3019 - 3027
Main Authors:	Scardamaglia, Mattia, Lisi, Simone, Lizzit, Silvano, Baraldi, Alessandro, Larciprete, Rosanna, Mariani, Carlo, Betti, Maria Grazia
Format:	Journal Article
Language:	English
Published:	Columbus, OH American Chemical Society 14-02-2013
Subjects:	Cross-disciplinary physics: materials science; rheology Exact sciences and technology Materials science Methods of nanofabrication Physics Self-assembly Moire fringes Self-assembled layers Coverage rate Core levels Thin films Self-assembly Electronic structure Iron complexes Graphene Metallophthalocyanine Free-standing film Absorption spectra X-ray photoelectron spectra
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Abstract	Iron-phthalocyanine molecules self-assemble on the moiré pattern of graphene/Ir(111) as a flat and weakly interacting layer, as determined by core-level photoemission and absorption spectroscopy. The graphene buffer layer decouples the FePc two-dimensional structure from the underlying metal; the electronic structure of the FePc molecular macrocycles is preserved; and the Fe-L2,3 edges present narrower and slightly modified resonances at the FePc single-layer coverage with respect to a thin film. The FePc layer induces a slight electron doping to the Ir-supported graphene resulting in the Dirac cone position expected for an ideal free-standing-like graphene layer with the standard Fermi velocity.
AbstractList	Iron-phthalocyanine molecules self-assemble on the moiré pattern of graphene/Ir(111) as a flat and weakly interacting layer, as determined by core-level photoemission and absorption spectroscopy. The graphene buffer layer decouples the FePc two-dimensional structure from the underlying metal; the electronic structure of the FePc molecular macrocycles is preserved; and the Fe-L2,3 edges present narrower and slightly modified resonances at the FePc single-layer coverage with respect to a thin film. The FePc layer induces a slight electron doping to the Ir-supported graphene resulting in the Dirac cone position expected for an ideal free-standing-like graphene layer with the standard Fermi velocity.
Author	Mariani, Carlo Scardamaglia, Mattia Lisi, Simone Lizzit, Silvano Baraldi, Alessandro Larciprete, Rosanna Betti, Maria Grazia
AuthorAffiliation	Università di Roma La Sapienza University of Trieste Sincrotrone Trieste IOM-CNR Laboratorio TASC CNR-ISC
AuthorAffiliation_xml	– name: University of Trieste – name: IOM-CNR Laboratorio TASC – name: Sincrotrone Trieste – name: Università di Roma La Sapienza – name: CNR-ISC
Author_xml	– sequence: 1 givenname: Mattia surname: Scardamaglia fullname: Scardamaglia, Mattia email: mattia.scardamaglia@roma1.infn.it, carlo.mariani@uniroma1.it – sequence: 2 givenname: Simone surname: Lisi fullname: Lisi, Simone – sequence: 3 givenname: Silvano surname: Lizzit fullname: Lizzit, Silvano – sequence: 4 givenname: Alessandro surname: Baraldi fullname: Baraldi, Alessandro – sequence: 5 givenname: Rosanna surname: Larciprete fullname: Larciprete, Rosanna – sequence: 6 givenname: Carlo surname: Mariani fullname: Mariani, Carlo email: mattia.scardamaglia@roma1.infn.it, carlo.mariani@uniroma1.it – sequence: 7 givenname: Maria Grazia surname: Betti fullname: Betti, Maria Grazia
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Keywords	Moire fringes Self-assembled layers Coverage rate Core levels Thin films Self-assembly Electronic structure Iron complexes Graphene Metallophthalocyanine Free-standing film Absorption spectra X-ray photoelectron spectra
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Snippet	Iron-phthalocyanine molecules self-assemble on the moiré pattern of graphene/Ir(111) as a flat and weakly interacting layer, as determined by core-level...
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SubjectTerms	Cross-disciplinary physics: materials science; rheology Exact sciences and technology Materials science Methods of nanofabrication Physics Self-assembly
Title	Graphene-Induced Substrate Decoupling and Ideal Doping of a Self-Assembled Iron-phthalocyanine Single Layer
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