Chiroselective Assembly of a Chiral Porphyrin−Fullerene Dyad: Photoconductive Nanofiber with a Top-Class Ambipolar Charge-Carrier Mobility
Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin−fullerene dyad 1 in CH2Cl2 self-assembles at 25 °C into nanofibers with a built-in donor/acceptor heterojunction, while its racemic form, under identical conditions, self-assembles into submicrometer-sized sp...
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| Published in: | Journal of the American Chemical Society Vol. 132; no. 19; pp. 6628 - 6629 |
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19-05-2010
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| Abstract | Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin−fullerene dyad 1 in CH2Cl2 self-assembles at 25 °C into nanofibers with a built-in donor/acceptor heterojunction, while its racemic form, under identical conditions, self-assembles into submicrometer-sized spheres with a donor/acceptor arrangement essentially different from that in the nanofiber assembly. Although a cast film of the latter hardly shows a photoconducting profile on micrometer-gap electrodes, the former sample clearly displays photoconduction with an ambipolar charge-transporting character. The electron and hole mobilities under zero electric field, as estimated from time-of-flight profiles, are 0.14 and 0.10 cm2 V−1 s−1, respectively, which are comparable to or even better than those reported for top-class organic materials with a donor/acceptor heterojunction. |
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| AbstractList | Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin-fullerene dyad 1 in CH(2)Cl(2) self-assembles at 25 degrees C into nanofibers with a built-in donor/acceptor heterojunction, while its racemic form, under identical conditions, self-assembles into submicrometer-sized spheres with a donor/acceptor arrangement essentially different from that in the nanofiber assembly. Although a cast film of the latter hardly shows a photoconducting profile on micrometer-gap electrodes, the former sample clearly displays photoconduction with an ambipolar charge-transporting character. The electron and hole mobilities under zero electric field, as estimated from time-of-flight profiles, are 0.14 and 0.10 cm(2) V(-1) s(-1), respectively, which are comparable to or even better than those reported for top-class organic materials with a donor/acceptor heterojunction. Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin−fullerene dyad 1 in CH2Cl2 self-assembles at 25 °C into nanofibers with a built-in donor/acceptor heterojunction, while its racemic form, under identical conditions, self-assembles into submicrometer-sized spheres with a donor/acceptor arrangement essentially different from that in the nanofiber assembly. Although a cast film of the latter hardly shows a photoconducting profile on micrometer-gap electrodes, the former sample clearly displays photoconduction with an ambipolar charge-transporting character. The electron and hole mobilities under zero electric field, as estimated from time-of-flight profiles, are 0.14 and 0.10 cm2 V−1 s−1, respectively, which are comparable to or even better than those reported for top-class organic materials with a donor/acceptor heterojunction. |
| Author | Hizume, Yumi Tashiro, Kentaro Yamamoto, Yohei Seki, Shu Saeki, Akinori Aida, Takuzo Charvet, Richard |
| Author_xml | – sequence: 1 givenname: Yumi surname: Hizume fullname: Hizume, Yumi – sequence: 2 givenname: Kentaro surname: Tashiro fullname: Tashiro, Kentaro email: aida@macro.t.u-tokyo.ac.jp, tashiro.kentaro@nims.go.jp, racharvet@yahoo.com – sequence: 3 givenname: Richard surname: Charvet fullname: Charvet, Richard email: aida@macro.t.u-tokyo.ac.jp, tashiro.kentaro@nims.go.jp, racharvet@yahoo.com – sequence: 4 givenname: Yohei surname: Yamamoto fullname: Yamamoto, Yohei – sequence: 5 givenname: Akinori surname: Saeki fullname: Saeki, Akinori – sequence: 6 givenname: Shu surname: Seki fullname: Seki, Shu – sequence: 7 givenname: Takuzo surname: Aida fullname: Aida, Takuzo email: aida@macro.t.u-tokyo.ac.jp, tashiro.kentaro@nims.go.jp, racharvet@yahoo.com |
| BackLink | https://www.ncbi.nlm.nih.gov/pubmed/20423102$$D View this record in MEDLINE/PubMed |
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| Snippet | Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin−fullerene dyad 1 in CH2Cl2 self-assembles at 25 °C into nanofibers... Upon slow admission of MeOH, the enantiomerically pure form of chiral amphiphilic porphyrin-fullerene dyad 1 in CH(2)Cl(2) self-assembles at 25 degrees C into... |
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| Title | Chiroselective Assembly of a Chiral Porphyrin−Fullerene Dyad: Photoconductive Nanofiber with a Top-Class Ambipolar Charge-Carrier Mobility |
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