Search Results - "Utschig, Lisa"
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Preface to the special issue: photosynthesis-inspired biohybrid and biomimetic systems
Published in Photosynthesis research (01-02-2020)“…Research of Photosynthetic-Inspired Biohybrid and Biomimetic Systems has gained significant momentum in recent years as an approach to both study and use solar…”
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Modular Homogeneous Chromophore–Catalyst Assemblies
Published in Accounts of chemical research (17-05-2016)“…Photosynthetic reaction center (RC) proteins convert incident solar energy to chemical energy through a network of molecular cofactors which have been…”
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Quantum Sensing of Electron Transfer Pathways in Natural Photosynthesis Using Time-Resolved High-Field Electron Paramagnetic Resonance/Electron–Nuclear Double Resonance Spectroscopy
Published in The journal of physical chemistry. B (29-04-2021)“…Photosynthetic integral membrane reaction center (RC) proteins capture and convert sunlight into chemical energy via efficient charge separation achieved…”
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Nature-Driven Photochemistry for Catalytic Solar Hydrogen Production: A Photosystem I–Transition Metal Catalyst Hybrid
Published in Journal of the American Chemical Society (19-10-2011)“…Solar energy conversion of water into the environmentally clean fuel hydrogen offers one of the best long-term solutions for meeting future energy demands…”
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EPR studies of ferredoxin in spinach and cyanobacterial thylakoids related to photosystem I-driven NADP + reduction
Published in Photosynthesis research (05-03-2024)“…Photosynthetic light-dependent reactions occur in thylakoid membranes where embedded proteins capture light energy and convert it to chemical energy in the…”
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Spin-Correlated Radical Pairs as Quantum Sensors of Bidirectional ET Mechanisms in Photosystem I
Published in The journal of physical chemistry. B (05-09-2019)“…Following light-generated electron transfer reactions in photosynthetic reaction center proteins, an entangled spin qubit (radical) pair is created. The…”
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Z-scheme solar water splitting via self-assembly of photosystem I-catalyst hybrids in thylakoid membranes
Published in Chemical science (Cambridge) (07-12-2018)“…Nature's solar energy converters, the Photosystem I (PSI) and Photosystem II (PSII) reaction center proteins, flawlessly manage photon capture and conversion…”
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Structure of a biohybrid photosystem I-platinum nanoparticle solar fuel catalyst
Published in Nature communications (04-11-2024)“…Biohybrid solar fuel catalysts leverage natural light-driven enzymes to produce valuable fuel products. One useful biological platform for such a system is…”
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Light-driven hydrogen production from Photosystem I-catalyst hybrids
Published in Current opinion in chemical biology (01-04-2015)“…•Sunlight is a clean and abundant source of energy.•New materials are needed to capture, convert, and store the sun's energy.•Nature's solar energy converters…”
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Coherences of Photoinduced Electron Spin Qubit Pair States in Photosystem I
Published in The journal of physical chemistry. B (30-11-2023)“…This publication presents the first comprehensive experimental study of electron spin coherences in photosynthetic reaction center proteins, specifically…”
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Theoretical examination of nuclear spin diffusion in light-induced spin coherences in photosystem I
Published in Applied physics letters (22-01-2024)“…Microsecond coherence times are predicted in spin dynamics calculations of a donor–acceptor electron spin pair P+A1A− created upon light excitation of…”
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EPR Spin-Trapping for Monitoring Temporal Dynamics of Singlet Oxygen during Photoprotection in Photosynthesis
Published in Biochemistry (Easton) (07-05-2024)“…A central goal of photoprotective energy dissipation processes is the regulation of singlet oxygen (1O2*) and reactive oxygen species in the photosynthetic…”
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Resolution of Electronic and Structural Factors Underlying Oxygen-Evolving Performance in Amorphous Cobalt Oxide Catalysts
Published in Journal of the American Chemical Society (29-08-2018)“…Non-noble-metal, thin-film oxides are widely investigated as promising catalysts for oxygen evolution reactions (OER). Amorphous cobalt oxide films…”
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Protein Delivery of a Ni Catalyst to Photosystem I for Light-Driven Hydrogen Production
Published in Journal of the American Chemical Society (11-09-2013)“…The direct conversion of sunlight into fuel is a promising means for the production of storable renewable energy. Herein, we use Nature’s specialized…”
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Light-Induced Charge Separation in Photosystem I from Different Biological Species Characterized by Multifrequency Electron Paramagnetic Resonance Spectroscopy
Published in International journal of molecular sciences (26-07-2024)“…Photosystem I (PSI) serves as a model system for studying fundamental processes such as electron transfer (ET) and energy conversion, which are not only…”
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In Vitro Encapsulation of Functionally Active Abiotic Photosensitizers Inside a Bacterial Microcompartment Shell
Published in The journal of physical chemistry letters (08-08-2024)“…Bacterial microcompartments (BMCs) are self-assembling, selectively permeable protein shells that encapsulate enzymes to enhance catalytic efficiency of…”
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Biohybrid photosynthetic charge accumulation detected by flavin semiquinone formation in ferredoxin-NADP reductase
Published in Chemical science (Cambridge) (07-06-2022)“…Flavin chemistry is ubiquitous in biological systems with flavoproteins engaged in important redox reactions. In photosynthesis, flavin cofactors are used as…”
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D‐Band EPR and ENDOR Spectroscopy of 15N‐Labeled Photosystem I
Published in Applied magnetic resonance (01-09-2022)“…For billions of years, nature has optimized the photosynthetic machinery that converts light energy into chemical energy. Key primary reactions of…”
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Directionality of Electron Transfer in Type I Reaction Center Proteins: High-Frequency EPR Study of PS I with Removed Iron–Sulfur Centers
Published in The journal of physical chemistry. B (29-10-2015)“…A key step of photosynthetic solar energy conversion involves rapid light-induced sequential electron-transfer steps that result in the formation of a…”
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Photocatalytic Hydrogen Production from Noncovalent Biohybrid Photosystem I/Pt Nanoparticle Complexes
Published in The journal of physical chemistry letters (03-02-2011)“…A photocatalytic hydrogen-evolving system based on intermolecular electron transfer between native Photosystem I (PSI) and electrostatically associated Pt…”
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