Search Results - "Solá, Ignacio R."
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Ultrafast photodissociation assisted by strong non-resonant Stark effect: the 'straddling' control pulse
Published in Journal of modern optics (20-03-2009)“…Control of the ultrashort photodissociation dynamics of a diatomic molecule on different excitation channels is investigated by Stark shift with a strong and…”
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2
Optimal protocols for entangling gates in N-qubit atomic systems
Published in AIP advances (01-11-2023)“…We use a novel optimization procedure that includes the temporal and spatial parameters of the pulses acting on arrays of trapped neutral atoms to prepare…”
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3
High vibrational excitation and bond breaking by generalized Raman ladder climbing
Published in Chemical physics letters (22-06-2001)“…By coherent stimulated non-resonant Raman techniques using chirped pulses, it is possible to invert the population between adjacent vibrational levels in a…”
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4
Absolute control over the quantum yield of a photodissociation reaction mediated by nonadiabatic couplings
Published in Chemical science (Cambridge) (23-08-2024)“…Control of molecular reaction dynamics with laser pulses has been developed in the last decades. Among the different magnitudes whose control has been actively…”
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5
Impact of Early Coherences on the Control of Ultrafast Photodissociation Reactions
Published in The journal of physical chemistry letters (08-02-2024)“…By coherent control, the yield of photodissociation reactions can be maximized, starting in a suitable superposition of vibrational states. In ultrafast…”
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6
Grid-Based Ehrenfest Model To Study Electron–Nuclear Processes
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (15-08-2019)“…The two-dimensional electron–nuclear Schrödinger equation using soft-core Coulomb potentials has been a cornerstone for modeling and predicting the behavior…”
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7
Geometrical Optimization Approach to Isomerization: Models and Limitations
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (02-11-2017)“…We study laser-driven isomerization reactions through an excited electronic state using the recently developed Geometrical Optimization procedure. Our goal is…”
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8
Selective excitation of vibrational states by shaping of light-induced potentials
Published in Physical review letters (13-11-2000)“…In this Letter we describe a method for population transfer using intense, ultrafast laser pulses. The selectivity is accomplished by careful shaping of…”
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9
Molecular events in the light of strong fields: A light-induced potential scenario
Published in International journal of quantum chemistry (15-04-2016)“…A new perspective on how to manipulate molecules by means of very strong laser pulses is emerging with insights from the so‐called light‐induced potentials,…”
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10
Controlling Non-Franck−Condon Transitions: Counterintuitive Schemes of Population Transfer in the Adiabatic and Strong Adiabatic Regimes
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (09-10-2003)“…Vibrationally selective population transfer in electronic transitions involving small Franck−Condon factors is studied by means of two-photon excitation with…”
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11
“Stirred, Not Shaken”: Vibrational Coherence Can Speed Up Electronic Absorption
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (27-08-2015)“…We have recently proposed a laser control scheme for ultrafast absorption in multilevel systems by parallel transfer ( J. Phys. Chem. Lett. 2015, 6, 1724 ). In…”
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12
State-Selective Excitation of Quantum Systems via Geometrical Optimization
Published in Journal of chemical theory and computation (08-09-2015)“…We lay out the foundations of a general method of quantum control via geometrical optimization. We apply the method to state-selective population transfer…”
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13
Ultrafast Population Inversion without the Strong Field Catch: The Parallel Transfer
Published in The journal of physical chemistry letters (07-05-2015)“…Quantum systems with sublevel structures, like molecules, prevent full population inversion from one manifold of sublevels to the other using ultrafast…”
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14
Ultrafast Control of the Internuclear Distance with Parabolic Chirped Pulses
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (22-03-2012)“…Recently, control over the bond length of a diatomic molecule with the use of parabolic chirped pulses was predicted on the basis of numerical calculations…”
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15
Mixed Quantum-Classical Dynamics in the Adiabatic Representation To Simulate Molecules Driven by Strong Laser Pulses
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (22-03-2012)“…The dynamics of molecules under strong laser pulses is characterized by large Stark effects that modify and reshape the electronic potentials, known as…”
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16
Laser control of the RbCs bond
Published in The European physical journal. D, Atomic, molecular, and optical physics (01-06-2017)“…We show numerically that it is possible to control the bond distance of the RbCs dimer and create laser-induced oscillations using a single chirped pulse. The…”
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17
Two-Pulse Control of Large-Amplitude Vibrations in H2
Published in Chemphyschem (10-05-2013)“…A laser‐adiabatic manipulation of the bond (LAMB) scheme using moderately intense fields is proposed to induce and control large‐amplitude oscillations in…”
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18
Optimizing Raman Ladder Climbing: Theory and Application in Na2
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (04-10-2001)“…The theory of vibrational ladder climbing excitation by coherent stimulated nonresonant Raman using chirped laser pulses is developed. We analytically obtain…”
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19
Quantum Wave-Packet Dynamics in Spin-Coupled Vibronic States
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (26-11-2012)“…Extending the Shin–Metiu two-electron Hamiltonian, we construct a new Hamiltonian with effective singlet–triplet couplings. The Born–Oppenheimer electronic…”
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20
Selective creation of maximum coherence in multi-level Λ system
Published in Molecular physics (16-02-2014)“…We consider the creation of the maximum Raman coherence in the six-level Λ system using optimal control theory. Optimal fields are designed for different…”
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