Search Results - "Schülli, Tobias U"
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Identifying Copper Vacancies and Their Role in the CuO Based Photocathode for Water Splitting
Published in Angewandte Chemie International Edition (02-12-2019)“…Metal oxides are an important family of semiconductors for effective photoelectrodes in solar‐to‐chemical energy conversion. Defect engineering, such as…”
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Epitaxial growth of an atom-thin layer on a LiNi0.5Mn1.5O4 cathode for stable Li-ion battery cycling
Published in Nature communications (23-03-2022)“…Transition metal dissolution in cathode active material for Li-based batteries is a critical aspect that limits the cycle life of these devices. Although…”
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Liquid-phase sintering of lead halide perovskites and metal-organic framework glasses
Published in Science (American Association for the Advancement of Science) (29-10-2021)“…Lead halide perovskite (LHP) semiconductors show exceptional optoelectronic properties. Barriers for their applications, however, lie in their polymorphism,…”
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Nanoscale Mapping of the 3D Strain Tensor in a Germanium Quantum Well Hosting a Functional Spin Qubit Device
Published in ACS applied materials & interfaces (18-01-2023)“…A strained Ge quantum well, grown on a SiGe/Si virtual substrate and hosting two electrostatically defined hole spin qubits, is nondestructively investigated…”
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Synchronous Densification and Conductivity Modulation of Nano‐Titanate for Pseudocapacitive Li‐ion Storage
Published in Advanced functional materials (01-03-2024)“…Abstract Nanostructured electrode materials have attracted enormous attention because of their kinetic advantages endorsed by nanoscale regime. Densification…”
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Growth Mechanism and Surface State of CuInS2 Nanocrystals Synthesized with Dodecanethiol
Published in Journal of the American Chemical Society (08-11-2017)“…Ternary metal chalcogenide nanocrystals (NCs) offer exciting opportunities as novel materials to be explored on the nanoscale showing optoelectronic properties…”
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Unveiling Core–Shell Structure Formation in a Ni3Fe Nanoparticle with In Situ Multi-Bragg Coherent Diffraction Imaging
Published in ACS nano (28-05-2024)“…Solid-state reactions play a key role in materials science. The evolution of the structure of a single 350 nm Ni3Fe nanoparticle, i.e., its morphology (facets)…”
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Capturing Catalyst Strain Dynamics during Operando CO Oxidation
Published in ACS nano (15-07-2024)“…Understanding the strain dynamic behavior of catalysts is crucial for the development of cost-effective, efficient, stable, and long-lasting catalysts. Using…”
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High‐Voltage Spinel Cathode Materials: Navigating the Structural Evolution for Lithium‐Ion Batteries
Published in Advanced materials (Weinheim) (01-07-2024)“…High‐voltage LiNi0.5Mn1.5O4 (LNMO) spinel oxides are highly promising cobalt‐free cathode materials to cater to the surging demand for lithium‐ion batteries…”
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Interface Aspects in All‐Solid‐State Li‐Based Batteries Reviewed
Published in Advanced energy materials (01-04-2021)“…Extensive efforts have been made to improve the Li‐ionic conductivity of solid electrolytes (SE) for developing promising all‐solid‐state Li‐based batteries…”
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Imaging the strain evolution of a platinum nanoparticle under electrochemical control
Published in Nature materials (01-06-2023)“…Surface strain is widely employed in gas phase catalysis and electrocatalysis to control the binding energies of adsorbates on active sites. However, in situ…”
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Nanoconfined Topochemical Conversion from MXene to Ultrathin Non‐Layered TiN Nanomesh toward Superior Electrocatalysts for Lithium‐Sulfur Batteries
Published in Small (Weinheim an der Bergstrasse, Germany) (01-08-2021)“…2D non‐layered materials (2DNLMs) featuring massive undercoordinated surface atoms and obvious lattice distortion have shown great promise in…”
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13
Impact of dual-layer solid-electrolyte interphase inhomogeneities on early-stage defect formation in Si electrodes
Published in Nature communications (01-07-2020)“…While intensive efforts have been devoted to studying the nature of the solid-electrolyte interphase (SEI), little attention has been paid to understanding its…”
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14
Twin boundary migration in an individual platinum nanocrystal during catalytic CO oxidation
Published in Nature communications (10-09-2021)“…At the nanoscale, elastic strain and crystal defects largely influence the properties and functionalities of materials. The ability to predict the structural…”
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Microstructure of Methylammonium Lead iodide Perovskite Thin Films: A Comprehensive Study of the Strain and Texture
Published in Advanced energy materials (01-05-2022)“…Controlling the microstructure of hybrid halide perovskite thin films is essential for optimizing their performance in optoelectronic devices. It is well…”
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Facet‐Dependent Strain Determination in Electrochemically Synthetized Platinum Model Catalytic Nanoparticles
Published in Small (Weinheim an der Bergstrasse, Germany) (01-05-2021)“…Studying model nanoparticles is one approach to better understand the structural evolution of a catalyst during reactions. These nanoparticles feature…”
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Bragg coherent diffraction imaging with the CITIUS charge‐integrating detector
Published in Journal of applied crystallography (01-08-2023)“…The CITIUS detector is a next‐generation high‐speed X‐ray imaging detector. It has integrating‐type pixels and is designed to show a consistent linear response…”
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The catalytic activity of KMoCo carbon spheres for higher alcohols synthesis from syngas
Published in Applied catalysis. A, General (05-09-2020)“…[Display omitted] •Bimetallic molybdenum-cobalt carbon spheres were prepared via in situ hydrothermal reduction using glucose.•The synergistic interaction…”
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Inversion Domain Boundaries in GaN Wires Revealed by Coherent Bragg Imaging
Published in ACS nano (22-09-2015)“…Interfaces between polarity domains in nitride semiconductors, the so-called Inversion Domain Boundaries (IDB), have been widely described, both theoretically…”
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Towards a quantitative determination of strain in Bragg Coherent X-ray Diffraction Imaging: artefacts and sign convention in reconstructions
Published in Scientific reports (22-11-2019)“…Bragg coherent X-ray diffraction imaging (BCDI) has emerged as a powerful technique to image the local displacement field and strain in nanocrystals, in three…”
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