Search Results - "Novoderezhkin, Vladimir I."
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Quantum design of photosynthesis for bio-inspired solar-energy conversion
Published in Nature (London) (16-03-2017)“…Photosynthesis is the natural process that converts solar photons into energy-rich products that are needed to drive the biochemistry of life. Two ultrafast…”
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Quantum coherence in photosynthesis for efficient solar-energy conversion
Published in Nature physics (01-09-2014)“…The crucial step in the conversion of solar to chemical energy in photosynthesis takes place in the reaction centre, where the absorbed excitation energy is…”
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Physical origins and models of energy transfer in photosynthetic light-harvesting
Published in Physical chemistry chemical physics : PCCP (01-01-2010)“…We perform a quantitative comparison of different energy transfer theories, i.e. modified Redfield, standard and generalized Förster theories, as well as…”
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How exciton-vibrational coherences control charge separation in the photosystem II reaction center
Published in Physical chemistry chemical physics : PCCP (01-01-2015)“…In photosynthesis absorbed sun light produces collective excitations (excitons) that form a coherent superposition of electronic and vibrational states of the…”
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Both electronic and vibrational coherences are involved in primary electron transfer in bacterial reaction center
Published in Nature communications (25-02-2019)“…Understanding the mechanism behind the near-unity efficiency of primary electron transfer in reaction centers is essential for designing performance-enhanced…”
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Energy transfer in photosynthesis: experimental insights and quantitative models
Published in Physical chemistry chemical physics : PCCP (21-02-2006)“…We overview experimental and theoretical studies of energy transfer in the photosynthetic light-harvesting complexes LH1, LH2, and LHCII performed during the…”
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Vibronic Coherence in the Charge Separation Process of the Rhodobacter sphaeroides Reaction Center
Published in The journal of physical chemistry letters (19-04-2018)“…Two-dimensional electronic spectroscopy was applied to a variant of the reaction center (RC) of purple bacterium Rhodobacter sphaeroides lacking the primary…”
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Dark States in the Light-Harvesting complex 2 Revealed by Two-dimensional Electronic Spectroscopy
Published in Scientific reports (09-02-2016)“…Energy transfer and trapping in the light harvesting antennae of purple photosynthetic bacteria is an ultrafast process, which occurs with a quantum efficiency…”
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The Role of Resonant Vibrations in Electronic Energy Transfer
Published in Chemphyschem (04-05-2016)“…Nuclear vibrations play a prominent role in the spectroscopy and dynamics of electronic systems. As recent experimental and theoretical studies suggest, this…”
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Multiple Charge-Separation Pathways in Photosystem II: Modeling of Transient Absorption Kinetics
Published in Chemphyschem (25-02-2011)“…We explain the transient absorption kinetics (E. Romero, I. H. M. van Stokkum, V. I. Novoderezhkin, J. P. Dekker, R. van Grondelle, Biochemistry 2010, 49,…”
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The nature of coherences in the B820 bacteriochlorophyll dimer revealed by two-dimensional electronic spectroscopy
Published in Physical chemistry chemical physics : PCCP (01-01-2014)“…Light-harvesting in photosynthesis is determined by the excitonic interactions in disordered antennae and the coupling of collective electronic excitations to…”
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Two Different Charge Separation Pathways in Photosystem II
Published in Biochemistry (Easton) (25-05-2010)“…Charge separation is an essential step in the conversion of solar energy into chemical energy in photosynthesis. To investigate this process, we performed…”
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Conformational Switching in a Light-Harvesting Protein as Followed by Single-Molecule Spectroscopy
Published in Biophysical journal (02-06-2015)“…Among the ultimate goals of protein physics, the complete, experimental description of the energy paths leading to protein conformational changes remains a…”
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Quantum – coherent dynamics in photosynthetic charge separation revealed by wavelet analysis
Published in Scientific reports (06-06-2017)“…Experimental/theoretical evidence for sustained vibration-assisted electronic (vibronic) coherence in the Photosystem II Reaction Center (PSII RC) indicates…”
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Dynamics of the Emission Spectrum of a Single LH2 Complex: Interplay of Slow and Fast Nuclear Motions
Published in Biophysical journal (15-04-2006)“…We have studied the relationship between the realizations of static disorder and the emission spectra observed for a single LH2 complex. We show that the…”
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Resonant vibrations produce quantum bridge over high-energy states in heterogeneous antenna
Published in Photosynthesis research (01-10-2023)“…Photosynthetic light-harvesting complexes usually contain several pools of molecules with a big difference in transition energies, for example, chlorophylls a…”
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Energy-Transfer Dynamics in the LHCII Complex of Higher Plants: Modified Redfield Approach
Published in The journal of physical chemistry. B (22-07-2004)“…We have modeled energy-transfer dynamics in the peripheral plant light-harvesting complex LHCII using both standard Redfield theory and its modification for…”
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The location of the low-energy states in Lhca1 favors excitation energy transfer to the core in the plant PSI-LHCI supercomplex
Published in Photosynthesis research (01-04-2023)“…Lhca1 is one of the four pigment-protein complexes composing the outer antenna of plant Photosystem I-light-havesting I supercomplex (PSI-LHCI). It forms a…”
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Dynamics of Exciton Relaxation in LH2 Antenna Probed by Multipulse Nonlinear Spectroscopy
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (28-04-2011)“…We explain the relaxation dynamics in the LH2-B850 antenna as revealed by multipulse pump−dump−probe spectroscopy ( Th. A. Cohen Stuart, M. Vengris, V. I…”
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Direct Visualization of Exciton Reequilibration in the LH1 and LH2 Complexes of Rhodobacter sphaeroides by Multipulse Spectroscopy
Published in Biophysical journal (04-05-2011)“…The dynamics of the excited states of the light-harvesting complexes LH1 and LH2 of Rhodobacter sphaeroides are governed, mainly, by the excitonic nature of…”
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