Search Results - "Mausolf, Edward"
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Hybridised production of technetium-99m and technetium-101 with fluorine-18 on a low-energy biomedical cyclotron
Published in EPJ techniques and instrumentation (10-02-2023)“…New modes of production and supply of short-lived radioisotopes using accelerators are becoming attractive alternatives to the use of nuclear reactors. In this…”
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Fusion-Based Neutron Generator Production of Tc-99m and Tc-101: A Prospective Avenue to Technetium Theranostics
Published in Pharmaceuticals (Basel, Switzerland) (29-08-2021)“…Presented are the results of 99mTc and 101Tc production via neutron irradiation of natural isotopic molybdenum (Mo) with epithermal/resonance neutrons…”
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Discovery, nuclear properties, synthesis and applications of technetium-101
Published in Communications chemistry (20-10-2022)“…Technetium-101 ( 101 Tc) has been poorly studied in comparison with other Tc isotopes, although it was first identified over ~80 years ago shortly after the…”
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Time-Resolved Infrared Reflectance Studies of the Dehydration-Induced Transformation of Uranyl Nitrate Hexahydrate to the Trihydrate Form
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (01-10-2015)“…Uranyl nitrate is a key species in the nuclear fuel cycle. However, this species is known to exist in different states of hydration, including the hexahydrate…”
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Nanostructure of metallic particles in light water reactor used nuclear fuel
Published in Journal of nuclear materials (01-06-2015)“…[Display omitted] •An extraordinary nano-structure has been observed in the noble metal particles that form in UO2 reactor fuels.•The composition of the…”
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Sequestration of radioactive iodine in silver-palladium phases in commercial spent nuclear fuel
Published in Journal of nuclear materials (15-12-2016)“…Radioactive iodine is the Achilles' heel in the design for the safe geological disposal of spent uranium oxide (UO2) nuclear fuel. Furthermore, iodine's high…”
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Separation of metallic residues from the dissolution of a high-burnup BWR fuel using nitrogen trifluoride
Published in Journal of fluorine chemistry (01-06-2014)“…Selective separation of volatiles: Mo, Tc, and Ru, from nanoparticulate noble metal (hcp) phase using NF3 and the non-volatile residue; acicular, micron…”
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Conditions for Critical Effects in the Mass Action Kinetics Equations for Water Radiolysis
Published in The journal of physical chemistry. A, Molecules, spectroscopy, kinetics, environment, & general theory (26-12-2014)“…We report on a subtle global feature of the mass action kinetics equations for water radiolysis that results in predictions of a critical behavior in H2O2 and…”
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Chemical stabilization of Hanford tank residual waste
Published in Journal of nuclear materials (01-03-2014)“…Three different chemical treatment methods were tested for their ability to stabilize residual waste from Hanford tank C-202 for reducing contaminant release…”
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Hexaammine-cobalt(III) pertechnetate: preparation, structure and solubility
Published in Journal of radioanalytical and nuclear chemistry (2017)“…A new pertechnetate salt, [Co(NH 3 ) 6 ][TcO 4 ] 3 ·2H 2 O, was prepared from the reaction of NH 4 TcO 4 and [Co(NH 3 ) 6 ]Cl 3 in water. The [Co(NH 3 ) 6…”
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Sequestration of radioactive iodine in silver-palladium phases in commercial spent nuclear fuel
Published in Journal of nuclear materials (01-12-2016)Get full text
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Technetium Chemistry in the Fuel Cycle: Combining Basic and Applied Studies
Published in Inorganic chemistry (01-04-2013)“…Technetium is intimately linked with nuclear reactions. The ultraminute natural levels in the environment are due to the spontaneous fission of uranium…”
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Nanostructure of metallic particles in light water reactor used nuclear fuel
Published in Journal of nuclear materials (01-06-2015)Get full text
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Chemical stabilization of Hanford tank residual waste
Published in Journal of nuclear materials (29-04-2016)Get full text
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Synthesis, Structure Elucidation, and Redox Properties of [superscript 99]Tc Complexes of Lacunary Wells-Dawson Polyoxometalates: Insights into Molecular [superscript 99]Tc-Metal Oxide Interactions
Published in Inorganic chemistry (17-11-2011)“…The isotope {sup 99}Tc ({beta}{sub max}, 293.7; half-life, 2.1 x 10{sup 5} years) is an abundant product of uranium-235 fission in nuclear reactors and is…”
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Technetium Chemistry in the Fuel Cycle: Combining Basic and Applied Studies
Published in Inorganic chemistry (28-06-2012)“…Technetium is intimately linked with nuclear reactions. The ultraminute natural levels in the environment are due to the spontaneous fission of uranium…”
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Separation of Pertechnetate from Uranium in a Simulated UREX Processing Solution Using Anion Exchange Extraction Chromatography
Published in Solvent extraction and ion exchange (01-07-2013)“…A process to separate technetium from uranium in a simulated process solution resulting from the uranium extraction (UREX) process was demonstrated using a new…”
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Spectroscopic and structural characterization of reduced technetium species in acetate media
Published in Journal of radioanalytical and nuclear chemistry (01-06-2011)“…The reduction of ammonium pertechnetate by sodium borohydride in 0.1 M NaOH/glacial acetic acid has been studied. The reduction products (solids and solutions)…”
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Formation of Tc metal in 12 M HCl using Zn as a reductant
Published in Journal of radioanalytical and nuclear chemistry (01-11-2013)“…Amorphous TcO 2 and NH 4 TcO 4 solubilized into 12 M HCl will spontaneously convert to hexachlorotechnetate (TcCl 6 2− ). This process is accelerated upon…”
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