Risk assessment due to natural radioactivity of stone dust and crushed stone Commercialized in construction stores in the state of Rio de Janeiro

A systematic study of the distribution of the Naturally Occurring Radioactivity in stone dust and crushed stone, has been carried out with an objective of establishing reliable baseline data on the radiation level and hence to evaluate hazard indices approach and the production of radioactive heat (...

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Published in:Applied radiation and isotopes Vol. 210; p. 111366
Main Authors: Silva, Leandro Barbosa, Faria da Silva, Lucas, Orejuela, Carlos Omar Pastrana, Mattos Barbosa, Caroline, Marzullo, Fernando Luiz, Monteiro de Lima, Alan Miranda, Silva, Ademir Xavier da
Format: Journal Article
Language:English
Published: England Elsevier Ltd 01-08-2024
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Summary:A systematic study of the distribution of the Naturally Occurring Radioactivity in stone dust and crushed stone, has been carried out with an objective of establishing reliable baseline data on the radiation level and hence to evaluate hazard indices approach and the production of radioactive heat (RHP) due to radiation exposure to the workers and to the inhabitants of the studied area. Twenty-six samples have been collected from different locations in the State of Rio de Janeiro (Brazil). To calculate the specific activity, gamma ray spectrometry and a detector of High Purity Germanium (HPGe; Canberra, 30% relative efficiency) was used. The activity concentration of 238U, 226Ra 232Th and 40K ranged from 29.3 ± 18.6 to 206.8 ± 21.5 Bq kg−1, 30.3 ± 1.0 to 134.3 ± 1.8, 27.9 ± 0.7 to 86.2 ± 0.9 Bq kg−1, and 734.9 ± 35.1 to 1204.8 ± 53.5 Bq kg−1, respectively. The mean values of the Iex, Iin, Iγ, Iα, AUI, IRP112Rn, IPA, IPI and IYu indices were 0.68 ± 0.09, 0.92 ± 0.12, 0.93 ± 0.12, 0.43 ± 0.07, 0.88 ± 0.20, 1.25 ± 0.21, 0.34 ± 0.05, 0.75 ± 0.10, 0.63 ± 0.08 and 34. ± 6.31, respectively. The average radioactive heat production (RHP) of 2.01 ± 0.28 μ Wm−3 was above the values found in the literature, which may contribute to the heat flow in the study area because the raw materials that make up the samples showed a high value of environmental radioactivity. The Brazilian Hazard Index to assess the radiological risk of crushed stone and stone dust was created and the average value was 0.74 ± 0.10, a value below 1, which means only moderate control over the use of these materials, with no indication of restriction to the its use. •High-res gamma spectrometer measured levels of natural radionuclides in stone dust, crushed stone.•Study assesses radionuclide exposure risks in building materials, safety for workers & residents.•Research helps build database to minimize ionizing radiation damage, inform public policy.•A Brazilian Risk Index for samples was created to better adapt to the reality of using these materials in Brazil.
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ISSN:0969-8043
1872-9800
DOI:10.1016/j.apradiso.2024.111366